当前位置：
X-MOL 学术
›
Atmos. Environ.
›
论文详情
Our official English website, www.x-mol.net, welcomes your
feedback! (Note: you will need to create a separate account there.)
An emission inventory for Cl2 and HOCl in Shanghai, 2017
Atmospheric Environment ( IF 4.2 ) Pub Date : 2020-02-01 , DOI: 10.1016/j.atmosenv.2019.117220 Li Li , Sijia Yin , Ling Huang , Xin Yi , Yangjun Wang , Kun Zhang , Chel Gee Ooi , David T. Allen
Atmospheric Environment ( IF 4.2 ) Pub Date : 2020-02-01 , DOI: 10.1016/j.atmosenv.2019.117220 Li Li , Sijia Yin , Ling Huang , Xin Yi , Yangjun Wang , Kun Zhang , Chel Gee Ooi , David T. Allen
Abstract Chlorine radical plays an important role in ozone formation. However, it has not generally been included in air quality modelling in China. In this study, an emission inventory for atomic chlorine precursors was developed for Shanghai in the year 2017. Total emissions of chlorine radical precursors were estimated at 8650 tons/year. The main source sectors of chlorine precursors in Shanghai include the volatilization of disinfectants, including in water treatment (850 tons/year, accounting for 9.8% among total emissions), in cooling towers (4,000 tons/year, 46.2%), in wastewater treatment (2,700 tons/year, 31.2%), in tap water (310 tons/year, 3.6%), in swimming pools (280 tons/year, 3.2%), and in the usage of chlorine-containing disinfectants (210 tons/year, 2.4%). The contribution of sea salt heterogeneous reactions with ozone to chlorine radical precursors is estimated as 90 tons/year; this represents a lower bound on the emissions from sea salt because of other reaction pathways (e.g., the reaction of particulate chloride with N2O5). Local emissions from coal combustion and chemical manufacturing were estimated to be relatively small. This study provides a basis for further study regarding the influence of chlorine chemistry on ozone formation in Shanghai.
更新日期：2020-02-01
京公网安备 11010802027423号