Principles of photothermal gas-phase heterogeneous CO2 catalysis,Energy & Environmental Science

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Principles of photothermal gas-phase heterogeneous CO2 catalysis
Energy & Environmental Science ( IF 32.4 ) Pub Date : 2019-01-08 00:00:00 , DOI: 10.1039/c8ee02790k
Mireille Ghoussoub _{1,

2,

3,

4,

5} , Meikun Xia _{1,

2,

3,

4,

5} , Paul N. Duchesne _{1,

2,

3,

4,

5} , Dvira Segal _{2,

3,

4,

5,

6} , Geoffrey Ozin _{1,

2,

3,

4,

5}

Affiliation

Photothermal catalysis is an emerging sub-discipline of heterogeneous catalysis. It is distinct from both thermochemical catalysis driven by heat and photochemical catalysis powered by sunlight. Instead, photothermal catalysis exploits broad absorption of the solar spectrum to stimulate a combination of thermochemical and photochemical processes, which contribute synergistically to driving catalytic reactions. In particular, it is proving an effective and promising strategy for converting CO₂ to synthetic fuels. This article provides a critical appraisal of the concepts and principles underpinning the theory and practice of photothermal CO₂ catalysis. Ultimately, the goal is to gain an appreciation of the scientific, technological, economic, and environmental challenges inevitably confronted by those pursuing the development of photothermal CO₂ refineries.

中文翻译：

光热气相多相CO ₂催化原理

光热催化是非均相催化的一个新兴子学科。它不同于由热驱动的热化学催化和由阳光驱动的光化学催化。相反，光热催化利用太阳光谱的广泛吸收来刺激热化学过程和光化学过程的组合，这些过程可协同促进驱动催化反应。特别是，它证明了将CO ₂转化为合成燃料的有效且有前途的策略。本文对支撑光热CO ₂理论和实践的概念和原理进行了严格的评估催化。最终，目标是要认识到那些追求光热CO ₂精炼厂发展所不可避免地面临的科学，技术，经济和环境挑战。

更新日期：2019-01-08

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