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Redox Non-Innocent Monoatomic Silicon(0) Complex (‘Silylone’): Its One-Electron-Reduction Induces an Intramolecular One-Electron-Oxidation of Silicon(0) to Silicon(I) J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-07 Shenglai Yao; Arseni Kostenko; Yun Xiong; Aleš Růžička; Matthias Driess
A monoatomic zero-valent silicon(0) complex (‘silylone’) stabilized by the chelating bis(silylenyl)-ortho-carborane ligand, 1,2-(LSi)2-1,2-C2B10H10 [L = PhC(NtBu)2], has been synthesized from the redox reaction of the dipotassium bis(silylenyl)-nido-carboranate salt, 1,2-(LSi)2-1,2-C2B10H10K2, and NHC-SiCl2 (NHC = {[HCN(2,6-iPr2C6H3)]2C:}). Markedly different from previous examples, this silylone is
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Gold Catalyzed Decarboxylative Cross-Coupling of Iodoarenes J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-07 Ryan A. Daley; Aaron S. Morrenzin; Sharon R. Neufeldt; Joseph J Topczewski
This report details a decarboxylative cross-coupling of (hetero)aryl carboxylates with iodoarenes in the presence of a gold cata-lyst (>25 examples, up to 96% yield). This reaction is site specific, which overcomes prior limitations associated with gold cat-alyzed oxidative coupling reactions. The reactivity of the (hetero)aryl carboxylate correlates qualitatively to the field effect pa-rameter (Fortho)
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Cation-Exchange Induced Precise Regulation of Single Copper Site Triggers Room-Temperature Oxidation of Benzene J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-25 Huang Zhou; Yafei Zhao; Jie Gan; Jie Xu; Ying Wang; Hongwei Lv; Shi Fang; Zhiyuan Wang; Ziliang Deng; Xiaoqian Wang; Peigen Liu; Wenxin Guo; Boyang Mao; Huijuan Wang; Tao Yao; Xun Hong; Shiqiang Wei; Xuezhi Duan; Jun Luo; Yuen Wu
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Bicelles Rich in both Sphingolipids and Cholesterol and Their Use in Studies of Membrane Proteins J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-23 James M. Hutchison; Kuo-Chih Shih; Holger A. Scheidt; Sarah M. Fantin; Kristine F. Parson; George A. Pantelopulos; Haley R. Harrington; Kathleen F. Mittendorf; Shuo Qian; Richard A. Stein; Scott E. Collier; Melissa G. Chambers; John Katsaras; Markus W. Voehler; Brandon T. Ruotolo; Daniel Huster; Robert L. McFeeters; John E. Straub; Mu-Ping Nieh; Charles R. Sanders
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Electric-field mediated chemistry: uncovering and exploiting the potential of (oriented) electric fields to exert chemical catalysis and reaction control. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-18 Sason Shaik,David Danovich,Jyothish Joy,Zhanfeng Wang,Thijs Stuyver
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Tetrahedral Geometry Induction of Stable Ag–Ti Nanoclusters by Flexible Trifurcate TiL3 Metalloligand J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-24 Mei-Yan Gao; Kai Wang; Yayong Sun; Dejing Li; Bai-Qiao Song; Yassin H. Andaloussi; Michael J. Zaworotko; Jian Zhang; Lei Zhang
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Quantum Spin Liquid State in a Two-Dimensional Semiconductive Metal–Organic Framework J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-04 Yuki Misumi; Akira Yamaguchi; Zhongyue Zhang; Taku Matsushita; Nobuo Wada; Masahisa Tsuchiizu; Kunio Awaga
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Capturing Substrate Translocation in an ABC Exporter at the Atomic Level J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-24 Hendrik Göddeke; Lars V. Schäfer
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Selenomelanin: An Abiotic Selenium Analogue of Pheomelanin J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-08 Wei Cao; Naneki C. McCallum; Qing Zhe Ni; Weiyao Li; Hannah Boyce; Haochuan Mao; Xuhao Zhou; Hao Sun; Matthew P. Thompson; Claudia Battistella; Michael R. Wasielewski; Ali Dhinojwala; Matthew D. Shawkey; Michael D. Burkart; Zheng Wang; Nathan C. Gianneschi
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Reductive Cross-Coupling between Unactivated C(aryl)–N and C(aryl)–O Bonds by Chromium Catalysis Using a Bipyridyl Ligand J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-26 Jinghua Tang; Fei Fan; Xuefeng Cong; Lixing Zhao; Meiming Luo; Xiaoming Zeng
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Aerobic Photocatalytic H2 Production by a [NiFe] Hydrogenase Engineered to Place a Silver Nanocluster in the Electron Relay J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-24 Liyun Zhang; Giorgio Morello; Stephen B. Carr; Fraser A. Armstrong
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Ethylene selectivity in electrocatalytic CO2 reduction on Cu nanomaterials: a crystal phase-dependent study. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-18 Ye Chen,Zhanxi Fan,Jiong Wang,Chongyi Ling,Wenxin Niu,Zhiqi Huang,Guigao Liu,Bo Chen,Zhuangchai Lai,XiaoZhi Liu,Bing Li,Yun Zong,Lin Gu,Jinlan Wang,Xin Wang,Hua Zhang
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Heterotrimetallic Precursor with 2:2:1 Metal Ratio Requiring at Least a Pentanuclear Molecular Assembly J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-23 Haixiang Han; Jesse C. Carozza; Zheng Zhou; Yuxuan Zhang; Zheng Wei; Artem M. Abakumov; Alexander S. Filatov; Yu-Sheng Chen; Daniel J. SantaLucia; John F. Berry; Evgeny V. Dikarev
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Synthesis of Anhydroryanodol J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-01 Kang Du; Matthew J. Kier; Zachary D. Stempel; Valer Jeso; Arnold L. Rheingold; Glenn C. Micalizio
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Cobalt/Lewis Acid Catalysis for Hydrocarbofunctionalization of Alkynes via Cooperative C–H Activation J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-23 Chang-Sheng Wang; Sabrina Di Monaco; Anh Ngoc Thai; Md. Shafiqur Rahman; Benjamin Piaoxiang Pang; Chen Wang; Naohiko Yoshikai
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Spotlights on Recent JACS Publications J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-07-07 ACS Contributing Correspondents
This article has not yet been cited by other publications.
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Spotlights on Recent JACS Publications J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-29 ACS Contributing Correspondents
This article has not yet been cited by other publications.
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n-Type Molecular Photovoltaic Materials: Design Strategies and Device Applications. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-27 Qihui Yue,Wuyue Liu,Xiaozhang Zhu
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Superoxide-Based K-O2 Batteries: Highly Reversible Oxygen Redox Solves Challenges in Air Electrodes. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-10 Lei Qin,Luke Schkeryantz,Jingfeng Zheng,Neng Xiao,Yiying Wu
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Catalytic Hydrogenolysis of Aryl C-F Bonds Using a Bimetallic Rhodium-Indium Complex. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-18 James Moore,Connie C Lu
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Magnesiation of Aryl Fluorides Catalyzed by a Rhodium-Aluminum Complex. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-09 Ikuya Fujii,Kazuhiko Semba,Qiao-Zhi Li,Shigeyoshi Sakaki,Yoshiaki Nakao
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High Proton Conductivity in Ba5Er2Al2ZrO13, a Hexagonal Perovskite-Related Oxide with Intrinsically Oxygen-Deficient Layers. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-15 Taito Murakami,James R Hester,Masatomo Yashima
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Ion-assisted Resonant Injection and Charge Storage in Carbon-based Molecular Junctions. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-21 Mustafa Supur,Shailendra K Saxena,Richard L McCreery
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Dinaphthothiepine Bisimide and Its Sulfoxide: Soluble Precursors for Perylene Bisimide. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-16 Sakiho Hayakawa,Kyohei Matsuo,Hiroko Yamada,Norihito Fukui,Hiroshi Shinokubo
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"Colloid-Atom Duality" in the Assembly Dynamics of Concave Gold Nanoarrows. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-16 Chang Liu,Zihao Ou,Fucheng Guo,Binbin Luo,Wenxiang Chen,Limin Qi,Qian Chen
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Enantioselective Si-H Insertion Reactions of Diarylcarbenes for the Synthesis of Silicon-Stereogenic Silanes. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-16 Jake R Jagannathan,James C Fettinger,Jared T Shaw,Annaliese K Franz
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Shape Complementarity Modulated Self-assembly of Nanoring and Nanosphere Hetero-nanostructures. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-21 Na Li,Fan Wu,Zihong Han,Xiaofeng Wang,Yi Liu,Chenglin Yi,Shunsheng Ye,Guowei Lu,Li Yu,Zhihong Nie,Baoquan Ding
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Discovery and Total Synthesis of a Bis(Cyclotryptamine) Alkaloid Bearing the Elusive Piperidinoindoline Scaffold. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-10 Jordan J Dotson,J Logan Bachman,Miguel A Garcia-Garibay,Neil K Garg
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Cross-Electrophile Coupling of Unactivated Alkyl Chlorides. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-20 Holt A Sakai,Wei Liu,Chi Chip Le,David W C MacMillan
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Probing Electric Field Distributions in the Double Layer of a Single-Crystal Electrode with Angstrom Spatial Resolution using Raman Spectroscopy. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-17 Bao-Ying Wen,Jia-Sheng Lin,Yue-Jiao Zhang,Petar Radjenovic,Xia-Guang Zhang,Zhong-Qun Tian,Jian-Feng Li
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Total Synthesis Provides Strong Evidence: Xestocyclamine A is the Enantiomer of Ingenamine. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-16 Zhanchao Meng,Alois Fürstner
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Dual Monitoring of Surface Reactions in Real Time by Combined Surface-Plasmon Resonance and Field-Effect Transistor Interrogation. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-14 Patrik Aspermair,Ulrich Ramach,Ciril Reiner-Rozman,Stefan Fossati,Bernadette Lechner,Sergio E Moya,Omar Azzaroni,Jakub Dostalek,Sabine Szunerits,Wolfgang Knoll,Johannes Bintinger
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Efficient Targeted Degradation via Reversible and Irreversible Covalent PROTACs. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-05 Ronen Gabizon,Amit Shraga,Paul Gehrtz,Ella Livnah,Yamit Shorer,Neta Gurwicz,Liat Avram,Tamar Unger,Hila Aharoni,Shira Albeck,Alexander Brandis,Ziv Shulman,Ben-Zion Katz,Yair Herishanu,Nir London
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Measuring Aptamer Folding Energy Using a Molecular Clamp. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-03 Hao Qu,Qihui Ma,Lu Wang,Yu Mao,Michael Eisenstein,Hyongsok Tom Soh,Lei Zheng
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In Situ ATR-SEIRAS of Carbon Dioxide Reduction at a Plasmonic Silver Cathode. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-29 Elizabeth R Corson,Recep Kas,Robert Kostecki,Jeffrey J Urban,Wilson A Smith,Bryan D McCloskey,Ruud Kortlever
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Alignment and Photopolymerization of Hexa-peri-hexabenzocoronene Derivatives Carrying Diacetylenic Side Chains for Charge Transporting Application. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-08 Fang-Ju Lin,Chih-Wen Yang,Hsiu-Hui Chen,Yu-Tai Tao
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Selectivity via Cooperativity: Preferential Stabilization of the p65/14-3-3 interaction with Semi-Synthetic Natural Products. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-05 Madita Wolter,Pim de Vink,Joao Filipe Neves,Sonja Srdanovic,Yusuke Higuchi,Nobuo Kato,Andrew J Wilson,Isabelle Landrieu,Luc Brunsveld,Christian Ottmann
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Thermoresponsive Polysaccharide Graft Polymer Vesicles with Tunable Size and Structural Memory. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-07 Tomoki Nishimura,Shen Shishi,Yoshihiro Sasaki,Kazunari Akiyoshi
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Hydrogen Migration-Triggered Diradicaloid Singlet-Fission Switch. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-10 Qing Li,Yu-He Kan,Hong-Liang Xu,Zhong-Min Su
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Effects of Non-covalent Interactions on High-spin Fe(IV)-oxido Complexes. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-03 Victoria F Oswald,Justin L Lee,Saborni Biswas,Andrew C Weitz,Kaustuv Mittra,Ruixi Fan,Jikun Li,Jiyong Zhao,Michael Y Hu,Esen E Alp,Emile L Bominaar,Yisong Guo,Michael T Green,Michael P Hendrich,Andrew Scott Borovik
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A peroxodiiron(III) intermediate mediating both N-hydroxylation steps in biosynthesis of the N-nitrosourea pharmacophore of streptozotocin by SznF. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-08 Molly McBride,Debangsu Sil,Tai L Ng,Anne Marie Crooke,Grace E Kenney,Christina R Tysoe,Bo Zhang,Emily P Balskus,Amie K Boal,Carsten Krebs,J Martin Bollinger
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On the Coupling of Electron Transfer to Proton Transfer at Electrified Interfaces J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-23 Aimin Ge; Georg Kastlunger; Jinhui Meng; Per Lindgren; Jia Song; Qiliang Liu; Alexander Zaslavsky; Tianquan Lian; Andrew A. Peterson
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Electrochemical Switching of a Fluorescent Molecular Rotor Embedded within a Bistable Rotaxane. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-29 Yilei Wu,Marco Frasconi,Wei-Guang Liu,Ryan M Young,William A Goddard,Michael R Wasielewski,J Fraser Stoddart
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Supramolecular chemistry-based one -pot high-efficient separation of solubilizer-free pure semiconducting single-walled carbon nano-tubes: molecular strategy and mechanism. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-15 Naotoshi Nakashima,Masashi Fukuzawa,Kanako Nishimura,Tsuyohiko Fujigaya,Yuichi Kato,Aleksandar Tsekov Staykov
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Donor-Acceptor Dihydropyrenes Switchable with Near-Infrared Light. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-05-31 Kristin Klaue,Wenjie Han,Pauline Liesfeld,Fabian Berger,Yves Garmshausen,Stefan Hecht
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Highly Selective β-Mannosylations and β-Rhamnosylations Catalyzed by a Bis-thiourea. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-11 Qiuhan Li,Samuel Levi,Eric N Jacobsen
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ROY Reclaims Its Crown: New Ways to Increase Polymorphic Diversity. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-08 Alexandre Levesque,Thierry Maris,James D Wuest
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Stereoselective Functionalization of Racemic Cyclopropylzinc Reagents via Enantiodivergent Relay Coupling. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-12 Lun An,Fei-Fei Tong,Shu Zhang,Xingang Zhang
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Vinylene-Bridged 2D Covalent Organic Frameworks via Knoevenagel Condensation of Tricyanomesitylene. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-12 Shuai Bi,Palani Thiruvengadam,Shice Wei,Wenbei Zhang,Fan Zhang,Lusha Gao,Junsong Xu,Dongqing Wu,Jie-Sheng Chen,Fan Zhang
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Mechanism of Oxygen Evolution Catalyzed by Cobalt Oxyhydroxide: Cobalt Superoxide Species as a Key Intermediate and Dioxygen Release as a Rate-Determining Step. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-15 Aliki Moysiadou,Seunghwa Lee,Chia-Shuo Hsu,Hao Ming Chen,Xile Hu
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Elucidating the weakly reversible Cs-Pb-Br perovskite nanocrystal reaction network with high-throughput maps and transformations. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-12 Jakob C Dahl,Xingzhi Wang,Xiao Huang,Emory M Chan,A Paul Alivisatos
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Lead-Free Cs4CuSb2Cl12 Layered Double Perovskite Nanocrystals. J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-08 Tong Cai,Wenwu Shi,Sooyeon Hwang,Kanishka Kobbekaduwa,Yasutaka Nagaoka,Hanjun Yang,Katie Hills-Kimball,Hua Zhu,Junyu Wang,Zhiguo Wang,Yuzi Liu,Dong Su,Jianbo Gao,Ou Chen
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Correction to “Tailoring Passivation Molecular Structures for Extremely Small Open-Circuit Voltage Loss in Perovskite Solar Cells” J. Am. Chem. Soc. (IF 14.612) Pub Date : 2020-06-24 Shuang Yang; Jun Dai; Zhenhua Yu; Yuchuan Shao; Yu Zhou; Xun Xiao; Xiao Cheng Zeng; Jinsong Huang
Page 5782. Some molecular structures were incorrect in Figure 1c (one more −CH2– should be added in this figure). The corrected figure is shown below. Page 5783. Some molecular structures were incorrect in Figure 2a (one more −CH2– should be added in this figure). The corrected figure is shown below. Page 5785. The molecular structure was incorrect in Figure 5 (one more −CH2– should be added in this
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Metal-Catalyzed Carbon–Carbon Bond Cleavage of Unstrained Alcohols Chem. Rev. (IF 52.758) Pub Date : 2020-07-08 Marius D. R. Lutz; Bill Morandi
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Confronting Racism in Chemistry Journals. Chem. Rev. (IF 52.758) Pub Date : 2020-06-19 Cynthia J Burrows,Jiaxiang Huang,Shu Wang,Hyun Jae Kim,Gerald J Meyer,Kirk Schanze,T Randall Lee,Jodie L Lutkenhaus,David Kaplan,Christopher Jones,Carolyn Bertozzi,Laura Kiessling,Mary Beth Mulcahy,Craig W Lindsley,M G Finn,Joel D Blum,Prashant Kamat,Wonyong Choi,Shane Snyder,Courtney C Aldrich,Stuart Rowan,Bin Liu,Dennis Liotta,Paul S Weiss,Deqing Zhang,Krishna N Ganesh,Harry A Atwater,J Justin Gooding
The following joint Editorial was originally published in ACS Applied Materials & Interfaces (DOI: 10.1021/acsami.0c10979). We confront the terrible reality that systemic racism and discrimination impacts the daily personal and professional lives of many members of the scientific community and broader society. In the U.S., the brutal killing of George Floyd while in police custody is one of the most
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Classical and Emerging Characterization Techniques for Investigation of Ion Transport Mechanisms in Crystalline Fast Ionic Conductors. Chem. Rev. (IF 52.758) Pub Date : 2020-04-29 Yirong Gao,Adelaide M Nolan,Peng Du,Yifan Wu,Chao Yang,Qianli Chen,Yifei Mo,Shou-Hang Bo
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Combining Chemometrics and Sensors: Toward New Applications in Monitoring and Environmental Analysis. Chem. Rev. (IF 52.758) Pub Date : 2020-05-04 James Chapman,Vi Khanh Truong,Aaron Elbourne,Sheeana Gangadoo,Samuel Cheeseman,Piumie Rajapaksha,Kay Latham,Russell J Crawford,Daniel Cozzolino
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Functional Supramolecular Polymeric Networks: The Marriage of Covalent Polymers and Macrocycle-Based Host-Guest Interactions. Chem. Rev. (IF 52.758) Pub Date : 2020-05-19 Danyu Xia,Pi Wang,Xiaofan Ji,Niveen M Khashab,Jonathan L Sessler,Feihe Huang
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Trends in the Usage of Bidentate Phosphines as Ligands in Nickel Catalysis. Chem. Rev. (IF 52.758) Pub Date : 2020-06-03 Andrew L Clevenger,Ryan M Stolley,Justis Aderibigbe,Janis Louie
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Artificial Metaphotonics Born Naturally in Two Dimensions. Chem. Rev. (IF 52.758) Pub Date : 2020-06-04 Zhigao Dai,Guangwei Hu,Qingdong Ou,Lei Zhang,Fengnian Xia,Francisco J Garcia-Vidal,Cheng-Wei Qiu,Qiaoliang Bao
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