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Amide-Assisted Synthesis of Iron Germanium Sulfide (Fe2GeS4) Nanostars: The Effect of LiN(SiMe3)2 on Precursor Reactivity for Favoring Nanoparticle Nucleation or Growth J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Rebecca C. Miller; James R. Neilson; Amy L. Prieto
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Efficient Ammonia Electrosynthesis from Nitrate on Strained Ruthenium Nanoclusters J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Jie Li; Guangming Zhan; Jianhua Yang; Fengjiao Quan; Chengliang Mao; Yang Liu; Bo Wang; Fengcai Lei; Lejing Li; Alice W. M. Chan; Liangpang Xu; Yanbiao Shi; Yi Du; Weichang Hao; Po Keung Wong; Jianfang Wang; Shi-Xue Dou; Lizhi Zhang; Jimmy C. Yu
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Cerium-Based Metal–Organic Layers Catalyze Hydrogen Evolution Reaction through Dual Photoexcitation J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Yang Song; Yunhong Pi; Xuanyu Feng; Kaiyuan Ni; Ziwan Xu; Justin S. Chen; Zhong Li; Wenbin Lin
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Gold–Carbon Contacts from Oxidative Addition of Aryl Iodides J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Rachel L. Starr; Tianren Fu; Evan A. Doud; Ilana Stone; Xavier Roy; Latha Venkataraman
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Identification of Water Hexamer on Cu(111) Surfaces J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Sai Duan; Igor Ying Zhang; Zhen Xie; Xin Xu
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Enforced Planar FOX-7-like Molecules: A Strategy for Thermally Stable and Insensitive π-Conjugated Energetic Materials J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Yongxing Tang; Wei Huang; Gregory H. Imler; Damon A. Parrish; Jean’ne M. Shreeve
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Synthesis of β-Phenethylamines via Ni/Photoredox Cross-Electrophile Coupling of Aliphatic Aziridines and Aryl Iodides J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Talia J. Steiman; Junyi Liu; Amanuella Mengiste; Abigail G. Doyle
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Discovering Large Isotropic Negative Thermal Expansion in Framework Compound AgB(CN)4 via the Concept of Average Atomic Volume J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Qilong Gao; Jiaqi Wang; Andrea Sanson; Qiang Sun; Erjun Liang; Xianran Xing; Jun Chen
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Homochiral Nickel Nitrite ABX3 (X = NO2–) Perovskite Ferroelectrics J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Bin-Bin Deng; Chu-Chu Xu; Ting-Ting Cheng; Yi-Ting Yang; Yan-Ting Hu; Pan Wang; Wen-Hui He; Meng-Juan Yang; Wei-Qiang Liao
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Host–Guest Allosteric Control of an Artificial Phosphatase J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-06 Joanna Czescik; Yanchao Lyu; Samuele Neuberg; Paolo Scrimin; Fabrizio Mancin
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The Role of Backbone Polarity on Aggregation and Conduction of Ions in Polymer Electrolytes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Nicole S. Schauser; Douglas J. Grzetic; Tarnuma Tabassum; Gabrielle A. Kliegle; My Linh Le; Ethan M. Susca; Ségolène Antoine; Timothy J. Keller; Kris T. Delaney; Songi Han; Ram Seshadri; Glenn H. Fredrickson; Rachel A. Segalman
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The Structural Origins of Intense Circular Dichroism in a Waggling Helicene Nanoribbon J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Nathaniel J. Schuster; Leo A. Joyce; Daniel W. Paley; Fay Ng; Michael L. Steigerwald; Colin Nuckolls
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AgN3-Catalyzed Hydroazidation of Terminal Alkynes and Mechanistic Studies J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Shanshan Cao; Qinghe Ji; Huaizhi Li; Maolin Pang; Haiyan Yuan; Jingping Zhang; Xihe Bi
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Unraveling Reaction Mechanisms of Mo2C as Cathode Catalyst in a Li-CO2 Battery J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Chao Yang; Kunkun Guo; Dingwang Yuan; Jianli Cheng; Bin Wang
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Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Jianwen Liang; Xiaona Li; Shuo Wang; Keegan R. Adair; Weihan Li; Yang Zhao; Changhong Wang; Yongfeng Hu; Li Zhang; Shangqian Zhao; Shigang Lu; Huan Huang; Ruying Li; Yifei Mo; Xueliang Sun
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Reversible Switching between Nonporous and Porous Phases of a New SIFSIX Coordination Network Induced by a Flexible Linker Ligand J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Bai-Qiao Song; Qing-Yuan Yang; Shi-Qiang Wang; Matthias Vandichel; Amrit Kumar; Clare Crowley; Naveen Kumar; Cheng-Hua Deng; Victoria GasconPerez; Matteo Lusi; Hui Wu; Wei Zhou; Michael J. Zaworotko
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[email protected]2 Core–Shell Heterostructure as SERS Platform to Reveal the Hydrogen Evolution Active Sites of Single-Layer MoS2 J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Junze Chen; Guigao Liu; Yue-zhou Zhu; Min Su; Pengfei Yin; Xue-jun Wu; Qipeng Lu; Chaoliang Tan; Meiting Zhao; Zhengqing Liu; Weimin Yang; Hai Li; Gwang-Hyeon Nam; Liping Zhang; Zhenhua Chen; Xiao Huang; Petar M. Radjenovic; Wei Huang; Zhong-qun Tian; Jian-feng Li; Hua Zhang
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Record Complexity in the Polycatenation of Three Porous Hydrogen-Bonded Organic Frameworks with Stepwise Adsorption Behaviors J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Yu-Lin Li; Eugeny V. Alexandrov; Qi Yin; Lan Li; Zhi-Bin Fang; Wenbing Yuan; Davide M. Proserpio; Tian-Fu Liu
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Enantioselective Tail-to-Head Cyclizations Catalyzed by Dual-Hydrogen-Bond Donors J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-03 Dennis A. Kutateladze; Daniel A. Strassfeld; Eric N. Jacobsen
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Expressed Protein Ligation without Intein J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Yuchen Qiao; Ge Yu; Kaci C. Kratch; Xiaoyan Aria Wang; Wesley Wei Wang; Sunshine Z. Leeuwon; Shiqing Xu; Jared S. Morse; Wenshe Ray Liu
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Grain-Boundary-Rich Copper for Efficient Solar-Driven Electrochemical CO2 Reduction to Ethylene and Ethanol J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Zhiqiang Chen; Tuo Wang; Bin Liu; Dongfang Cheng; Congling Hu; Gong Zhang; Wenjin Zhu; Huaiyuan Wang; Zhi-Jian Zhao; Jinlong Gong
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Cellular Force Nanoscopy with 50 nm Resolution Based on Integrin Molecular Tension Imaging and Localization J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Yuanchang Zhao; Kaushik Pal; Ying Tu; Xuefeng Wang
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Mechanistic Insights into the Origin of Stereoselectivity in an Asymmetric Chlorolactonization Catalyzed by (DHQD)2PHAL J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Roozbeh Yousefi; Aritra Sarkar; Kumar Dilip Ashtekar; Daniel C. Whitehead; Tayeb Kakeshpour; Daniel Holmes; Paul Reed; James E. Jackson; Babak Borhan
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Facets Directed Connecting Perovskite Nanocrystals J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Biswajit Hudait; Sumit Kumar Dutta; Avijit Patra; Diptam Nasipuri; Narayan Pradhan
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Electrostatic Interactions Control the Functionality of Bacterial Ice Nucleators J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 M. Lukas; R. Schwidetzky; A. T. Kunert; U. Pöschl; J. Fröhlich-Nowoisky; M. Bonn; K. Meister
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Stark Spectroscopic Evidence that a Spin Change Accompanies Light Absorption in Transition Metal Polypyridyl Complexes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-02 Andrew B. Maurer; Gerald J. Meyer
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Transformation Strategy for Highly Crystalline Covalent Triazine Frameworks: From Staggered AB to Eclipsed AA Stacking J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Zhenzhen Yang; Hao Chen; Song Wang; Wei Guo; Tao Wang; Xian Suo; De-en Jiang; Xiang Zhu; Ilja Popovs; Sheng Dai
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High-Flux Vertically Aligned 2D Covalent Organic Framework Membrane with Enhanced Hydrogen Separation J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Hongwei Fan; Manhua Peng; Ina Strauss; Alexander Mundstock; Hong Meng; Jürgen Caro
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Electrical Conductivity in a Porous, Cubic Rare-Earth Catecholate J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Grigorii Skorupskii; Mircea Dincă
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Fluoride Migration Catalysis Enables Simple, Stereoselective, and Iterative Glycosylation J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Girish C. Sati; Joshua L. Martin; Yishu Xu; Tanmay Malakar; Paul M. Zimmerman; John Montgomery
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Targeted Degradation of the Oncogenic MicroRNA 17-92 Cluster by Structure-Targeting Ligands J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Xiaohui Liu; Hafeez S. Haniff; Jessica L. Childs-Disney; Anton Shuster; Haruo Aikawa; Alexander Adibekian; Matthew D. Disney
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Ions Tune Interfacial Water Structure and Modulate Hydrophobic Interactions at Silica Surfaces J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Aashish Tuladhar; Shalaka Dewan; Simone Pezzotti; Flavio Siro Brigiano; Fabrizio Creazzo; Marie-Pierre Gaigeot; Eric Borguet
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Sodium Hexamethyldisilazide: Using 15N–29Si Scalar Coupling to Determine Aggregation and Solvation States J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Ryan A. Woltornist; David B. Collum
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Near-Infrared Fluorescent Macromolecular Reporters for Real-Time Imaging and Urinalysis of Cancer Immunotherapy J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Shasha He; Jingchao Li; Yan Lyu; Jiaguo Huang; Kanyi Pu
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Design of Ru(II)-NHC-Diamine Precatalysts Directed by Ligand Cooperation: Applications and Mechanistic Investigations for Asymmetric Hydrogenation J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Wei Li; Tobias Wagener; Lars Hellmann; Constantin G. Daniliuc; Christian Mück-Lichtenfeld; Johannes Neugebauer; Frank Glorius
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Metastable Rock Salt Oxide-Mediated Synthesis of High-Density Dual-Protected [email protected] for Long-Life Rechargeable Zinc–Air Batteries with Record Power Density J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Tang Tang; Wen-Jie Jiang; Xiao-Zhi Liu; Jun Deng; Shuai Niu; Bin Wang; Shi-Feng Jin; Qiang Zhang; Lin Gu; Jin-Song Hu; Li-Jun Wan
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An Exceptionally Stable Metal–Organic Framework Constructed from Chelate-Based Metal–Organic Polyhedra J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Jerika A. Chiong; Jie Zhu; Jake B. Bailey; Mark Kalaj; Rohit H. Subramanian; Wenqian Xu; Seth M. Cohen; F. Akif Tezcan
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Splitting Mono- and Dibranched Alkane Isomers by a Robust Aluminum-Based Metal–Organic Framework Material with Optimal Pore Dimensions J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Liang Yu; Xinglong Dong; Qihan Gong; Shree Ram Acharya; Yuhan Lin; Hao Wang; Yu Han; Timo Thonhauser; Jing Li
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New Neutral Nickel and Palladium Sandwich Catalysts: Synthesis of Ultra-High Molecular Weight Polyethylene (UHMWPE) via Highly Controlled Polymerization and Mechanistic Studies of Chain Propagation J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Quan H. Tran; Maurice Brookhart; Olafs Daugulis
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On the Nature of C(sp3)–C(sp2) Bond Formation in Nickel-Catalyzed Tertiary Radical Cross-Couplings: A Case Study of Ni/Photoredox Catalytic Cross-Coupling of Alkyl Radicals and Aryl Halides J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Mingbin Yuan; Zhihui Song; Shorouk O. Badir; Gary A. Molander; Osvaldo Gutierrez
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Sequence-Specific Quantitation of Mutagenic DNA Damage via Polymerase Amplification with an Artificial Nucleotide J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-04-01 Claudia M. N. Aloisi; Arman Nilforoushan; Nathalie Ziegler; Shana J. Sturla
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Perylene Diimide-Embedded Double [8]Helicenes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Bo Liu; Marcus Böckmann; Wei Jiang; Nikos L. Doltsinis; Zhaohui Wang
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Biosynthesis of a New Benzazepine Alkaloid Nanangelenin A from Aspergillus nanangensis Involves an Unusual l-Kynurenine-Incorporating NRPS Catalyzing Regioselective Lactamization J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Hang Li; Cameron L. M. Gilchrist; Chin-Soon Phan; Heather J. Lacey; Daniel Vuong; Stephen A. Moggach; Ernest Lacey; Andrew M. Piggott; Yit-Heng Chooi
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Intrinsic Kinetic Limitations in Substituted Lithium-Layered Transition-Metal Oxide Electrodes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Antonin Grenier; Philip J. Reeves; Hao Liu; Ieuan D. Seymour; Katharina Märker; Kamila M. Wiaderek; Peter J. Chupas; Clare P. Grey; Karena W. Chapman
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Engineering Cytochrome P450s for Enantioselective Cyclopropenation of Internal Alkynes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Kai Chen; Frances H. Arnold
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Kinetic Control in the Synthesis of a Möbius Tris((ethynyl)[5]helicene) Macrocycle Using Alkyne Metathesis J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Xing Jiang; Summer D. Laffoon; Dandan Chen; Salvador Pérez-Estrada; Andrew S. Danis; Joaquín Rodríguez-López; Miguel A. Garcia-Garibay; Jun Zhu; Jeffrey S. Moore
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Highly Selective Removal of Trace Isomers by Nonporous Adaptive Pillararene Crystals for Chlorobutane Purification J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Yujuan Zhou; Kecheng Jie; Run Zhao; Errui Li; Feihe Huang
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Spotlights on Recent JACS Publications J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 ACS Contributing Correspondents
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Catalytic, Asymmetric Dearomative Synthesis of Complex Cyclohexanes via a Highly Regio- and Stereoselective Arene Cyclopropanation Using α-Cyanodiazoacetates J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-31 Kendrick L. Smith; Cody L. Padgett; William D. Mackay; Jeffrey S. Johnson
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Heterometallic Titanium–Organic Frameworks by Metal-Induced Dynamic Topological Transformations J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Natalia M. Padial; Belén Lerma-Berlanga; Neyvis Almora-Barrios; Javier Castells-Gil; Iván da Silva; Marı́a de la Mata; Sergio I. Molina; Jesús Hernández-Saz; Ana E. Platero-Prats; Sergio Tatay; Carlos Martı́-Gastaldo
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Fabricating Covalent Organic Framework Capsules with Commodious Microenvironment for Enzymes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Mingmin Li; Shan Qiao; Yunlong Zheng; Yassin H. Andaloussi; Xia Li; Zhenjie Zhang; Ang Li; Peng Cheng; Shengqian Ma; Yao Chen
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Thiol–Ene Networks from Sequence-Defined Polyurethane Macromers J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Emily A. Hoff; Guilhem X. De Hoe; Christopher M. Mulvaney; Marc A. Hillmyer; Christopher A. Alabi
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Multielectron, Cation and Anion Redox in Lithium-Rich Iron Sulfide Cathodes J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Charles J. Hansen; Joshua J. Zak; Andrew J. Martinolich; Jesse S. Ko; Nicholas H. Bashian; Farnaz Kaboudvand; Anton Van der Ven; Brent C. Melot; Johanna Nelson Weker; Kimberly A. See
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Pervasive Charge Solvation Permeates Native-like Protein Ions and Dramatically Influences Top-down Sequencing Data J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Daniel A. Polasky; Sugyan M. Dixit; Michael F. Keating; Varun V. Gadkari; Philip C. Andrews; Brandon T. Ruotolo
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Ligand-Enabled Monoselective β-C(sp3)–H Acyloxylation of Free Carboxylic Acids Using a Practical Oxidant J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Zhe Zhuang; Alastair N. Herron; Zhoulong Fan; Jin-Quan Yu
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Isotactic Poly(propylene oxide): A Photodegradable Polymer with Strain Hardening Properties J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Bryce M. Lipinski; Lilliana S. Morris; Meredith N. Silberstein; Geoffrey W. Coates
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Synthesis of a Black Dye with Absorption Capabilities Across the Visible-to-Near-Infrared Region: A MO-Mixing Approach via Heterometal Coordination of Expanded Porphyrinoid J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Yue Wang; Hiroto Kai; Masatoshi Ishida; Sabapathi Gokulnath; Shigeki Mori; Tomotaka Murayama; Atsuya Muranaka; Masanobu Uchiyama; Yuhsuke Yasutake; Susumu Fukatsu; Yusuke Notsuka; Yoshihisa Yamaoka; Mamiko Hanafusa; Michito Yoshizawa; Gakhyun Kim; Dongho Kim; Hiroyuki Furuta
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Photosynergetic Electrochemical Synthesis of Graphene Oxide J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Duhong Chen; Zhen Lin; Matthew M. Sartin; Teng-Xiang Huang; Jia Liu; Qiugen Zhang; Lianhuan Han; Jian-Feng Li; Zhong-Qun Tian; Dongping Zhan
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Solvent-Assisted Self-Assembly of a Metal–Organic Framework Based Biocatalyst for Cascade Reaction Driven Photodynamic Therapy J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Liangcan He; Qianqian Ni; Jing Mu; Wenpei Fan; Lu Liu; Zhantong Wang; Ling Li; Wei Tang; Yijing Liu; Yaya Cheng; Longguang Tang; Zhen Yang; Yuan Liu; Jianhua Zou; Weijing Yang; Orit Jacobson; Fan Zhang; Pintong Huang; Xiaoyuan Chen
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Ultrafine Titanium Monoxide (TiO1+x) Nanorods for Enhanced Sonodynamic Therapy J. Am. Chem. Soc. (IF 14.695) Pub Date : 2020-03-30 Xianwen Wang; Xiaoyan Zhong; Lixin Bai; Jun Xu; Fei Gong; Ziliang Dong; Zhijuan Yang; Zhijie Zeng; Zhuang Liu; Liang Cheng
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