-
Caged AIEgens: Multicolor and White Emission Triggered by Mechanical Activation J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-22 Yunyan Sun, Kecheng Wang, Xiao Huang, Shixuan Wei, Enrique Contreras, Prashant K. Jain, Luis M. Campos, Heather J. Kulik, Jeffrey S. Moore
-
Facet-Engineered BiVO4 Photocatalysts for Water Oxidation: Lifetime Gain Versus Energetic Loss J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-21 Tianhao He, Yue Zhao, Daniele Benetti, Benjamin Moss, Lei Tian, Shababa Selim, Rengui Li, Fengtao Fan, Qian Li, Xiuli Wang, Can Li, James R. Durrant
-
Unlocking Lattice Oxygen on Selenide-Derived NiCoOOH for Amine Electrooxidation and Efficient Hydrogen Production J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-21 Long Chen, Zhao-Hua Yin, Jun-Yuan Cui, Chao-Qun Li, Kepeng Song, Hong Liu, Jian-Jun Wang
-
Surfactant-Free Preparation of Conjugated Polymer Nanoparticles in Aqueous Dispersions Using Sulfate Functionalized Fluorene Monomers J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Marcin Gwiazda, Benjamin J. Lidster, Charlotte Waters, Jaruphat Wongpanich, Michael L. Turner
-
Hydride Transfer-Based CO2 Reduction Catalysis: Navigating Metal Hydride to Organic Hydride in the Catalytic Loop Acc. Chem. Res. (IF 16.4) Pub Date : 2024-09-18 Joyanta Choudhury, Ritu Bhardwaj, Sanajit Kumar Mandal
-
Ligand-Controlled Regiodivergent Ring Expansion of Benzosilacyclobutenes with Alkynes en Route to Axially Chiral Silacyclohexenyl Arenes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-21 Xiaoxiao Tang, Yulang Tang, Ju Peng, Huimin Du, Liying Huang, Jiahui Gao, Shiyang Liu, Dongxu Wang, Wanshu Wang, Lu Gao, Yu Lan, Zhenlei Song
-
Concise and Efficient Synthesis of Sequentially Isomeric Hetero[3]rotaxanes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-21 Christopher K. Lee, Yuanning Feng, Mohammad Tajik, Jake P. Violi, William A. Donald, J. Fraser Stoddart, Dong Jun Kim
-
When van der Waals Met Kagome: A 2D Antimonide with a Vanadium-Kagome Network J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-21 Aishwarya Mantravadi, Bradyn C. Weaver, Shiya Chen, Shahnaz Mukta, Yao Abusa, Arka Sarkar, Yang Sun, Yaroslav Mudryk, Alexander Gundlach-Graham, Kai-Ming Ho, Oleg I. Lebedev, Julia V. Zaikina
-
(Z)-Selective Isomerization of 1,1-Disubstituted Alkenes by Scandium-Catalyzed Allylic C–H Activation J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Shao-Jie Lou, Pan Wang, Xin Wen, Aniket Mishra, Xuefeng Cong, Qingde Zhuo, Kun An, Masayoshi Nishiura, Yi Luo, Zhaomin Hou
-
Distortion Engineering: A Strategy to Modulate Molecular Upconversion with Molecular Cluster-Aggregates J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Diogo A. Gálico, Alexandros A. Kitos, Rayan Ramdani, Jeffrey S. Ovens, Muralee Murugesu
-
Engineering Screw Dislocations in Covalent Organic Frameworks J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Bhausaheb Dhokale, Kira Coe-Sessions, Michael J. Wenzel, Alathea E. Davies, Taylor Kelsey, Jonathan A. Brant, Laura de Sousa Oliveira, Bruce A. Parkinson, John O. Hoberg
-
Photocatalytic Acetylene Hydrochlorination by Pairing Proton Reduction and Chlorine Oxidation over g-C3N4/BiOCl Catalysts J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Zhi-Hao Zhao, Huan Wang, Jinjin Li, Xingyue Qiao, Zhenpeng Liu, Zhipeng Ren, Menglei Yuan, Jian Zhang
-
Integrated CO2 Capture and Conversion by a Robust Cu(I)-Based Metal–Organic Framework J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Debabrata Sengupta, Saptasree Bose, Xiaoliang Wang, Neil M. Schweitzer, Christos D. Malliakas, Haomiao Xie, Joshua Duncan, Kent O. Kirlikovali, Taner Yildirim, Omar K. Farha
-
Aldehyde–Olefin Couplings Via Sulfoxylate-Mediated Oxidative Generation of Ketyl Radical Anions J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Zhihang Li, Joseph A. Tate, Adam Noble
-
Efficient Strategy to Discover DNA Aptamers Against Low Abundance Cell Surface Proteins in Scarce Samples J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Xiaoqiu Wu, Yuqing Liu, Dengwei Zhang, Jingjing Yu, Mingxin Zhang, Shuwei Feng, Lifei Zhang, Ting Fu, Yamin Tan, Tao Bing, Weihong Tan
-
Manipulating d-Band Center of Nickel by Single-Iodine-Atom Strategy for Boosted Alkaline Hydrogen Evolution Reaction J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Chongjing Liu, Beibei Sheng, Quan Zhou, Yujian Xia, Ying Zou, Peter Joseph Chimtali, Dengfeng Cao, Yongheng Chu, Sirui Zhao, Ran Long, Shuangming Chen, Li Song
-
Catalyst-Free Oxidation of Styrene to Styrene Oxide Using Circulating Microdroplets in an Oxygen Atmosphere J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Lian Xue, Weida Chen, Peng Zheng, Jiao Geng, Feng Zhang, Xinyao Li, Zhibing Zhang, Xingbang Hu
-
Chemically Separable Co(II) Spin-State Isomers J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Amelia M. Wheaton, Jill A. Chipman, Rebecca K. Walde, Heike Hofstetter, John F. Berry
-
Enhancing the Acidity Window of Zeolites by Low-Temperature Template Oxidation with Ozone J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Julien Devos, Vitaly L. Sushkevich, Ibrahim Khalil, Sven Robijns, Rodrigo de Oliveira-Silva, Dimitrios Sakellariou, Jeroen van Bokhoven, Michiel Dusselier
-
Revealing the Bro̷nsted Acidic Nature of Penta-Coordinated Aluminum Species in Dealuminated Zeolite Y with Solid-State NMR Spectroscopy J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mingji Zheng, Qiang Wang, Yueying Chu, Xuechao Tan, Weidong Huang, Yujie Xi, Yongxiang Wang, Guodong Qi, Jun Xu, Suk Bong Hong, Feng Deng
-
Tautomer-Selective Fluorescence Spectroscopy of Oxyluciferin Anions J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Iden Djavani-Tabrizi, Thomas Toft Lindkvist, Jeppe Langeland, Christina Kjær, Marlowe Graham, Henrik G. Kjaergaard, Steen Brøndsted Nielsen
-
Repetitive Rolling of Triptycene-Based Molecules on Cu Surfaces J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mine Konuk, Melihat Madran, Mehmet Tuna Uysal, Deniz Beşer, Alimet Sema Özen, Zehra Akdeniz, Sondan Durukanoğlu
-
Modulating Decarboxylative Oxidation Photocatalysis by Ligand Engineering of Atomically Precise Copper Nanoclusters J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mohammad Bodiuzzaman, Kathiravan Murugesan, Peng Yuan, Bholanath Maity, Arunachalam Sagadevan, Naveen Malenahalli H, Song Wang, Partha Maity, Mohammed F. Alotaibi, De-en Jiang, Mutalifu Abulikemu, Omar F. Mohammed, Luigi Cavallo, Magnus Rueping, Osman M. Bakr
-
Anionic Ionomer: Released Surface-Immobilized Cations and an Established Hydrophobic Microenvironment for Efficient and Durable CO2-to-Ethylene Electrosynthesis at High Current over One Month J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mingwei Fang, Xiang Miao, Zihao Huang, Meiling Wang, Xiaochen Feng, Zewen Wang, Ying Zhu, Liming Dai, Lei Jiang
-
In Situ Surfaced Mn–Mn Dimeric Sites Dictate CO Hydrogenation Activity and C2 Selectivity over MnRh Binary Catalysts J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Ke-Xiang Zhang, Zhi-Pan Liu
-
Crystal Structure Determination from Powder Diffraction Patterns with Generative Machine Learning J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Eric A. Riesel, Tsach Mackey, Hamed Nilforoshan, Minkai Xu, Catherine K. Badding, Alison B. Altman, Jure Leskovec, Danna E. Freedman
-
Photo- and Electrocatalytic Hydrogen Evolution by Heteroleptic Dirhodium(II,II) Complexes: Role of the Bridging and Diimine Ligands J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Piyush Gupta, Curtis E. Moore, Claudia Turro
-
Formal [2σ + 2σ]-Cycloaddition of Aziridines with Bicyclo[1.1.0]butanes: Access to Enantiopure 2-Azabicyclo[3.1.1]heptane Derivatives J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Shubham Dutta, Constantin G. Daniliuc, Christian Mück-Lichtenfeld, Armido Studer
-
Correction to “Photoelectrochemical CO2 Reduction to CO Enabled by a Molecular Catalyst Attached to High-Surface-Area Porous Silicon” J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Xiaofan Jia, Eleanor Stewart-Jones, Jose L. Alvarez-Hernandez, Gabriella P. Bein, Jillian L. Dempsey, Carrie L. Donley, Nilay Hazari, Madison N. Houck, Min Li, James M. Mayer, Hannah S. Nedzbala, Rebecca Powers
The original article contained an error in the resistivity of p-type Si wafers on page S2 of the Supporting Information. The sentence should read as follows: “All p-type wafers are B doped, <100>, SSP Prime Grade with an estimated resistance of 1–10 Ω·cm–1.” A complete corrected version of the Supporting Information is presented here. The resistivity of the wafers is correctly listed in the caption
-
Heavy-Atom Tunneling in Ring-Closure Reactions of Beryllium Ozonide Complexes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Yangyu Zhou, Wenbin Fan, Jingjing Tang, Wei Fang, Mingfei Zhou
-
Cavity Manipulation of Attosecond Charge Migration in Conjugated Dendrimers J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Baicheng Zhang, Yonghao Gu, Victor Manuel Freixas, Shichao Sun, Sergei Tretiak, Jun Jiang, Shaul Mukamel
-
Structural Isomerism in Bimetallic Ag20Cu12 Nanoclusters J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Guocheng Deng, Sami Malola, Taeyoung Ki, Xiaolin Liu, Seungwoo Yoo, Kangjae Lee, Megalamane S. Bootharaju, Hannu Häkkinen, Taeghwan Hyeon
-
Rechargeable Mg–Br2 Battery with Ultrafast Bromine Chemistry J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Longyuan Guo, Aosai Chen, Aoxuan Wang, Zhenglin Hu, Haiming Zhang, Jiayan Luo
-
Rapid Characterization of Point Defects in Solid-State Ion Conductors Using Raman Spectroscopy, Machine-Learning Force Fields, and Atomic Raman Tensors J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Willis O’Leary, Manuel Grumet, Waldemar Kaiser, Tomáš Bučko, Jennifer L. M. Rupp, David A. Egger
-
Adaptive Photochemical Amination via Co(II) Catalysis J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Geyang Song, Jiameng Song, Qi Li, Tengfei Kang, Jianyang Dong, Gang Li, Juan Fan, Chao Wang, Dong Xue
-
Ultrasonic Control of Protein Splicing by Split Inteins J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Chuanjiang He, Yu Zhou, Junlin Chen, Rostislav Vinokur, Fabian Kiessling, Andreas Herrmann
-
Metal–Organic Framework Nanofluidic Synapse J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Si-Yuan Yu, Jin Hu, Zheng Li, Yi-Tong Xu, Cheng Yuan, Dechen Jiang, Wei-Wei Zhao
-
Synthesis of Chiral Endocyclic Allenes and Alkynes via Pd-Catalyzed Asymmetric Higher-Order Dipolar Cycloaddition J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Bin Shi, Meng Xiao, Jin-Pu Zhao, Zhihan Zhang, Wen-Jing Xiao, Liang-Qiu Lu
-
Correction to “Terminal Hydride Complex of High-Spin Mn” J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Alex Drena, Addison Fraker, Niklas B. Thompson, Peter E. Doan, Brian M. Hoffman, Alex McSkimming
The following statement was omitted from the Acknowledgments: This work was supported by the NSF, Grant CHE-2333907, and the NIH, Grant GM111097 to B.M.H. This article has not yet been cited by other publications.
-
Uncovering the Pathway of Serine Octamer Magic Number Cluster Formation during Electrospray Ionization: Experiments and Simulations J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Vida Alinezhad, Yuen Ki Ng, Sanvid Mehta, Lars Konermann
-
A Bioorthogonal Precision Tool for Human N-Acetylglucosaminyltransferase V J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Yu Liu, Ganka Bineva-Todd, Richard W. Meek, Laura Mazo, Beatriz Piniello, Olga Moroz, Sean A. Burnap, Nadima Begum, André Ohara, Chloe Roustan, Sara Tomita, Svend Kjaer, Karen Polizzi, Weston B. Struwe, Carme Rovira, Gideon J. Davies, Benjamin Schumann
-
Oxadiazolines as Photoreleasable Labels for Drug Target Identification J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Corentin Bon, Benedikt Goretzki, Marie Flamme, Claude Shelton, Holly Davis, Fabio Lima, Francisco Garcia, Scott Brittain, Cara E. Brocklehurst
-
Revealing the Chemical and Structural Complexity of Electrochemical Ion Exchange in Layered Oxide Materials J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Linqin Mu, Dong Hou, Emily E. Foley, Minyi Dai, Jin Zhang, Zhisen Jiang, Muhammad Mominur Rahman, Yanbao Fu, Lu Ma, Enyuan Hu, Sami Sainio, Dennis Nordlund, Jue Liu, Jia-Mian Hu, Yijin Liu, Raphaële J. Clément, Feng Lin
-
Covalent Probes To Capture Legionella pneumophila Dup Effector Enzymes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Max S. Kloet, Rishov Mukhopadhyay, Rukmini Mukherjee, Mohit Misra, Minwoo Jeong, Cami M. P. Talavera Ormeño, Angeliki Moutsiopoulou, Rayman T. N. Tjokrodirijo, Peter A. van Veelen, Donghyuk Shin, Ivan Đikić, Aysegul Sapmaz, Robbert Q. Kim, Gerbrand J. van der Heden van Noort
-
Enantioselective Decarboxylative C(sp3)-C(sp3) Cross-Coupling of Aliphatic Redox-Active Esters with gem-Borazirconocene Alkanes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Jing Wang, Songlin Bai, Chao Yang, Xiangbing Qi
-
Development of a Deactivation-Resistant Dialkylbiarylphosphine Ligand for Pd-Catalyzed Arylation of Secondary Amines J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Kaibo Feng, Elaine Reichert Raguram, James R. Howard, Ellyn Peters, Cecilia Liu, Matthew S. Sigman, Stephen L. Buchwald
-
A Transient Iron Carbide Generated by Cyaphide Cleavage J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Duleeka C. Wannipurage, Eric S. Yang, Austin D. Chivington, Jess Fletcher, Debanik Ray, Nobuyuki Yamamoto, Maren Pink, Jose M. Goicoechea, Jeremy M. Smith
-
Photoexcited Copper-Catalyzed Enantioselective Allylic C(sp3)–H Acyloxylation of Acyclic Internal Alkenes J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-17 Sheng Tang, Hui Xu, Yanfeng Dang, Shouyun Yu
-
Mechanistic Understanding of the Underlying Energy Storage Mechanism of α-MnO2-based Pseudo-Supercapacitors Adv. Mater. (IF 27.4) Pub Date : 2024-09-20 Lei Deng, Zaifa Wang, Hantao Cui, Yunna Guo, Zhangran Ye, Hui Li, Xinyu Zhang, Peng Jia, Qiaobao Zhang, Liqiang Zhang
-
Unveiling the Unique Reactivity of Anionic Mn(I) Complexes via Metal–Ligand Cooperation: Nucleophilic Attack on C(sp3)–X Bonds J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Hengxu Li, Mingjie Fan, Qiang Liu
-
Visualizing Triplet Energy Transfer in Organic Near-Infrared Phosphorescent Host-Guest Materials Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Zihao Deng, Fan-Cheng Kong, Ziqi Deng, Jiaming Zhou, Shengyi Yang, Shan He, Jianyu Zhang, Yunfei Zuo, Jin Wang, Xinmeng Chen, Ryan T. K. Kwok, Guocheng Jia, Philip C. Y. Chow, David Lee Phillips, Parvej Alam, Jacky W. Y. Lam, Ben Zhong Tang
Limited by the energy gap law, purely organic materials with efficient near-infrared room temperature phosphorescence are rare and difficult to achieve. Additionally, the exciton transition process among different emitting species in host-guest phosphorescent materials remains elusive, presenting a significant academic challenge. Herein, using a modular nonbonding orbital-π bridge-nonbonding orbital
-
Metal-N Coordination in Lithium-Sulfur Batteries: Inhibiting Catalyst Passivation Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Xin Ao, Yang Kong, Shangquan Zhao, Zhongxin Chen, Yong Li, Xingyu Liao, Bingbing Tian
Lithium-sulfur (Li-S) batteries exhibit great potential as the next-generation energy storage techniques. Application of catalyst is widely adopted to accelerate the redox kinetics of polysulfide conversion reactions and improve battery performance. Although significant attention has been devoted to seeking new catalysts, the problem of catalyst passivation remains underexplored. Herein, we find that
-
Harnessing the Unconventional Cubic Phase in 2D LaNiO3 Perovskite for Highly Efficient Urea Oxidation Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Zhiao Wu, Miao Fan, Huiyu Jiang, Jiao Dai, Kaisi Liu, Rong Hu, Shutong Qin, Weilin Xu, Yonggang Yao, Jun Wan
Phase engineering is a critical strategy in electrocatalysis, as it allows for the modulation of electronic, geometric, and chemical properties to directly influence the catalytic performance. Despite its potential, phase engineering remains particularly challenging in thermodynamically stable perovskites, especially in a 2D structure constraint. Herein, we report phase engineering in 2D LaNiO3 perovskite
-
Nucleophilic Fluoride Anion Delivery from Triazacyclononane-Supported Molecular Ca–F Complexes Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Omar Apolinar, Job J. C. Struijs, Debotra Sarkar, Véronique Gouverneur, Simon Aldridge
The major source of fluoride, namely calcium difluoride (CaF2), is derived from the mineral fluorspar. Recent advances in the activation of CaF2 via mechanochemical methods have inspired investigation of the fundamental properties of Ca–F bonds in molecular complexes. However, the paucity of well-defined molecular Ca–F-containing complexes undermines systematic understanding of the factors governing
-
Quantum Spin Exchange Interactions Trigger O p Band Broadening for Enhanced Aqueous Zinc-Ion Battery Performance Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Shiyu Wang, Shuyun Yao, Feike Zhang, Kang Ji, Yingjie Ji, Jingxian Li, Weijie Fu, Yuanming Liu, Jinghua Yang, Ruilong Liu, Jiangzhou Xie, Zhiyu Yang, Yi-Ming Yan
The pressing demand for large-scale energy storage solutions has propelled the development of advanced battery technologies, among which zinc-ion batteries (ZIBs) are prominent due to their resource abundance, high capacity, and safety in aqueous environments. However, the use of manganese oxide cathodes in ZIBs is challenged by their poor electrical conductivity and structural stability, stemming
-
As Aggregation-Induced Emission Meets with Noncovalent Conformational Locks: Subtly Regulating NIR-II Molecules for Multimodal Imaging-Navigated Synergistic Therapies Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Jiangao Li, Niu Niu, Deliang Wang, Jun Zhu, Xue Li, Qiyu Kong, Ben Zhong Tang, Dong Wang
Phototheranostics is growing into a sparking frontier in disease treatment. Developing single molecular species synchronously featured by powerful absorption capacity, superior second near-infrared (NIR-II) fluorescence and prominent photothermal conversion ability is highly desirable for phototheranostics, yet remains formidably challenging. In this work, we propose a molecular design philosophy that
-
LiLnGeS4 (Ln = La–Nd): Designing High Performance Infrared Nonlinear Optical Sulfides through “Band Reformation of AGS” Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Qian-Qian Liu, Xin Liu, Mei-Ze Li, Rui-Xi Wang, Bingxuan Li, Li-Ming Wu, Ling Chen
AgGaS2 (AGS) is the most commonly used commercial infrared nonlinear optical material. However, AGS has a narrow band gap (Eg = 2.58 eV) and a low laser-induced damage threshold (LIDT), primarily attributed to its mobile liquid-like Ag+ constituent and the unstable Ag–S chemical bond. Herein, we propose a “band reformation of AGS” strategy, which leads to the success syntheses of four lanthanide sulfides
-
Solution-processing induced H-aggregate of Perylene-Diimide Zwitterion Exhibiting Compact Molecular Stacking toward Efficient Cathode Modification in Organic Solar Cells Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Zhi-Guo Zhang, Zhe Li, Yanhe Xiang, Jiayu Li, Luxin Feng, Ming Zhang, Shouke Yan, Bowei Xu
High-performance organic cathode interlayers (CILs) play a crucial role in the advance of organic solar cells (OSCs). However, organic CILs have exhibited inferior performances to their inorganic counterparts over a long time, due to the inherent shortcoming of poor charge transporting capability. Here, we designed and synthesized a perylene-diimide (PDI) zwitterion PDI-B as high-performance organic
-
Disilicon-Mediated Carbon Monoxide Activation: From a 1,2,3-Trisila- to 1,3-Disilacyclopentadienes with Hypercoordinate λ4Si-λ3C Double Bonds Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Matthias Driess, Shenglai Yao, Markus Stefan Budde, Yun Xiong, Xing Yang, Lili Zhao
The facile reaction of the SiPh2-bridged bis-silylene (LSi:)2SiPh2 (L = PhC(NBut)2) with diphenylacetylene affords the unprecedented 1,2,3-trisilacyclopentadiene (LSi)2(PhC)2SiPh2 1 with a hypercoordinate λ4Si-λ3Si double bond. Compound 1 is very oxophilic and consumes three molar equivalents of inert N2O to form the bicyclic oxygenation product 2 through O-atom insertion in the Si=Si and Si-Si bonds
-
Recent Advances of Organic Cocrystals in Emerging Cutting-Edge Properties and Applications Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-21 Xin Wang, Zongrui Wang, Xiang Wang, Fangyuan Kang, Qianfeng Gu, Qichun Zhang
Organic cocrystals, representing one type of new functional materials, have gathered significant interest in various engineering areas. Owing to their diverse stacking modes, rich intermolecular interactions and abundant functional components, the physicochemical properties of organic cocrystals can be tailored to meet different requirements and exhibit novel characteristics. The past few years have