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Two-step mineral carbonation using seawater-based industrial wastewater: an eco-friendly carbon capture, utilization, and storage process
Journal of Material Cycles and Waste Management ( IF 2.7 ) Pub Date : 2019-12-04 , DOI: 10.1007/s10163-019-00950-1
Injun Kim , Yunsung Yoo , Juhee Son , Jinwon Park , Il-Sang Huh , Dongwoo Kang

Carbon dioxide is contained in the flue gas of many industrial plants, including those producing cement and power, and makes a significant contribution to climate change. Thus, methods to reduce carbon dioxide emissions are under intensive investigation. Carbon capture, utilization, and storage (CCUS) is a technology for converting captured carbon into useful chemical compounds while reducing CO2 emissions. Thus, CCUS technology is a promising method for combating global warming. In this study, we focused on a mineral carbonation CCUS process using seawater-based industrial wastewater (SBIW). A two-step CCUS process using NaOH as an absorbent for CO2 capture was used to produce two types of metal carbonate. Inductively coupled plasma optical emission spectroscopy, X-ray diffractometry, thermogravimetric analysis, and field-emission scanning electron microscopy techniques were used for analysis. Using our new technique, we obtained high-purity NaHCO3 (92.2%) and MgCO3 ·3H2O (93%). We also found that it is possible to improve the utilization of the cations present in seawater.



中文翻译:

使用基于海水的工业废水进行两步矿物碳化:一种环保的碳捕获,利用和存储过程

许多工厂(包括生产水泥和电力的工厂)的烟道气中都含有二氧化碳,对二氧化碳的排放做出了重大贡献。因此,减少二氧化碳排放的方法正在深入研究中。碳捕获,利用和存储(CCUS)是一项用于在减少CO 2排放的同时将捕获的碳转化为有用的化合物的技术。因此,CCUS技术是应对全球变暖的一种有前途的方法。在这项研究中,我们集中于使用基于海水的工业废水(SBIW)进行矿物碳化CCUS工艺。使用NaOH作为CO 2吸收剂的两步CCUS工艺捕集用于生产两种类型的金属碳酸盐。电感耦合等离子体发射光谱,X射线衍射,热重分析和场发射扫描电子显微镜技术被用于分析。使用我们的新技术,我们获得了高纯度NaHCO 3(92.2%)和MgCO 3 ·3H 2 O(93%)。我们还发现可以提高海水中存在的阳离子的利用率。

更新日期:2019-12-04
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