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Tuning Reaction Kinetics of Fluorinated Molecules to Construct Robust Solid Electrolyte Interphases on SiOx Anode Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Shiming Chen, Zhikang Deng, Jiangxiao Li, Wenguang Zhao, Bowen Nan, Yue Zuo, Jianjun Fang, Yuxiang Huang, Zu-Wei Yin, Feng Pan, Luyi Yang
Introducing fluorinated electrolyte additives to construct LiF-rich solid-electrolyte interphase (SEI) on Si-based anodes is proven an effective strategy for coping with its massive volume changes during cycling. However, most current research on fluorine-containing additives focuses on their thermodynamics of decomposition, lacking studies on the correlation between the molecular structure of additives
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Structure-Guided Discovery of a Potent Inhibitor of the Ferric Citrate Binding Protein FecB in Vibrio Bacteria Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Jinyan Jiang, Suguru Okuda, Hideaki Itoh, Ken Okamoto, Hiromi Nakanishi, Michio Suzuki, Peng Lu, Koji Nagata
Infections caused by Gram-negative bacteria present a significant risk to human health worldwide. Novel strategies are needed to deal with the challenge caused by drug-resistant bacteria. Here, we report a new approach to combat infections by targeting iron-binding proteins to suppress bacterial growth. We investigated the function of the conserved periplasmic binding protein FecB from Vibrio alginolyticus
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Directional Ring Translocation in a pH- and Redox-Driven Tristable [2]Rotaxane Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Leonardo Andreoni, Jessica Groppi, Özlem Seven, Massimo Baroncini, Alberto Credi, Serena Silvi
We describe the synthesis and characterization of a [2]rotaxane comprising a dibenzo-24-crown-8 (DB24C8) macrocyclic component and a thread containing three recognition sites: ammonium (AmH+), bipyridinium (Bpy2+) and triazolium (Trz+). AmH+ and Bpy2+ are responsive to fully orthogonal stimuli, pH and electrochemical, which allows to precisely control the directional translation of the macrocycle along
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Competitive Li-ion Coordination Constructing Three-Dimensional Transport Network for Ultra-High Ionic Conductivity of Composite Solid-State Electrolyte Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-21 Yiteng Ma, Yong Qiu, Ke Yang, Shun Lv, Yuhang Li, Xufei An, Guanyou Xiao, Zhuo Han, Yuetao Ma, Likun Chen, Danfeng Zhang, Wei Lv, Yun Tian, Tingzheng Hou, Ming Liu, Zhen Zhou, Feiyu Kang, Yanbing He
The porous structure of poly(vinylidene fluoride) (PVDF)-based polymer electrolytes and their disordered ion transport properties restrict the continuous and highly efficient transport of lithium ion (Li+), which exists as the major challenge to further improve the ionic conductivity. Herein, we construct a compact composite solid-state electrolyte with a three-dimensional continuous Li+ transport
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A 'Seat-Squatting' Strategy via Lithium Substitution to Suppress Fe-Migration in Na layered Oxide Cathodes Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-20 Yaoshen Niu, Zilin Hu, Huican Mao, Lin Zhou, Liguang Wang, Xiaobing Lou, Bo Zhang, Dongdong Xiao, Yang Yang, Feixiang Ding, Xiaohui Rong, Ju-Ping Xu, Wen Yin, Nian Zhang, Zhiwei Li, Yaxiang Lu, Bingwen Hu, Jun Lu, Ju Li, Yong-Sheng Hu
Na-ion batteries (NIBs) are emerging as a promising alternative to Li-ion batteries (LIBs). To align with sustainability principles, the design of electrode materials must incorporate considerations for abundant and environmentally friendly elements, such as redox-active Fe. Despite its appeal, the enduring challenge of Fe migration in layered cathodes remains inadequately addressed over decades. Here
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Stabilizing LiCoO2 at 4.6 V by regulating anti-oxidative solvents Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-20 Hengyu Ren, Guorui Zheng, Yuhang Li, Shiming Chen, Xiaohu Wang, Mingzheng Zhang, Wenguang Zhao, Haocong Yi, Weiyuan Huang, Jianjun Fang, Tongchao Liu, Luyi Yang, Ming Liu, Qinghe Zhao, Feng Pan
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Air-stable and Lithium-compatible Garnet Pellet Enabled by Surface Doping for High Performance Solid-state Batteries Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-20 An-Min Cao, Sijie Guo, Tingting Wu, Siqi Lu, Suting Weng, Muyao Qi, Bing Li, Yong-Gang Sun, Sidong Zhang, Xuefeng Wang, Hong-Shen Zhang
Garnet-type solid-state electrolytes (SSEs), typically Li6.5La3Zr1.5Ta0.5O12 (LLZT), hold great promises for next-generation lithium metal batteries (LMBs). However, LLZT with a high content of reactive Li+ is air sensitive, which forms insulating and lithiophobic impurities to jeopardize its practical applications. Here, we demonstrate that crust-localized Fe3+ doping of the LLZT pellet (CF-LLZT)
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Constructing Weakly Solvating Electrolytes for Next-Generation Zn-ion Batteries Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-19 Diyu Xu, Dezhou Zheng, Fuxin Wang, Xuefeng Shang, Yi Wang, Xihong Lu
Zn-ion batteries (ZIBs) are considered as a viable candidate for grid-scale energy storage with admirable capacity, high safety and low cost, but are severely hampered by the undesirable dendrite growth and parasitic reactions at the Zn anode side. The compositions of electrolytes are critical to the performance enhancement of ZIBs. Conventional electrolytes are unable to meet the ever-growing requirements
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Electrolyte Failure and Reconstruction towards Li–S Batteries Operating from –20 °C to 100 °C Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-19 Dong Guo, Simil Thomas, Jehad El-Demellawi, Zixiong Shi, Zhiming Zhao, Christian G Canlas, Yongjiu Lei, Jian Yin, Yaping Zhang, Mohamed Nejib Hedhili, Muhammad Arsalan, Yunpei Zhu, Osman M. Bakr, Omar F F. Mohammed, Husam N. Alshareef
Lithium-sulfur (Li-S) batteries are deemed one of the most promising high-energy battery technologies. However, their operation under thermal extremes, e.g., subzero and above 60 °C, remains largely underexplored. Especially, high temperatures (HT) exacerbate sulfur dissolution and undesired side reactions, presenting significant challenges for electrolyte design. In this work, contrary to traditional
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Boosting hydrogen evolution activity: next-nearest oxygen coordination in dual-phase supra-nanostructured multiprincipal element alloy catalysts Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Fucong Lyu, Chang Liu, Shanshan Zeng, Xiuming Bu, Yuhan Chen, Zhe Jia, Youneng Xie, Ligang Sun, Zhengyi Mao, Junda Shen, Gan Li, Juanhua Luan, Yang Yan, Lu Yao, Lanxi Li, Xianying Wang, Ge Wu, Yang Yang Li, Jian Lu
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Simultaneous and efficient utilization of photogenerated electrons and holes: a case of single-atom Pd-anchored CdS twins Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Yuan Tang, Zhong-Fei Xu, Yan Sun, Chunyang Wang, Yuchen Guo, Weichang Hao, Xin Tan, Jinhua Ye, Tao Yu
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Multifunctional ternary semitransparent organic solar cell module with area above 100 cm2 and average visible transmittance above 30% Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Juxuan Xie, Ju Zhao, Zhisheng Zhou, Kai Zhang, Jiangkai Yu, Chang Zhu, Fei Huang
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Interlayer reinforcement for improved mechanical reliability for wearable perovskite solar cells Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Weilun Cai, Pengchen Zou, shiqi rong, Hui Wang, Xin Chen, Zheng Zhang, yajie wang, Chou Liu, Tinghuan Yang, Tianqi Niu, Shengye Jin, Wenming Tian, Jianxi Yao, Shengzhong Frank Liu, Kui Zhao
Flexible perovskite solar cells (F-PSCs) are emerging as a promising solution for weight-sensitive, wearable, portable, and flexible applications. However, F-PSCs still suffer from poor mechanical reliability due to weak interlayer adhesion and stress mismatch. In this study, we present a successful approach using a polyacrylamide (PAM) interlayer at the buried interface to alleviate interfacial stress
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Harnessing Trace Water for Enhanced Photocatalytic Oxidation of Biomass-Derived Alcohol to Aldehyde Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Wenhua Xue, Jian Ye, Zhi Zhu, Reeti Kumar, Jun Zhao
The photocatalytic conversion of biomass into valuable chemicals offers a more energy-efficient and low-carbon alternative to traditional thermal catalysis, representing a promising strategy for fine chemicals production without relying on fossil fuels. While most studies have focused on catalyst design to improve efficiency, the precise tuning of solvents has been neglected. This study examines the
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Surface Hydroxyl Group Dominating Aerobic Oxidation of Methane below Room Temperature† Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Baiyang Yu, Lu Cheng, Jiaju Wu, Bing Yang, Hong Li, Jing Xu, Ying Zhang, Chengsi Pan, Xiaoming Cao, Yongfa Zhu, Yang Lou
Direct oxidation of methane (DOM) using molecular oxygen (O2) and hydrogen (H2) is currently considered to be triggered by in-situ produced H2O2 or free hydroxyl radicals (•OH). However, the role of the surface hydroxyl group in DOM that is in situ formed from O2 and H2 has been long ignored. Herein, we provide experimental evidence that DOM using H2 and O2 over titanium silicate–supported single Pd
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Chemo-mechanical stable cathode interphase via interface in-situ catalytic-conversion integrated design for all solid-state batteries Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Xuanyi Zhou, Biao Zhang, Pengbo Lyu, Lei Xi, Fangkun Li, Zengsheng Ma, Min Zhu, Jun Liu
All-solid-state lithium batteries (ASSLBs) based on LiNi1-x-yCoxMnyO2 cathode suffer from rock-ribbed electrolyte-cathode interface issues such as oxygen escape and side reactions with electrolyte at high operating voltage, result in severe structure deterioration and rapid capacity decay. Herein, a kind of synergistic “catalytic conversion” integrated mechanisms is strategically exploited to in-situ
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Ion-Conductive Crystals of Poly (vinylidene fluoride) Enables Fast Charging Solid-State Lithium Metal Batteries Energy Environ. Sci. (IF 32.4) Pub Date : 2024-09-18 Chen Dai, MoWei Weng, BoWen Cai, Junfeng Liu, ShaoKe Guo, Hao Xu, Lei Yao, Florian J. Stadler, Zhong-Ming Li, Yanfei Huang
The crystalline phases of solid-state polymer electrolytes (SPEs) are commonly believed as ionic insulators. Here we show that contrary to this prevailing view, lithium-ion (Li+) can transport in crystalline phases of poly(vinylidene fluoride) (PVDF) after incorporating dipolar defects into crystals. Through increasing the interchain distance, these defects enable an easy flipping and vibrating of
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Current development, optimisation strategies and future perspectives for lead-free dielectric ceramics in high field and high energy density capacitors Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-20 Hareem Zubairi, Zhilun Lu, Yubo Zhu, Ian M. Reaney, Ge Wang
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Bioinspired superwetting oil–water separation strategy: toward the era of openness Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-20 Zhuoxing Liu, Yifan Si, Cunlong Yu, Lei Jiang, Zhichao Dong
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Enhancing electrochemical reactions in organic synthesis: the impact of flow chemistry Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-19 Morgan Regnier, Clara Vega, Dimitris I. Ioannou, Timothy Noël
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Correction: Recent progress in SERS monitoring of photocatalytic reactions Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-18 Xinlu Zheng, Ziwei Ye, Zeeshan Akmal, Chun He, Jinlong Zhang, Lingzhi Wang
Correction for ‘Recent progress in SERS monitoring of photocatalytic reactions’ by Xinlu Zheng et al., Chem. Soc. Rev., 2024, 53, 656–683, https://doi.org/10.1039/D3CS00462G.
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Stability of electrocatalytic OER: from principle to application Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-18 HuangJingWei Li, Yu Lin, Junyuan Duan, Qunlei Wen, Youwen Liu, Tianyou Zhai
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In situ characterization techniques of protein corona around nanomaterials Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-18 Fangqin Fu, Daniel Crespy, Katharina Landfester, Shuai Jiang
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The potential utility of dendritic fibrous nanosilica as an adsorbent and a catalyst in carbon capture, utilization, and storage Chem. Soc. Rev. (IF 40.4) Pub Date : 2024-09-16 Sam Yeol Lim, Sherif A. Younis, Ki-Hyun Kim, Jechan Lee
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(Z)-Selective Isomerization of 1,1-Disubstituted Alkenes by Scandium-Catalyzed Allylic C–H Activation J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Shao-Jie Lou, Pan Wang, Xin Wen, Aniket Mishra, Xuefeng Cong, Qingde Zhuo, Kun An, Masayoshi Nishiura, Yi Luo, Zhaomin Hou
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Integrated CO2 Capture and Conversion by a Robust Cu(I)-Based Metal–Organic Framework J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Debabrata Sengupta, Saptasree Bose, Xiaoliang Wang, Neil M. Schweitzer, Christos D. Malliakas, Haomiao Xie, Joshua Duncan, Kent O. Kirlikovali, Taner Yildirim, Omar K. Farha
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Aldehyde–Olefin Couplings Via Sulfoxylate-Mediated Oxidative Generation of Ketyl Radical Anions J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Zhihang Li, Joseph A. Tate, Adam Noble
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Design Principles of Catalytic Materials for CO2 Hydrogenation to Methanol Adv. Mater. (IF 27.4) Pub Date : 2024-09-19 Thaylan Pinheiro Araújo, Sharon Mitchell, Javier Pérez-Ramírez
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Maximizing Photon-to-Electron Conversion for Atom Efficient Photoredox Catalysis J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Felicity Draper, Stephen DiLuzio, Hannah J. Sayre, Le Nhan Pham, Michelle L. Coote, Egan H. Doeven, Paul S. Francis, Timothy U. Connell
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Distortion Engineering: A Strategy to Modulate Molecular Upconversion with Molecular Cluster-Aggregates J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Diogo A. Gálico, Alexandros A. Kitos, Rayan Ramdani, Jeffrey S. Ovens, Muralee Murugesu
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Engineering Screw Dislocations in Covalent Organic Frameworks J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Bhausaheb Dhokale, Kira Coe-Sessions, Michael J. Wenzel, Alathea E. Davies, Taylor Kelsey, Jonathan A. Brant, Laura de Sousa Oliveira, Bruce A. Parkinson, John O. Hoberg
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The Loss of Interfacial Water-Adsorbate Hydrogen Bond Connectivity Position Surface-Active Hydrogen as a Crucial Intermediate to Enhance Nitrate Reduction Reaction J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Shisheng Zheng, Xinzhe Yang, Zhong-Zhang Shi, Haowen Ding, Feng Pan, Jian-Feng Li
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Photocatalytic Acetylene Hydrochlorination by Pairing Proton Reduction and Chlorine Oxidation over g-C3N4/BiOCl Catalysts J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-20 Zhi-Hao Zhao, Huan Wang, Jinjin Li, Xingyue Qiao, Zhenpeng Liu, Zhipeng Ren, Menglei Yuan, Jian Zhang
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Efficient Strategy to Discover DNA Aptamers Against Low Abundance Cell Surface Proteins in Scarce Samples J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Xiaoqiu Wu, Yuqing Liu, Dengwei Zhang, Jingjing Yu, Mingxin Zhang, Shuwei Feng, Lifei Zhang, Ting Fu, Yamin Tan, Tao Bing, Weihong Tan
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Manipulating d-Band Center of Nickel by Single-Iodine-Atom Strategy for Boosted Alkaline Hydrogen Evolution Reaction J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Chongjing Liu, Beibei Sheng, Quan Zhou, Yujian Xia, Ying Zou, Peter Joseph Chimtali, Dengfeng Cao, Yongheng Chu, Sirui Zhao, Ran Long, Shuangming Chen, Li Song
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Catalyst-Free Oxidation of Styrene to Styrene Oxide Using Circulating Microdroplets in an Oxygen Atmosphere J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Lian Xue, Weida Chen, Peng Zheng, Jiao Geng, Feng Zhang, Xinyao Li, Zhibing Zhang, Xingbang Hu
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Revealing the Bro̷nsted Acidic Nature of Penta-Coordinated Aluminum Species in Dealuminated Zeolite Y with Solid-State NMR Spectroscopy J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mingji Zheng, Qiang Wang, Yueying Chu, Xuechao Tan, Weidong Huang, Yujie Xi, Yongxiang Wang, Guodong Qi, Jun Xu, Suk Bong Hong, Feng Deng
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Tautomer-Selective Fluorescence Spectroscopy of Oxyluciferin Anions J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Iden Djavani-Tabrizi, Thomas Toft Lindkvist, Jeppe Langeland, Christina Kjær, Marlowe Graham, Henrik G. Kjaergaard, Steen Brøndsted Nielsen
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Repetitive Rolling of Triptycene-Based Molecules on Cu Surfaces J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mine Konuk, Melihat Madran, Mehmet Tuna Uysal, Deniz Beşer, Alimet Sema Özen, Zehra Akdeniz, Sondan Durukanoğlu
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Modulating Decarboxylative Oxidation Photocatalysis by Ligand Engineering of Atomically Precise Copper Nanoclusters J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mohammad Bodiuzzaman, Kathiravan Murugesan, Peng Yuan, Bholanath Maity, Arunachalam Sagadevan, Naveen Malenahalli H, Song Wang, Partha Maity, Mohammed F. Alotaibi, De-en Jiang, Mutalifu Abulikemu, Omar F. Mohammed, Luigi Cavallo, Magnus Rueping, Osman M. Bakr
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The Alkynyl π Bond of sp-C Enhanced Rapid, Reversible Li–C Coupling to Accelerate Reaction Kinetics of Lithium Ions J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Jingchi Gao, Xingru Yan, Xiangyao Gu, Xinlong Fu, Qian Chang, Zhihui Zhang, Yi Wang, Changshui Huang, Yuliang Li
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Anionic Ionomer: Released Surface-Immobilized Cations and an Established Hydrophobic Microenvironment for Efficient and Durable CO2-to-Ethylene Electrosynthesis at High Current over One Month J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Mingwei Fang, Xiang Miao, Zihao Huang, Meiling Wang, Xiaochen Feng, Zewen Wang, Ying Zhu, Liming Dai, Lei Jiang
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In Situ Surfaced Mn–Mn Dimeric Sites Dictate CO Hydrogenation Activity and C2 Selectivity over MnRh Binary Catalysts J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Ke-Xiang Zhang, Zhi-Pan Liu
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Crystal Structure Determination from Powder Diffraction Patterns with Generative Machine Learning J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Eric A. Riesel, Tsach Mackey, Hamed Nilforoshan, Minkai Xu, Catherine K. Badding, Alison B. Altman, Jure Leskovec, Danna E. Freedman
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Photo- and Electrocatalytic Hydrogen Evolution by Heteroleptic Dirhodium(II,II) Complexes: Role of the Bridging and Diimine Ligands J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Piyush Gupta, Curtis E. Moore, Claudia Turro
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Electrocatalytic Aromatic Alcohols Splitting to Aldehydes and H2 Gas J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Zhao Zhang, Bing-Liang Leng, Shi-Nan Zhang, Dong Xu, Qi-Yuan Li, Xiu Lin, Jie-Sheng Chen, Xin-Hao Li
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Carbodiphosphorane-Activated Distibene and Dibismuthene Dications J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Philipp Dabringhaus, Andrew Molino, Robert J. Gilliard, Jr.
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Formal [2σ + 2σ]-Cycloaddition of Aziridines with Bicyclo[1.1.0]butanes: Access to Enantiopure 2-Azabicyclo[3.1.1]heptane Derivatives J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Shubham Dutta, Constantin G. Daniliuc, Christian Mück-Lichtenfeld, Armido Studer
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Correction to “Photoelectrochemical CO2 Reduction to CO Enabled by a Molecular Catalyst Attached to High-Surface-Area Porous Silicon” J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-19 Xiaofan Jia, Eleanor Stewart-Jones, Jose L. Alvarez-Hernandez, Gabriella P. Bein, Jillian L. Dempsey, Carrie L. Donley, Nilay Hazari, Madison N. Houck, Min Li, James M. Mayer, Hannah S. Nedzbala, Rebecca Powers
The original article contained an error in the resistivity of p-type Si wafers on page S2 of the Supporting Information. The sentence should read as follows: “All p-type wafers are B doped, <100>, SSP Prime Grade with an estimated resistance of 1–10 Ω·cm–1.” A complete corrected version of the Supporting Information is presented here. The resistivity of the wafers is correctly listed in the caption
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Synthesis of Mesoporous Catechin Nanoparticles as Biocompatible Drug-Free Antibacterial Mesoformulation J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Runfeng Lin, Gaoyang Li, Qianfeng He, Junfeng Song, Yanming Ma, Yating Zhan, Minjia Yuan, Qi Li, Dongliang Chao, Xiaomin Li, Peiyuan Wang, Tiancong Zhao, Dongyuan Zhao
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A Self-Healing Crystal That Repairs Multiple Cracks J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 Javed R. Pathan, Haripriya Balan, Patrick Commins, Arthi Ravi, Marieh B. Al-Handawi, Ian Cheng-Yi Hou, Panče Naumov, Kana M. Sureshan
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Spotlights on Recent JACS Publications, Volume 146, Issue 37 J. Am. Chem. Soc. (IF 14.4) Pub Date : 2024-09-18 ACS Contributing Correspondents
This article has not yet been cited by other publications.
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Switching CO2 Electroreduction Pathways between Ethylene and Ethanol via Tuning Microenvironment of the Coating on Copper Nanofibers Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Buxing Han, Xing Tong, Pei Zhang, Peng Chen, Zhuosen He, Xinchen Kang, Yaoyu Yin, Yingying Cheng, Meng Zhou, Lihong Jing, Ce Wang, Baocai Xu, Lirong Zheng, Xueqing Xing, Zhonghua Wu
Engineering the microenvironment of electrode surface is one of the effective means to tune the reaction pathways in CO2RR. In this work, we prepared copper nanofibers with conductive polypyrrole coating by polymerization of pyrrole using polyvinyl pyrrolidone (PVP) as template. As a result, the obtained copper nanofibers Cu/Cu2+1O/SHNC, exhibited a superhydrophobic surface, which demonstrated very
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How Can Materials Chemists Contribute to Food Supply Security in the Age of AI and Robotics? Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Ludovico Cademartiri
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Rational Design of Crystalline and Enantiomerically Pure Helicenes with Open-Shell Singlet Ground States Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Xinping Wang, Tao Wang, Shuxuan Tang, Xue Dong, Yu Zhao, Quanchun Sun, Shanshan Kong, Yue Zhao
Helicene diradical derivatives have attracted widespread attentions because of their unique magnetic and chiroptoelectronic properties, however, crystalline and enantiomerically pure forms of helicene diradicals are extremely rare. Herein, we describe the rational design and synthesis of o-quinone functionalized helicene diradicals with crystalline enantiomerical purity. Diradical dianion salt Rac-3K
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Honeycomb-Structured IrOx Foam Platelets as the Building Block of Anode Catalyst Layer in PEM Water Electrolyzer Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Zhoubing Xie, Hui Chen, Xiyang Wang, Yimin A. Wu, Zizhun Wang, Subhajit Jana, Yongcun Zou, Xiao Liang, Xiao Zhao, Xiaoxin Zou
Achieving robust long-term durability with high catalytic activity at low iridium loading remains one of great challenges for proton exchange membrane water electrolyzer (PEMWE). Herein, we report the low-temperature synthesis of iridium oxide foam platelets comprising edge-sharing IrO6 octahedral honeycomb framework, and demonstrate the structural advantages of this material for multilevel tuning
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A CaI2-Based Electrolyte Enabled by Borate Ester Anion Receptors for Reversible Ca-Organic and Ca-Se Batteries Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Zhen Hou, Rui Zhou, Kai Liu, Junwu Zhu, Biao Zhang
Passivating solid electrolyte interphases (SEIs) in Ca metal anodes constitute a long-standing challenge, as they block Ca2+ transport and inhibit reversible Ca deposition/stripping. Current solutions focus primarily on boron/aluminum-based electrolytes to mitigate such interfacial issues by producing Ca2+-conductive species, yet the complex synthetic procedure of these salts restricts the widespread
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Dynamic Organic Phosphorescence Glass by Rigid-Soft Coupling Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Meng Zhang, Xiaohui Lan, Meijuan Ding, Chaoyi Han, Xing Wang Liu, Zhengong Meng, Zhen-Qiang Yu, Zhongfu An
Organic phosphorescence glass has garnered considerable attention owing to the excellent shaping ability and photophysical behavior, but facile construction from single-component phosphors is still challenging. Herein, a rigid-soft coupling design is adopted in organic phosphors of ICO, CCO and PCO, thus preparing phosphorescence glasses through melting-quenching method to give excellent shaping ability
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Partitioning / self-assembly of artificial water channels - toward controlled permselectivity through bilayer membrane Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Dan-Dan Su, Arie van der Lee, Mihail Barboiu
Artificial water channels (AWCs) have been extensively explored to mimic natural proteins, which enables to effectively transport water while blocking ions. As one of the first AWCs, self-assembled I-quartets (HCx) have showcased high water-permselectivity that can be enhanced by improving their distribution and stability within membrane. The use of long alkyl chains (n>8) is constrained by their low
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A Low-Acidity Chloride Electrolyte Enables Exceptional Reversibility and Stability in Aqueous Tin Metal Batteries Angew. Chem. Int. Ed. (IF 16.1) Pub Date : 2024-09-20 Songyang Chang, Wentao Hou, Angelica Del Valle-Perez, Irfan Ullah, Shen Qiu, Jeileen Luciano Rodriguez, Liz M. Díaz-Vázquez, Lisandro Cunci, Gerardo Morell, Xianyong Wu
Tin (Sn) metal has emerged as a promising anode for aqueous batteries, due to its high capacity, non-toxicity, and cost-effectiveness. However, Sn metal has often been coupled with strong and corrosive sulfuric acids (2-3 M), leading to severe electrode corrosion and hydrogen evolution issues. Although high efficiency and long cycling were reported, the results were achieved using high currents to