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From scalable solution fabrication of perovskite films towards commercialization of solar cells
Energy & Environmental Science ( IF 32.4 ) Pub Date : 2018-11-30 00:00:00 , DOI: 10.1039/c8ee03025a Fei Huang 1, 2 , Mengjie Li 1, 2 , Peter Siffalovic 3, 4, 5 , Guozhong Cao 6, 7, 8 , Jianjun Tian 1, 2
Energy & Environmental Science ( IF 32.4 ) Pub Date : 2018-11-30 00:00:00 , DOI: 10.1039/c8ee03025a Fei Huang 1, 2 , Mengjie Li 1, 2 , Peter Siffalovic 3, 4, 5 , Guozhong Cao 6, 7, 8 , Jianjun Tian 1, 2
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Organic–inorganic halide perovskite solar cells (PSCs) have achieved amazing progress in terms of power conversion efficiency (PCE), rising from 3.8% to over 23.3%. Owing to perovskites’ low nucleation and crystallization activation energy (56.6–97.3 kJ mol−1), a range of low temperature and large-scale solution fabrication processes have been actively investigated for potential commercialization. Although many excellent research institutes and enterprises have emerged to advance commercialization of PSCs, the performance of devices which have large areas still lag much farther behind those of smaller lab scales. The performances of PSCs are predominantly determined by the quality of the perovskite film, which in turn, is controlled by the fabrication process. A comprehensive and in-depth understanding of the nucleation and growth process during perovskite crystallization is imperative for the further advancement of large-scale manufacturing of high quality perovskite films. This review summarizes recent advances in the commercialization of the PSCs market, and critically reviews promising large-scale solution manufacturing methods combined with their physical properties and relevant challenges with the crystallization thermodynamics and kinetics of perovskites. The hurdles and challenges of commercialization and possible approaches and solutions are discussed.
中文翻译：
从钙钛矿薄膜的可扩展解决方案制造到太阳能电池的商业化
有机-无机卤化物钙钛矿太阳能电池（PSC）在功率转换效率（PCE）方面取得了惊人的进步，从3.8％上升到23.3％以上。由于钙钛矿的低成核和结晶活化能（56.6-97.3 kJ mol -1），已经积极研究了一系列低温和大规模溶液制造工艺，以实现潜在的商业化。尽管已经出现了许多优秀的研究机构和企业来推动PSC的商业化，但是面积较大的设备的性能仍然远远落后于较小规模的实验室。PSC的性能主要取决于钙钛矿薄膜的质量，而钙钛矿薄膜的质量又受制造工艺的控制。钙钛矿结晶过程中成核和生长过程的全面深入的了解对于大规模生产高质量钙钛矿薄膜是必不可少的。这篇评论总结了PSC市场商业化的最新进展，并严格审查了有前途的大规模溶液制造方法，以及它们的物理性质以及钙钛矿的结晶热力学和动力学方面的相关挑战。讨论了商业化的障碍和挑战以及可能的方法和解决方案。
更新日期：2018-11-30
中文翻译：
从钙钛矿薄膜的可扩展解决方案制造到太阳能电池的商业化
有机-无机卤化物钙钛矿太阳能电池（PSC）在功率转换效率（PCE）方面取得了惊人的进步，从3.8％上升到23.3％以上。由于钙钛矿的低成核和结晶活化能（56.6-97.3 kJ mol -1），已经积极研究了一系列低温和大规模溶液制造工艺，以实现潜在的商业化。尽管已经出现了许多优秀的研究机构和企业来推动PSC的商业化，但是面积较大的设备的性能仍然远远落后于较小规模的实验室。PSC的性能主要取决于钙钛矿薄膜的质量，而钙钛矿薄膜的质量又受制造工艺的控制。钙钛矿结晶过程中成核和生长过程的全面深入的了解对于大规模生产高质量钙钛矿薄膜是必不可少的。这篇评论总结了PSC市场商业化的最新进展，并严格审查了有前途的大规模溶液制造方法，以及它们的物理性质以及钙钛矿的结晶热力学和动力学方面的相关挑战。讨论了商业化的障碍和挑战以及可能的方法和解决方案。
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