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Palladium-catalysed stereoselective [3 + 2] annulation of vinylethylene carbonates and tryptanthrin-based ketones Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-22 Yang Fan, Qing-Zhu Li, Jun-Long Li, Bin Zhang, Zhen Dai, Ke Xie, Rong Zeng, Liang Zou, Xiang Zhang
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The applications of catalytic asymmetric halocyclization in natural product synthesis Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-18 Jiahang Yan, Zhiqiang Zhou, Qiaoqiao He, Guzhou Chen, Hongbo Wei, Weiqing Xie
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Fissisternoids A and B, two 2′,5′-quinodihydrochalcone-based meroterpenoid enantiomers with unusual carbon skeletons from Fissistigma bracteolatum Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-19 Gui-Min Xue, Chen-Guang Zhao, Jin-Feng Xue, Hui Chen, Zhen-Zhu Zhao, Ying-Ying Si, Kun Du, Yan-Le Zhi, Wei-Sheng Feng
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A multifaceted approach towards understanding the peculiar behavior of (α)-hydroxyiminophosphonates Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-22 Thomas Toupy, Christopher Kune, Kristof Van Hecke, Loïc Quinton, Jean-Christophe M. Monbaliu
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The first N-ligand assisted Pd catalyzed asymmetric synthesis of 3-arylsuccinimides as novel antifungal leads Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-22 Jixing Lai, Juan Yang, Chen Yang, René Csuk, Baoan Song, Shengkun Li
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A mechanistic study on the regioselective Ni-catalyzed methylation–alkenylation of alkyne with AlMe3 and allylic alcohol Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-17 Jiao Liu, Deguang Liu, Wan Nie, Haizhu Yu, Jing Shi
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In situ phosphonium-containing Lewis base-catalyzed 1,6-cyanation reaction: a facile way to obtain α-diaryl and α-triaryl acetonitriles Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-11 Jian-Ping Tan, Yuan Chen, Xiaoyu Ren, Yumeng Guo, Bing Yi, Hongkui Zhang, Guowei Gao, Tianli Wang
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Key role of a π–π complex in diaryl cross-coupling between aryldiazonium salts and arylboronic acids using photosensitizer-free gold/photoredox catalysis Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-17 Yanhong Liu, Rongxiu Zhu, Chengbu Liu, Dongju Zhang
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Gold self-relay catalysis for accessing functionalized cyclopentenones bearing an all-carbon quaternary stereocenter Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-18 Fan-Tao Meng, Jing-Long Chen, Xiao-Yan Qin, Tian-Shu Zhang, Shu-Jiang Tu, Bo Jiang, Wen-Juan Hao
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Palladium-catalyzed direct construction of oxazoline-containing polycyclic scaffolds via tandem addition/cyclization of nitriles and arylboronic acids Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-15 Shu-Qiang Cui, Na Cheng, Qian-Qian Ma, Zhong-Lin Wei, Wei-Wei Liao
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Insight into the mechanism of the arylation of arenes via norbornene relay palladation through meta- to para-selectivity Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Shengnan Liu, Qiong Wang, Fang Huang, Wenjuan Wang, Chong Yang, Jianbiao Liu, Dezhan Chen
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Transition-metal-free hydroamination/defluorination/cyclization of perfluoroalkyl alkynes with amidines Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-16 Li-Wen Sun, Zi-Lun Yu, Xin-Long Luo, Mengtao Ma, Zhi-Liang Shen, Xue-Qiang Chu
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Gold-catalysed synthesis of phosphonate-substituted oxetan-3-ones – an easy access to highly strained HWE reagents Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-12 Shaista Tahir, Jonas F. Wunsch, Matthias Rudolph, Frank Rominger, A. Stephen K. Hashmi
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One-pot enantioselective construction of 3,4-dihydro-2H-1,4-oxazines over Ru/Au relay catalysis and its mechanistic serendipity Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-17 Dongfeng Yang, Chengyi Wang, Yu Wang, Guohua Liu, Tanyu Cheng, Rui Liu
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“The red cage”: implementation of pH-responsiveness within a macrobicyclic pyridinium-based molecular host Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Pablo Cortón, Hongye Wang, Iago Neira, Arturo Blanco-Gómez, Elena Pazos, Carlos Peinador, Hao Li, Marcos D. García
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Three decades of unveiling the complex chemistry of C-nitroso species with computational chemistry Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Pauline Bianchi, Jean-Christophe M. Monbaliu
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DBU-catalyzed dearomative annulation of 2-pyridylacetates with α,β-unsaturated pyrazolamides for the synthesis of multisubstituted 2,3-dihydro-4H-quinolizin-4-ones Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Yao-Bin Shen, Jian-Qiang Zhao, Zhen-Hua Wang, Yong You, Ming-Qiang Zhou, Wei-Cheng Yuan
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Alkyl-modified nucleobases with 6/5/7/5 ring systems from the insect Cyclopelta parva Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-05 Yong-Ming Yan, Heng Chen, Wen-Long Chen, Dai-Wei Wang, Li Liao, Qing Lu, Yong-Xian Cheng
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Electrochemical synthesis of functionalized gem-difluoroalkenes with diverse alkyl sources via a defluorinative alkylation process Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-03 Haoxiang Zhang, Mengze Liang, Xiao Zhang, Meng-Ke He, Chao Yang, Lin Guo, Wujiong Xia
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Sequence-sorted redox-switchable hetero[3]rotaxanes Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-27 Marius Gaedke, Henrik Hupatz, Felix Witte, Susanne M. Rupf, Clara Douglas, Hendrik V. Schröder, Lukas Fischer, Moritz Malischewski, Beate Paulus, Christoph A. Schalley
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A combined experimental and computational study of NHC-catalyzed allylation of allenoate with MBH esters: new regiospecific and stereoselective access to 1,5-enyne Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Fang Sun, Fangfang Lu, Xue Song, Wenchao Wu, Kai Zhang, Chenxia Yu, Tuanjie Li, Donghui Wei, Changsheng Yao
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Enantioselective total syntheses of marine natural products (+)-cylindricines C, D, E and their diastereomers Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Ying-Hong Huang, Zhan-Jiang Liu, Pei-Qiang Huang
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Mechanisms and origins of regioselectivities of nickel-catalyzed β,δ-vinylarylation of alkenyl esters with vinyl triflates and arylzinc reagents Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-04 Yupan Li, Wan Xu, Ting Wang, Hui Chen, Juan Li
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Pseudeurglobosins A–F, six rearranged [11]-chaetoglobosins with immunosuppressive activities from Pseudeurotium bakeri P1-1-1 Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-09 Fang-Fang Duan, Ying Gao, Jun-Jun Liu, Lin Liu, Xiao-Gang Peng, Han-Li Ruan
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Derivatization based on tetrazine scaffolds: synthesis of tetrazine derivatives and their biomedical applications Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-19 Hongbao Sun, Qinghe Xue, Chang Zhang, Haoxing Wu, Ping Feng
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Recent advances in sustainable organic transformations using methanol: expanding the scope of hydrogen-borrowing catalysis Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-27 Lalit Mohan Kabadwal, Sourajit Bera, Debasis Banerjee
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Metal-hydride hydrogen atom transfer (MHAT) reactions in natural product synthesis Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-09 Jinghua Wu, Zhiqiang Ma
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Three-component photoredox 1,2-alkylamination of styrenes with alkanes and nitrogen nucleophiles via C(sp3)–H bond cleavage Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-03 Jing Huang, Yun-Yan Liang, Xuan-Hui Ouyang, Yu-Ting Xiao, Jing-Hao Qin, Ren-Jie Song, Jin-Heng Li
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Design of chiral ferrocenylphosphine-spiro phosphonamidite ligands for ruthenium-catalyzed highly enantioselective coupling of 1,2-diols with amines Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-03 Xiao Yi, Yirui Chen, An Huang, Dingguo Song, Jiaying He, Fei Ling, Weihui Zhong
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Dinuclear zinc-catalyzed asymmetric [3 + 2] cyclization reaction for direct assembly of chiral α-amino-γ-butyrolactones bearing three stereocenters Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-06 Wen-Peng Yang, Shi-Kun Jia, Tian-Tian Liu, Yuan-Zhao Hua, Min-Can Wang
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Construction of polysubstituted spiro[2.3] or [3.3] cyclic frameworks fused with a tosylated pyrrolidine promoted by visible-light-induced photosensitization Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-04 Xintao Gu, Yin Wei, Min Shi
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Access to azonanes via Pd-catalyzed decarboxylative [5 + 4] cycloaddition with exclusive regioselectivity Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-30 Yin Liu, Yicheng He, Yang Liu, Kun Wei, Wusheng Guo
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Copper-catalyzed deaminative alkynylation of secondary amines with alkynes: selectivity switch in the synthesis of diverse propargylamines Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-10 Shengyun Hu, Huangdi Feng, Hui Xi, Yuchen Meng, Ming Li, Liliang Huang, Junhai Huang
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Construction of 6H-benzo[c]thiochromenes via a tandem reaction of arynes with thionoesters Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-10 Yi An, Fang Zhang, Guangfen Du, Zhihua Cai, Lin He
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Pt(II)-Chiral diene-catalyzed enantioselective formal [4 + 2] cycloaddition initiated by C–C bond cleavage and elucidation of a Pt(II)/(IV) cycle by DFT calculations Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-28 Takanori Shibata, Natsumi Shiozawa, Shun Nishibe, Hideaki Takano, Satoshi Maeda
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Molecular rotor based on an oxidized resorcinarene Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-02 Daniel T. Payne, Jan Labuta, Zdeněk Futera, Václav Březina, Lenka Hanyková, Mandeep K. Chahal, Jonathan P. Hill
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Nickel-catalyzed reductive aminocarbonylation of vinyl triflates with nitro compounds for the synthesis of α,β-unsaturated amides Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-01 Yong-Wang Huo, Lingyun Yao, Xinxin Qi, Xiao-Feng Wu
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Synthesis of functionalized diarylbenzofurans via Ru-catalyzed C–H activation and cyclization under air: rapid access to the polycyclic scaffold of diptoindonesin G Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-04 Lufeng Ouyang, Zhigeng Lin, Shiqi Li, Baoyin Chen, Jidan Liu, Wen-Jing Shi, Liyao Zheng
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Condensation of pyrylium salts with mixed anhydrides: aryl ethers, aryl amines and sterically congested aromatics Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-02 Daniel Grabowski, Susanne Alef, Steven Becker, Ute Müller, Gregor Schnakenburg, Sigurd Höger
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Metal-free electrochemical synthesis of α-ketoamides via decarboxylative coupling of α-keto acids with isocyanides and water Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Feng Zhao, Na Meng, Ting Sun, Jiangwei Wen, Xiaohui Zhao, Wei Wei
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Facile construction of peptidomimetics by sequential C–S/C–N bond activation of Ugi-adducts Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-30 Chao Liu, Liangliang Song, Vsevolod A. Peshkov, Erik V. Van der Eycken
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Diboron-controlled product selectivity switch in copper-catalyzed decarboxylative substitutions of alkynyl cyclic carbonates Org. Chem. Front. (IF 5.281) Pub Date : 2021-11-02 Guojing Pei, Hui Chen, Wan Xu, Tao Chen, Juan Li
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Site-specific C–H chalcogenation of quinoxalin-2(1H)-ones enabled by Selectfluor reagent Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-30 Jin-Wei Yuan, Yang Zhang, Guang-Chao Huang, Meng-Yao Ma, Teng-Yu Yang, Liang-Ru Yang, Shou-Ren Zhang, Pu Mao, Ling-Bo Qu
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Two reaction modes of 1-sulfonyl-1,2,3-triazoles and pyridinium 1,4-zwitterionic thiolates: catalyst-free synthesis of pyrido[1,2-a]pyrazine derivatives and 1,4-thiazine derivatives Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-27 Shengguo Duan, Cong Chen, Yidian Chen, Yuchen Jie, Huan Luo, Ze-Feng Xu, Bin Cheng, Chuan-Ying Li
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The dark side of photocatalysis: near-infrared photoredox catalysis for organic synthesis Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-28 Nicolas Sellet, Morgan Cormier, Jean-Philippe Goddard
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Nickel-catalyzed direct cross-coupling of heterocyclic phosphonium salts with aryl bromides Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Yan-Ying Cui, Wen-Xin Li, Na-Na Ma, Chuanji Shen, Xiaocong Zhou, Xue-Qiang Chu, Weidong Rao, Zhi-Liang Shen
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Cp*Ir(III)/chiral carboxylic acid-catalyzed enantioselective C–H alkylation of ferrocene carboxamides with diazomalonates Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Qi Mou, Ruyuan Zhao, Ruihan Niu, Seiya Fukagawa, Taiki Shigeno, Tatsuhiko Yoshino, Shigeki Matsunaga, Bo Sun
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Transfer hydrogenation of N-heteroarenes with 2-propanol and ethanol enabled by manganese catalysis Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Yingjie Gong, Jingxi He, Xiaoting Wen, Hui Xi, Zhihong Wei, Weiping Liu
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Catalyst-free synthesis of α,α-disubstituted carboxylic acid derivatives under ambient conditions via a Wolff rearrangement reaction Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Xin Ji, Zhikun Zhang, Yuzhu Wang, Yazhe Han, Huiling Peng, Fangzhu Li, Lu Liu
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NIR absorbing aromatic (antiaromatic) vinylogous carbasapphyrins (3.3.1.0.1) with built-in fused dipolar aromatic hydrocarbon: synthesis and characterization Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-25 Sumit Sahoo, Gunasekaran Velmurugan, Buddhadeb Chakraborty, Peter Comba, Harapriya Rath
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A photoredox/nickel dual-catalytic strategy for benzylic C–H alkoxylation Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-26 Min Dong, Yuqi Jia, Wei Zhou, Jinlai Gao, Xiaoqing Lv, Fan Luo, Yongqiang Zhang, Shihui Liu
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Direct intramolecular C(sp3)–H bond sulfonamidation to synthesize benzosultam derivatives under metal-free conditions Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-22 He Zhang, Meng-Chan Sun, Li-Ming Yin, Donghui Wei, Mao-Ping Song, Dandan Yang, Jun-Long Niu
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Silver-catalyzed decarboxylative radical relay difluoroalkylation–carbocyclization: convenient access to CF2-containing quinolinones Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-21 Feng Zhao, Sa Guo, Yan Zhang, Ting Sun, Bing Yang, Yong Ye, Kai Sun
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Ruthenium-catalysed chemoselective alkylation of nitroarenes with alkanols Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-13 Shuang-Shuang Ma, Rui Sun, Zi-Heng Zhang, Zheng-Kun Yu, Bao-Hua Xu
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Alkoxycarbonyl radicals from alkyloxalyl chlorides: photoinduced synthesis of isoquinolinediones under visible light irradiation Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-22 Mingjuan Ji, Liang Xu, Xiangxiang Luo, Minghui Jiang, Siyu Wang, Jian-Qiang Chen, Jie Wu
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Ring-closing metathesis of N-alkenyl-cyanamides Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-19 Damien F. Dewez, Christina Diacofotaki, Gwilherm Evano
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B(C6F5)3-catalyzed three-component tandem reaction to construct novel polycyclic quinone derivatives: synthesis of a carbonate salt chromogenic chemosensor Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-18 Bei Wang, Hong Xu, Hua Zhang, Guo-Ming Zhang, Fu-Yu Li, Shuai He, Zhi-Chuan Shi, Ji-Yu Wang
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Dual roles of bisphosphines and epoxides: Rh-catalyzed highly chemoselective and diastereoselective (3 + 2) transannulations of 1,2,3-thiadiazoles with cyanoepoxides Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-18 Ziyang Dong, Cunzhi Chen, Jing Wang, Jiaxi Xu, Zhanhui Yang
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Catalytic radical cascade cyclization of alkene-tethered enones to fused bicyclic cyclopropanols Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-12 Ying Xie, Wei Huang, Song Qin, Shaomin Fu, Bo Liu
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Wanzlick's equilibrium in tri- and tetraaminoolefins Org. Chem. Front. (IF 5.281) Pub Date : 2021-10-14 Julian Messelberger, Manoj Kumar, Stephen J. Goodner, Dominik Munz
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