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Thao T. Tran Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-29
“My biggest motivation is to bring my heart and soul, when strongly supported by rigorous scientific evidence, into both the doing and the communicating of science … .I chose my current career path because it provides me with a unique opportunity to support and mentor the next generation of scientists …” Find out more about Thao T. Tran in her Introducing … Profile.
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Corrigendum: Mechanistic Studies on the Organocatalytic α-Chlorination of Aldehydes: The Role and Nature of Off-Cycle Intermediates Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-28
Angew. Chem. Int. Ed. 2022, 61, e202214643 This Corrigendum was incorrectly published with the byline of the article being corrected. The Corrigendum is being issued by the journal to correct the record and should not have contained a byline. We apologize for the error.
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The Collaboration Among the Ibáñez–Brutchey–Arbiol Groups Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-28
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An Analytical Specialty Team Enabling Merck's Pipeline with Pioneering Measurement Science Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-24
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An Enzymatically Gated Catalytic Hairpin Assembly Delivered by Lipid Nanoparticles for the Tumor-Specific Activation of Signal Amplification in miRNA Imaging Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-16 Qing Liu, Yuanyu Huang, Zhengping Li, Lele Li, Yuliang Zhao, Mengyuan Li
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Zirconium Carbide Mediates Coke-Resistant Methane Dry Reforming on Nickel-Zirconium Catalysts Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-15 Leander Haug, Christoph Thurner, Maged F. Bekheet, Benjamin Bischoff, Aleksander Gurlo, Martin Kunz, Bernhard Sartory, Simon Penner, Bernhard Klötzer
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Advancing Critical Chemical Processes for a Sustainable Future: Challenges for Industry and the Max Planck–Cardiff Centre on the Fundamentals of Heterogeneous Catalysis (FUNCAT) Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-09 Michael Bowker, Serena DeBeer, Nicholas F. Dummer, Graham J. Hutchings, Matthias Scheffler, Ferdi Schüth, Stuart H. Taylor, Harun Tüysüz
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Minimum Information Standards in Chemistry: A Call for Better Research Data Management Practices Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Sonja Herres-Pawlis, Felix Bach, Ian J. Bruno, Stuart J. Chalk, Nicole Jung, Johannes C. Liermann, Leah R. McEwen, Steffen Neumann, Christoph Steinbeck, Matthias Razum, Oliver Koepler
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Organocatalytic Enantioselective Diels–Alder Reaction of 2-Trifluoroacetamido-1,3-dienes with α,β-Unsaturated Ketones Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Xin-Qi Zhu, Qian Wang, Jieping Zhu
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Reversible Switching CuII/CuI Single Sites Catalyze High-rate and Selective CO2 Photoreduction Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Xiaolong Zu, Yuan Zhao, Xiaodong Li, Runhua Chen, Weiwei Shao, Li Li, Panzhe Qiao, Wensheng Yan, Yang Pan, Qian Xu, Junfa Zhu, Yongfu Sun, Yi Xie
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Charge-Transfer Complex Doped Photothermal Hydrogels for Discriminating Circularly Polarized Near-Infrared Light Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Zhuoer Wang, Aiyou Hao, Pengyao Xing
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Tunable Strategy for the Asymmetric Synthesis of Sulfoglycolipids from Mycobacterium tuberculosis To Elucidate the Structure and Immunomodulatory Property Relationships Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Soumik Mondal, Chieh-Jen Tseng, Janet Jia-Yin Tan, Ding-Yuan Lin, Hsien-Ya Lin, Jui–Hsia Weng, Chun-Hung Lin, Kwok-Kong Tony Mong
A tunable asymmetric strategy for the synthesis of sulfoglycolipids (SGLs) was developed. The strategy features a suite of asymmetrically protected trehaloses for acylation and sulfation. A practical synthetic route was explored for the preparation of polydeoxypropionate fatty acids, which together with the trehaloses enabled the synthesis of different classes of SGLs for immunological studies.
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α-Synuclein as a Target for Metallo-Anti-Neurodegenerative Agents Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Kaiming Cao, Yang Zhu, Zhuanghao Hou, Manman Liu, Yanyan Yang, Hongze Hu, Yi Dai, Yu Wang, Siming Yuan, Guangming Huang, Jiaming Mei, Peter J. Sadler, Yangzhong Liu
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Bioinspired Gradient Stretchable Aerogels for Ultrabroad-Range-Response Pressure-Sensitive Wearable Electronics and High-Efficient Separators Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-08 Xiaoyu Zhang, Zhenyu Hu, Qi Sun, Xing Liang, Puzhong Gu, Jia Huang, Guoqing Zu
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Diboron(4)-Catalyzed Remote [3+2] Cycloaddition of Cyclopropanes via Dearomative/Rearomative Radical Transmission through Pyridine Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Ming Xu, Zhijun Wang, Zhaohui Sun, Yizhao Ouyang, Zhengwei Ding, Tao Yu, Liang Xu, Pengfei Li
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Large-area Free-standing Metalloporphyrin-based Covalent Organic Framework Films by Liquid-air Interfacial Polymerization for Oxygen Electrocatalysis Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Jiaqi Tang, Zuozhong Liang, Haonan Qin, Xiangquan Liu, Binbin Zhai, Zhen Su, Qianqian Liu, Haitao Lei, Kaiqiang Liu, Chuan Zhao, Rui Cao, Yu Fang
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Chemical Synthesis of Proteins with Base-Labile Posttranslational Modifications Enabled by a Boc-SPPS Based General Strategy Towards Peptide C-Terminal Salicylaldehyde Esters Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Wenjie Ma, Hongxiang Wu, Sha Liu, Tongyao Wei, Xiang David Li, Han Liu, Xuechen Li
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Nitrenoid from Oxime: A Practical Synthesis of Planar Chiral Ferrocenyl Phenanthridines via Nitrene-Involved Ring-Expansion Reaction Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Na Li, Biqiong Hong, Jinbo Zhao, Zhenhua Gu
A new Grignard reagent-mediated synthesis of ferrocene-based phenanthridines from oximes was developed. The tertiary magnesium-zinc nitrenoid was proposed as the key intermediate, which underwent ring-expansion/rearrangement to form pyridine skeleton.
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Enantioselective Hydrosilylation of β,β-Disubstituted Enamides to Construct α-Aminosilanes with Vicinal Stereocenters Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Wen-Wen Zhang, Bi-Jie Li
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Perfectly Encoding π-Conjugated Anions in the RE5(C3N3O3)(OH)12 (RE=Y, Yb, Lu) Family with Strong Second Harmonic Generation Response and Balanced Birefringence Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Xianghe Meng, Xingyu Zhang, Qingxiong Liu, Zhengyang Zhou, Xingxing Jiang, Yonggang Wang, Zheshuai Lin, Mingjun Xia
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Anionic Magnesium and Calcium Hydrides: Transforming CO into Unsaturated Disilyl Ethers Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Jacob S. McMullen, Ryan Huo, Petra Vasko, Alison J. Edwards, Jamie Hicks
CO has directly been transformed into small organic starting materials using earth-abundant, anionic group 2 hydride reagents.
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A Platinum(II)-Based Molecular Cage with Aggregation-Induced Emission for Enzymatic Photocyclization of Alkynylaniline Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Zhong Wei, Xu Jing, Yang Yang, Jiayou Yuan, Mingxu Liu, Cheng He, Chunying Duan
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Dithiol-Activated Bioorthogonal Chemistry for Endoplasmic Reticulum-Targeted Synergistic Chemophototherapy Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Jian Sun, Xiaoran Zhang, Xia Wang, Jinlei Peng, Gang Song, Yufei Di, Fude Feng, Shu Wang
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Formyl Radical Generation from α-Chloro N-Methoxyphthalimides Enables Selective Aldehyde Synthesis Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Dan Liu, Kai Yang, Di Fang, Shi-Jun Li, Yu Lan, Yiyun Chen
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Encapsulating Metal Nanoparticles into a Layered Zeolite Precursor with Surface Silanol Nests Enhances Sintering Resistance** Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Ang Li, Yuyan Zhang, Christopher J. Heard, Kinga Gołąbek, Xiaohui Ju, Jiří Čejka, Michal Mazur
IPC-1P, a layered zeolite precursor with a relatively high density of surface silanols can be swollen using docosyltrimethylammonium hydroxide and functionalized with ultra-small Rh nanoparticles. The resulting mesoporous zeolitic material Rh@IPC_C22 has a high layer disordering without microporosity. In situ heating STEM imaging and DFT simulations show strong metal-silanol interactions stabilizing
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In Vivo Biocatalytic Cascades Featuring an Artificial-Enzyme-Catalysed New-to-Nature Reaction** Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-07 Linda Ofori Atta, Zhi Zhou, Gerard Roelfes
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Water-soluble Self-assembled {Pd84}Ac Polyoxopalladate Nano-wheel as a Supramolecular Host Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-06 Zoë L. Sinclair, Nicola L. Bell, Jessica R. Bame, De-Liang Long, Leroy Cronin
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Oxidation and Reduction Pathways in the Knowles Hydroamination via a Photoredox-Catalyzed Radical Reaction** Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-06 Yu Harabuchi, Hiroki Hayashi, Hideaki Takano, Tsuyoshi Mita, Satoshi Maeda
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Dr. Markus Stöckl Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04
“My group has fun by pulling me into a competition who makes the best cake … My biggest motivation is to keep an working environment where all workers can unfold their capabilities …” Find out more about Markus Stöckl in his Introducing … Profile.
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A Polyfluoroalkyl-Containing Non-fullerene Acceptor Enables Self-Stratification in Organic Solar Cells Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-05 Shihao Chen, Ling Hong, Minghao Dong, Wanyuan Deng, Lin Shao, Yuanqing Bai, Kai Zhang, Chunchen Liu, Hongbin Wu, Fei Huang
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A De Novo-Designed Type 3 Copper Protein Tunes Catechol Substrate Recognition and Reactivity Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-05 Fabio Pirro, Salvatore La Gatta, Federica Arrigoni, Antonino Famulari, Ornella Maglio, Pompea Del Vecchio, Mario Chiesa, Luca De Gioia, Luca Bertini, Marco Chino, Flavia Nastri, Angela Lombardi
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Catalytically Stable Potassium Single-Atom Solid Superbases Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Song-Song Peng, Xiang-Bin Shao, Meng-Xuan Gu, Guo-Song Zhang, Chen Gu, Yao Nian, Yiming Jia, You Han, Xiao-Qin Liu, Lin-Bing Sun
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A Low-Concentration Electrolyte for High-Voltage Lithium-Metal Batteries: Fluorinated Solvation Shell and Low Salt Concentration Effect Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Rongyu Deng, Fulu Chu, Felix Kwofie, Zengqiang Guan, Jieshuangyang Chen, Feixiang Wu
A low-concentration electrolyte was employed in high-voltage lithium metal batteries. The synergistic effects of fluorinated solvation shell and low salt concentration generated robust and LiF-rich SEI and fewer unfavorable decomposition products. The excellent performance implies that the optimization of low concentration electrolyte is a successful solution for low-cost and large-scale electrolyte
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Cobalt-Catalyzed Regiodivergent Double Hydrosilylation of Arylacetylenes Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Zhaoyang Cheng, Minghua Li, Xu-Yang Zhang, Yue Sun, Qing-Lei Yu, Xing-Hong Zhang, Zhan Lu
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In Situ Enzyme Immobilization by Covalent Organic Frameworks Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Clémence Sicard
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Remarkable White Circularly Polarized Electroluminescence Based on Chiral Co-assembled Helix Nanofiber Emitters Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Yu Zhang, Yupeng Li, Yiwu Quan, Shanghui Ye, Yixiang Cheng
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Imine Directed Cp*RhIII-Catalyzed N−H Functionalization and Annulation with Amino Amides, Aldehydes, and Diazo Compounds Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Adam J. Zoll, Jenna C. Molas, Brandon Q. Mercado, Jonathan A. Ellman
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A Crosslinked Ionic Organic Framework for Efficient Iodine and Iodide Remediation in Water Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Mingshi Zhang, Jayanta Samanta, Benjamin A. Atterberry, Richard Staples, Aaron J. Rossini, Chenfeng Ke
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Tumor-Selective Activation of Toll-Like Receptor 7/8 Agonist Nano-Immunomodulator Generates Safe Anti-Tumor Immune Responses upon Systemic Administration Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-04 Yanyun Hao, Hui Li, Xiaoyan Ge, Yang Liu, Xia Li, Yutong Liu, Hongfei Chen, Shiying Zhang, Jing Zou, Lingling Huang, Fabao Zhao, Dongwei Kang, Bruno G. De Geest, Zhiyue Zhang
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Alternately π-Stacked Systems Assisted by o-Carborane: Dual Excimer Emission and Color Modulation by Bcage-Methylation Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Junki Ochi, Kazuo Tanaka, Yoshiki Chujo
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Rhodium-Catalyzed Dynamic Kinetic Asymmetric Hydrosilylation to Access Silicon-Stereogenic Center Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Yan Zeng, Xiao-Jun Fang, Ren-He Tang, Jing-Yu Xie, Feng-Jiao Zhang, Zheng Xu, Yi-Xue Nie, Li-Wen Xu
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Durable Lithium Metal Anodes Enabled by Interfacial Layers Based on Mechanically Interlocked Networks Capable of Energy Dissipation Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Jun Zhao, Min Hong, Zhijin Ju, Xuzhou Yan, Yanzhe Gai, Zheng Liang
Mechanically interlocked network (MIN) with robustness and unique energy dissipation capability was used as the interfacial layer which survived and suppressed repeated Li protrusion in long-term and high-capacity cycling to afford durable lithium metal anodes. This work highlights the importance of the energy dissipation feature in stabling Li metal anode, promising MIN's future success in other battery-related
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Heterogeneous Electrospinning Nanofiber Membranes with pH-regulated Ion Gating for Tunable Osmotic Power Harvesting Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Haoyang Ling, Weiwen Xin, Yongchao Qian, Xiaofeng He, Linsen Yang, Weipeng Chen, Yadong Wu, Huaqing Du, Yang Liu, Xiang-Yu Kong, Lei Jiang, Liping Wen
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Multilayered Ceramic Membrane with Ion Conducting Thin Layer Induced by Interface Reaction for Stable Hydrogen Production Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Guanghu He, Qianqian Lan, Mengke Liu, Guixuan Wu, Rafal E. Dunin-Borkowski, Heqing Jiang
Inspired by the architectural structure of the rooted grasses in soil, an interface-reaction-induced reassembly approach for the direct fabrication of ion-conducting thin layers rooted in multilayered ceramic membranes has been developed. This novel technique paves the way for the development of high-performance multilayered ceramics with functional layers for various applications, from ceramic fuel
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Organocatalyzed Controlled Radical Copolymerization toward Hybrid Functional Fluoropolymers Driven by Light Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Yang Zeng, Qinzhi Quan, Peng Wen, Zexi Zhang, Mao Chen
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Bifunctional Europium for Operando Catalyst Thermometry in an Exothermic Chemical Reaction Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Bas J. P. Terlingen, Tjom Arens, Thomas P. van Swieten, Freddy T. Rabouw, P. Tim Prins, Michiel M. de Beer, Andries Meijerink, Mathieu P. Ahr, Eline M. Hutter, Coert E. J. van Lare, Bert M. Weckhuysen
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Biocatalytic Thionation of Epoxides for Enantioselective Synthesis of Thiiranes Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Ran Ma, Xia Hua, Cheng-Li He, Hui-Hui Wang, Zhu-Xiang Wang, Bao-Dong Cui, Wen-Yong Han, Yong-Zheng Chen, Nan-Wei Wan
A biocatalytic thionation method is presented for the enantioselective synthesis of thiiranes from epoxides by a halohydrin dehalogenase catalyzed kinetic resolution approach using thiocyanate as a sulfur donor. Various chiral thiiranes bearing aryl and alkyl substituents were synthesized in good yields and enantioselectivities by using recombinant Escherichia coli cells expressing the engineered halohydrin
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Edge-to-Center Propagation of Photochemical Reaction during Single-Crystal-to-Single-Crystal Photomechanical Transformation of 2,5-Distyrylpyrazine Crystals** Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Kohei Morimoto, Daichi Kitagawa, Hikaru Sotome, Syoji Ito, Hiroshi Miyasaka, Seiya Kobatake
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Broadband Photoresponses from Ultraviolet to Near-Infrared (II) Region through Light-induced Pyroelectric Effects in a Hybrid Perovskite Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Wuqian Guo, Haojie Xu, Wen Weng, Liwei Tang, Yu Ma, Yi Liu, Lina Hua, Beibei Wang, Junhua Luo, Zhihua Sun
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Conversion of Polyethylenes into Fungal Secondary Metabolites Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-03 Chris Rabot, Yuhao Chen, Swati Bijlani, Yi-Ming Chiang, C. Elizabeth Oakley, Berl R. Oakley, Travis J. Williams, Clay C. C. Wang
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The Marriage of Sierpiński Triangles and Platonic Polyhedra Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-02 Jun Wang, Zhilong Jiang, Weiya Liu, Zihao Wu, Rui Miao, Fan Fu, Jia-Fu Yin, Bangtang Chen, Qiangqiang Dong, He Zhao, Kaixiu Li, Guotao Wang, Die Liu, Panchao Yin, Yiming Li, Mingzhao Chen, Pingshan Wang
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Spin-Selective Charge Transport in Lead-Free Chiral Perovskites: The Key towards High-Anisotropy in Circularly-Polarized Light Detection Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-02 Abhishek Maiti, Amlan J. Pal
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Photo-Induced Microfluidic Production of Ultrasmall Glyco Gold Nanoparticles Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-02 Patricia Perez Schmidt, Katiuscia Pagano, Cristina Lenardi, Marta Penconi, Ruth Mateu Ferrando, Claudio Evangelisti, Luigi Lay, Laura Ragona, Marcello Marelli, Laura Polito
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Reticular Synthesis of One-Dimensional Covalent Organic Frameworks with 4-c sql Topology for Enhanced Fluorescence Emission Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-02 Ziao Chen, Kai Wang, Yumeng Tang, Lan Li, Xuening Hu, Mingxi Han, Zhiyong Guo, Hongbing Zhan, Banglin Chen
A series of 1D-COFs were synthesized by combining vertices with different symmetries and matching the nonlinear edges. The 1D-COFs, which employed AIEgens as the vertex, showed enhanced fluorescence emission properties compared with their 2D analogs.
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Convergent Assembly of the Tricyclic Labdane Core Enables Synthesis of Diverse Forskolin-like Molecules Angew. Chem. Int. Ed. (IF 16.823) Pub Date : 2022-11-02 Paweł M. Szczepanik, Andrey A. Mikhaylov, Ondřej Hylse, Roman Kučera, Petra Daďová, Marek Nečas, Lukáš Kubala, Kamil Paruch, Jakub Švenda
Labdane-type terpenes are a large family of bioactive natural products. Their often-complex structures present challenges to semisynthesis and de novo chemical synthesis in search of analogs with improved properties. To enable new modifications of the well-known tricyclic terpene forskolin, we have developed a distinct and potentially general synthetic scheme for the preparation of analogs of complex
更新日期：2022-11-15
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