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Comparative Evaluation of Light-Driven Catalysis: A Framework for Standardized Reporting of Data** Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-13 Dirk Ziegenbalg, Andrea Pannwitz, Sven Rau, Benjamin Dietzek-Ivanšić, Carsten Streb
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Corrigendum: Ferrocene-Induced Perpetual Recovery on All Elemental Defects in Perovskite Solar Cells Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-10 Qing Chang, Fangfang Wang, Wenxin Xu, Aifei Wang, You Liu, Juangan Wang, Yikai Yun, Song Gao, Kang Xiao, Liangliang Zhang, Lin Wang, Jianpu Wang, Wei Huang, Tianshi Qin
It has come to the authors attention that incorrect versions of Figures 1, 2, and 4 were inadvertently used during the final stages of manuscript preparation. The correct figures are shown below. This does not affect the interpretation of data or the conclusion given in this Research Article. Figure 1 Open in figure viewerPowerPoint Illustrations of sustainably eliminating on comprehensive defects
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Corrigendum: Rhodium-Catalyzed Stereoselective Deuteration of Benzylic C–H Bonds via Reversible η6-Coordination Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-10 Qi-Kai Kang, Yuntong Li, Kai Chen, Hui Zhu, Wen-Qiang Wu, Yunzhi Lin, Hang Shi
The authors have found that the ss values (the percentage of the reaction that proceeds with stereoretention) of compounds 56 to 64 in Table 3 are different from those given in the Supporting Information, which are correct. Corrections to the Reference section are also required, as described below. The ss values of 56 to 64 in Table 3 of this Research Article should be corrected as follows: compound
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Corrigendum: Mediated Inner-Sphere Electron Transfer Induces Homogeneous Reduction of CO2 via Through-Space Electronic Conjugation Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-10 Shelby L. Hooe, Juan J. Moreno, Amelia G. Reid, Emma N. Cook, Charles W. Machan
It has come to the authors attention that the experimental turnover frequencies (TOFs) were calculated incorrectly by using a second-order rate constant for the reaction instead of the first-order observed rate constant as defined in the original derivation.1, 2 The presented TOF values from re-analyzed experimental electrolysis data are shown below in an updated version of Table 1. These values should
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Native Ambient Mass Spectrometry of an Intact Membrane Protein Assembly and Soluble Protein Assemblies Directly from Lens Tissue Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-06 Oliver J. Hale, Helen J. Cooper
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Methylamine Lithium Borohydride as Electrolyte for All-Solid-State Batteries Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-04 Jakob B. Grinderslev, Lasse N. Skov, Jacob G. Andreasen, Shaiq Ghorwal, Jørgen Skibsted, Torben R. Jensen
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Daniël Laurens Johannes Broere Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-02
“The most important quality of a mentor is that they help you achieve your goals even though it might sometimes disadvantage them. I have been fortunate to have found this quality in my PhD and postdoc advisors … My favorite thing about my lab group is their commitment and passion to push the boundaries of science as a team with me …” Find out more about Daniël Broere in his Introducing … Profile.
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Highly Active Si Sites Enabled by Negative Valent Ru for Electrocatalytic Hydrogen Evolution in LaRuSi Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Shijie Shen, Zhiyun Hu, Huanhuan Zhang, Kai Song, Zongpeng Wang, Zhiping Lin, Qinghua Zhang, Lin Gu, Wenwu Zhong
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Discovery and Genetic Code Expansion of a Polyethylene Terephthalate (PET) Hydrolase from the Human Saliva Metagenome for the Degradation and Bio-Functionalization of PET Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Bhumrapee Eiamthong, Piyachat Meesawat, Thanakrit Wongsatit, Jariya Jitdee, Raweewan Sangsri, Maturada Patchsung, Kanokpol Aphicho, Surased Suraritdechachai, Nicolas Huguenin-Dezot, Shan Tang, Wipa Suginta, Boonchoat Paosawatyanyong, M. Madan Babu, Jason W. Chin, Danaya Pakotiprapha, Worawan Bhanthumnavin, Chayasith Uttamapinant
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Embedding Multiphoton Active Units within Metal–Organic Frameworks for Turning on High-Order Multiphoton Excited Fluorescence for Bioimaging Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Bo Li, Xin Lu, Yupeng Tian, Dandan Li
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Nitric-Oxide-Releasing aza-BODIPY: A New Near-Infrared J-Aggregate with Multiple Antibacterial Modalities Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Xinyao Bao, Shaoqiu Zheng, Lei Zhang, Aizong Shen, Guoying Zhang, Shiyong Liu, Jinming Hu
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Straightforward Access to Multifunctional π-Conjugated P-Heterocycles Featuring an Internal Ylidic Bond** Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Thomas Delouche, Elsa Caytan, Marie Cordier, Thierry Roisnel, Grégory Taupier, Yann Molard, Nicolas Vanthuyne, Boris Le Guennic, Muriel Hissler, Denis Jacquemin, Pierre-Antoine Bouit
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Enantioselective Hydrocarbamoylation of Alkenes Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Sheng Feng, Yuyang Dong, Stephen L. Buchwald
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Formal β-C−H Arylation of Aldehydes and Ketones by Cooperative Nickel and Photoredox Catalysis Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-03 Kun Liu, Armido Studer
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Tailored Multivalent Targeting of Siglecs with Photosensitizing Liposome Nanocarriers Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-02 Verónica Almeida-Marrero, Fleur Bethlehem, Sara Longo, M. Candelaria Bertolino, Tomás Torres, Jurriaan Huskens, Andrés de la Escosura
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Umpolung AlaB Reagents for the Synthesis of Non-Proteogenic Amino Acids, Peptides and Proteins** Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-02 Feng Zhu, Eric Miller, Wyatt C. Powell, Kelly Johnson, Alexander Beggs, Garrett E. Evenson, Maciej A. Walczak
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Synthetic Reprogramming of Kinases Expands Cellular Activities of Proteins Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Veronika M. Shoba, Dhanushka N. P. Munkanatta Godage, Santosh K. Chaudhary, Arghya Deb, Sachini U. Siriwardena, Amit Choudhary
A high-yielding synthetic route to bifunctional molecules that reprogram activities of protein kinase C and engineered Abelson kinase to induce phosphorylation on neo-substrates is reported. These phosphorylations have promising inhibitory effects on the activity of Bruton's tyrosine kinase (BTK) and BCR-ABL-dependent cancer cells.
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Bioinspired and Ligand-Regulated Unnatural Prenylation and Geranylation of Oxindoles with Isoprene under Pd Catalysis Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Chao-Yang Zhao, Ying-Ying Liu, Xiang-Xin Zhang, Gu-Cheng He, Heng Liu, Ding-Wei Ji, Yan-Cheng Hu, Qing-An Chen
A practical strategy has been developed for the bioinspired and ligand-regulated chemoselective unnatural prenylation and geranylation of oxindoles with isoprene under Pd catalysis. The selectivity was governed by modulating the coordination geometry of the Pd catalyst.
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Precision Synthesis of Various Low-Bandgap Donor–Acceptor Alternating Conjugated Polymers via Living Suzuki–Miyaura Catalyst-Transfer Polymerization Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Hwangseok Kim, Jaeho Lee, Taehyun Kim, Minyoung Cho, Tae-Lim Choi
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Enzymatic Enantioselective anti-Markovnikov Hydration of Aryl Alkenes Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Hui Lin, Yinyin Meng, Na Li, Yanhong Tang, Shuang Dong, Zhongliu Wu, Cuilian Xu, Romas Kazlauskas, Hongge Chen
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Mild Acidosis-Directed Signal Amplification in Tumor Microenvironment via Spatioselective Recruitment of DNA Amplifiers Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Zhenghan Di, Xueguang Lu, Jian Zhao, Ana Jaklenec, Yuliang Zhao, Robert Langer, Lele Li
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Reversible Switchability of Magnetic Anisotropy and Magnetodielectric Effect Induced by Intermolecular Motion Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Shan-Nan Du, Dan Su, Ze-Yu Ruan, Ying-Qian Zhou, Wei Deng, Wei-Xiong Zhang, Young Sun, Jun-Liang Liu, Ming-Liang Tong
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Highly Active and Stable Li2S−Cu Nanocomposite Cathodes Enabled by Kinetically Favored Displacement Interconversion between Cu2S and Li2S Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Lulu Tan, Anran Li, Yusi Yang, Jianwen Zhang, Xiaogang Niu, Nan Li, Limin Liu, Lin Guo, Yujie Zhu
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Accelerated Degradation of Microplastics at the Liquid Interface of Ice Crystals in Frozen Aqueous Solutions Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Chen Tian, Jiaxin Lv, Wenchao Zhang, Han Wang, Jin Chao, Liyuan Chai, Zhang Lin
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Restoration of the Immunogenicity of Tumor Cells for Enhanced Cancer Therapy via Nanoparticle-Mediated Copper Chaperone Inhibition Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Feixiang Ding, Fei Li, Dongsheng Tang, Bin Wang, Junyan Liu, Xiaoyuan Mao, Jiye Yin, Haihua Xiao, Jing Wang, Zhaoqian Liu
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Highly Robust CuI-TADF Emitters for Vacuum-Deposited OLEDs with Luminance up to 222 200 cd m−2 and Device Lifetimes (LT90) up to 1300 hours at an Initial Luminance of 1000 cd m−2 Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Rui Tang, Shuo Xu, Tsz-Lung Lam, Gang Cheng, Lili Du, Qingyun Wan, Jun Yang, Faan-Fung Hung, Kam-Hung Low, David Lee Phillips, Chi-Ming Che
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Water Networks Repopulate Protein–Ligand Interfaces with Temperature Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-06-01 Timothy R. Stachowski, Murugendra Vanarotti, Jayaraman Seetharaman, Karlo Lopez, Marcus Fischer
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Alkyl/Glycosyl Sulfoxides as Radical Precursors and Their Use in the Synthesis of Pyridine Derivatives** Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Demeng Xie, Yingwei Wang, Xia Zhang, Zhengyan Fu, Dawen Niu
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A Novel AgI-DNA Rod Comprising a One-Dimensional Array of 11 Silver Ions within a Double Helical Structure Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Takahiro Atsugi, Akira Ono, Miho Tasaka, Natsumi Eguchi, Shoji Fujiwara, Jiro Kondo
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Ru–Co Pair Sites Catalyst Boosts the Energetics for the Oxygen Evolution Reaction Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Xiaobo Zheng, Jiarui Yang, Zhongfei Xu, Qishun Wang, Jiabin Wu, Erhuan Zhang, Shixue Dou, Wenping Sun, Dingsheng Wang, Yadong Li
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A Practical and Scalable Approach to Fluoro-Substituted Bicyclo[1.1.1]pentanes Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Roman Bychek, Pavel K. Mykhailiuk
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Intramolecular Energy and Solvent-Dependent Chirality Transfer within a BINOL-Perylene Hetero-Cyclophane Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Guanghui Ouyang, Jessica Rühe, Yang Zhang, Mei-Jin Lin, Minghua Liu, Frank Würthner
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Diastereodivergent Synthesis of Cyclopentyl Boronic Esters Bearing Contiguous Fully Substituted Stereocenters Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Molly E. Fairchild, Adam Noble, Varinder K. Aggarwal
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Electrochemical Preparation of Porous Organic Polymer Films for High-Performance Memristors Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 You Tao, Hui Liu, Hui-Yuan Kong, Tian-Xiong Wang, Huijuan Sun, Yong Jun Li, Xuesong Ding, Lianfeng Sun, Bao-Hang Han
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S,O-Ligand Promoted meta-C−H Arylation of Anisole Derivatives via Palladium/Norbornene Catalysis Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-31 Verena Sukowski, Manuela van Borselen, Simon Mathew, M. Ángeles Fernández-Ibáñez
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Electrocatalytic Reduction of CO2 to Ethanol at Close to Theoretical Potential via Engineering Abundant Electron-Donating Cuδ+ Species Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Chengying Guo, Yihe Guo, Yanmei Shi, Xianen Lan, Yuting Wang, Yifu Yu, Bin Zhang
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Fe2+/Fe3+ Cycling for Coupling Self-Powered Hydrogen Evolution and Preparation of Electrode Catalysts Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Chang Chen, Zhengqian Fu, Fenggang Qi, Yafeng Chen, Ge Meng, Ziwei Chang, Fantao Kong, Libo Zhu, Han Tian, Haitao Huang, Xiangzhi Cui, Jianlin Shi
An Fe2+/Fe3+ cycling system has been established for efficient self-powered hydrogen evolution, in which a Zn−Fe battery with Fe3+ reduction reaction coupled Zn oxidation powers the electrolyzers of Fe2+ oxidation reaction (Fe2+OR) coupled hydrogen evolution reaction. Meanwhile, this Fe2+/Fe3+ cycling is used to prepare a multifunctional catalyst by the Fe2+OR-promoted dispersion of Pt nanoparticles
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Stabilization of Cu+ via Strong Electronic Interaction for Selective and Stable CO2 Electroreduction Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Yixiang Zhou, Yebo Yao, Rui Zhao, Xiaoxuan Wang, Zhenzhen Fu, Dewei Wang, Huaizhi Wang, Liang Zhao, Wei Ni, Zhiyu Yang, Yi-Ming Yan
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Mesoporous Polyimide-Linked Covalent Organic Framework with Multiple Redox-Active Sites for High-Performance Cathodic Li Storage Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Xiya Yang, Lei Gong, Xiaolin Liu, Pianpian Zhang, Bowen Li, Dongdong Qi, Kang Wang, Feng He, Jianzhuang Jiang
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Sirtuin-Derived Covalent Binder for the Selective Recognition of Protein Crotonylation Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Yanli Ji, Lin Sun, Yao Chen, Hongqiang Qin, Weimin Xuan
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Asymmetrically Doping a Platinum Atom into a Au38 Nanocluster for Changing the Electron Configuration and Reactivity in Electrocatalysis Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Xu Liu, Endong Wang, Meng Zhou, Yan Wan, Yuankun Zhang, Haoqi Liu, Yue Zhao, Jin Li, Yi Gao, Yan Zhu
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Electrostatic-Induced Crystal-Rearrangement of Porous Organic Cage Membrane for CO2 Capture Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Kai Qu, Jipeng Xu, Liheng Dai, Yixing Wang, Hongyan Cao, Dezhu Zhang, Yulin Wu, Weiyi Xu, Kang Huang, Cheng Lian, Xuhong Guo, Wanqin Jin, Zhi Xu
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Highly Selective Carbonylation of CH3Cl to Acetic Acid Catalyzed by Pyridine-Treated MOR Zeolite Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-30 Xudong Fang, Fuli Wen, Xiangnong Ding, Hanbang Liu, Zhiyang Chen, Zhaopeng Liu, Hongchao Liu, Wenliang Zhu, Zhongmin Liu
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Reductive Carbon–Carbon Coupling on Metal Sites Regulates Photocatalytic CO2 Reduction in Water Using ZnSe Quantum Dots Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-29 Zhi-Kun Xin, Mao-Yong Huang, Yang Wang, Yu-Ji Gao, Qing Guo, Xu-Bing Li, Chen-Ho Tung, Li-Zhu Wu
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Creation of a Yeast Strain with Co-Translationally Acylated Nucleosomes Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-29 Dan Wu, Yunfeng Zhang, Zhiheng Tang, Xiaoxu Chen, Xinyu Ling, Longtu Li, Wenbing Cao, Wei Zheng, Jiale Wu, Hongting Tang, Xiaoyun Liu, Xiaozhou Luo, Tao Liu
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From Stable PH-Ylides to α-Carbanionic Phosphines as Ligands for Zwitterionic Catalysts Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-29 Jana-Alina Zur, Michelle Schmidt, Kai-Stephan Feichtner, Prakash Duari, Julian Löffler, Thorsten Scherpf, Viktoria H. Gessner
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Spatially Controlled CO2 Conversion Kinetics in Natural Leaves for Motion Generation Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-29 Ambrose A. Melvin, Bertrand Goudeau, Wojciech Nogala, Alexander Kuhn
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Supported Anionic Gold Nanoparticle Catalysts Modified Using Highly Negatively Charged Multivacant Polyoxometalates Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-29 Kang Xia, Takafumi Yatabe, Kentaro Yonesato, Tomohiro Yabe, Soichi Kikkawa, Seiji Yamazoe, Ayako Nakata, Kazuya Yamaguchi, Kosuke Suzuki
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Synthesis of an N-Heterocylic Boryl-Stabilized Disilyne and Its Application to the Activation of Dihydrogen and C−H Bonds Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-27 Yazhou Ding, Yang Li, Jianying Zhang, Chunming Cui
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Merging the Non-Natural Catalytic Activity of Lipase and Electrosynthesis: Asymmetric Oxidative Cross-Coupling of Secondary Amines with Ketones Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-27 Chao-Jiu Long, Huan Cao, Ben-Kun Zhao, Yu-Fang Tan, Yan-Hong He, Chu-Sheng Huang, Zhi Guan
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Atroposelective Construction of Nine-Membered Carbonate-Bridged Biaryls Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-27 Shiqi Jia, Yuhong Tian, Xin Li, Pengfei Wang, Yu Lan, Hailong Yan
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Intramolecular C−H Activation as an Easy Toolbox to Synthesize Pyridine-Fused Bipolar Hosts for Blue Organic Light-Emitting Diodes Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-27 Fei Wang, Luoqiang Zhang, Weiguo Han, Zhengyang Bin, Jingsong You
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Robert Tuba Angew. Chem. Int. Ed. (IF 15.336) Pub Date : 2022-05-26
“The most important quality of a role model is humility … My favorite science outreach activity is inviting young students to our labs and showing them how beautiful the chemistry is …” Find out more about Robert Tuba in his Introducing … Profile.