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Terahertz gas phase spectroscopy using a high-finesse Fabry–Pérot cavity
Optica ( IF 10.4 ) Pub Date : 2019-11-21 , DOI: 10.1364/optica.6.001449
Francis Hindle , Robin Bocquet , Anastasiia Pienkina , Arnaud Cuisset , Gaël Mouret

The achievable instrument sensitivity is a critical parameter for the continued development of terahertz (THz) applications. Techniques such as cavity-enhanced techniques and cavity ring-down spectroscopy have not yet been employed at THz frequency due to the difficulties to construct a high-finesse Fabry–Pérot cavity. Here, we describe such a THz resonator based on a low-loss oversized corrugated waveguide with highly reflective photonic mirrors obtaining a finesse above 3000 around 620 GHz. These components enable a Fabry–Pérot THz absorption spectrometer with an equivalent interaction length of 1 km giving access to line intensities as low as 1027 cm1/(molecule/cm2) with a S/N ratio of 3. In addition, the intracavity optical power has allowed the Lamb dip effect to be studied with a low-power emitter; an absolute frequency accuracy better than 5 kHz can be easily obtained providing an additional solution for rotational spectroscopy.

中文翻译:

使用高级Fabry–Pérot腔的太赫兹气相光谱

可达到的仪器灵敏度是太赫兹(THz)应用持续发展的关键参数。由于难以构建高精细的法布里-珀罗腔,因此尚未在THz频率使用诸如腔增强技术和腔衰荡光谱学等技术。在这里,我们描述了一种基于THz谐振器,该谐振器基于具有高反射光子镜的低损耗超大型波纹状波导,在620 GHz频率下可获得3000以上的精细度。这些组件使法布里-珀罗特THz吸收光谱仪的等效相互作用长度为1 km,从而可以获得低至的谱线强度。10-27 厘米-1个/分子/厘米2个信噪比为3。此外,腔内光功率允许使用低功率发射器研究羔羊倾角效应。可以轻松获得优于5 kHz的绝对频率精度,从而为旋转光谱学提供了另一种解决方案。
更新日期:2019-12-21
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