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Advanced 3D nanohybrid foam based on graphene oxide: Facile fabrication strategy, interfacial synergetic mechanism, and excellent photocatalytic performance
Science China Materials ( IF 6.8 ) Pub Date : 2019-07-31 , DOI: 10.1007/s40843-019-9473-2
Xiaoyuan Zhang , Wenfeng Wei , Shan Zhang , Bianying Wen , Zhiqiang Su

Herein, a unique nanohybrid foam was fabricated with titanium dioxide (TiO2)-carbon quantum dots (CQDs) nanoparticles intercalated between graphene oxide (GO) layers via a facile and low-cost solvothermal method. Compared with pure GO foam, the fabricated GO-TiO2-CQDs foam displayed high degradation rate towards methyl orange (MO), methylene blue (MB), and rhodamine B (RhB), respectively, under the Xenon lamp irradiation. The composite foam can be used for several times and remain a high degradation rate without structural damage. The photochemical property was attributed to the 3D porous structure of GO-TiO2-CQDs foam, in which ultrafine hydrogenated TiO2-CQDs nanoparticles were densely anchored on the GO sheets. This paper provides an efficient strategy to tune the charge transport and thus enhance the photocatalytic performance by combining the semi-conductive GO and quantum dots.



中文翻译:

先进的基于氧化石墨烯的3D纳米混合泡沫:简便的制备策略,界面协同机理和出色的光催化性能

在这里,独特的纳米混合泡沫由二氧化钛(TiO 2)-碳量子点(CQDs)纳米粒子通过简便且低成本的溶剂热方法插入到氧化石墨烯(GO)层之间制成。与纯GO泡沫相比,在氙灯照射下,制成的GO-TiO 2 -CQDs泡沫分别对甲基橙(MO),亚甲基蓝(MB)和若丹明B(RhB)表现出较高的降解率。该复合泡沫可以使用多次,并且保持高降解速率而不会破坏结构。光化学性质归因于GO-TiO 2 -CQDs泡沫的3D多孔结构,其中超细氢化TiO 2-CQDs纳米颗粒紧密地锚固在GO片材上。本文提供了一种有效的策略来调节电荷传输,从而通过结合半导体GO和量子点来增强光催化性能。

更新日期:2019-07-31
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