MIL-101(Cr)/graphene aerogel (MIL-101(Cr)/GA) was synthesized using a two-step synthesis and used as a high efficient adsorbent for wastewater purification. The as-prepared MIL-101(Cr)/GA was characterized using XRD, FTIR and Raman spectroscopy, XPS and FESEM to investigate its structure, composition and morphology. MIL-101(Cr)/GA exhibited a 3D interconnected macroporous framework comprised of graphene sheets, on which MIL-101(Cr) particles were dispersed uniformly. Dyes, organic solvents and oils were used to evaluate the adsorption performance of MIL-101(Cr)/GA, which exhibited an excellent adsorption capacity for both anionic methyl orange (331.5 mg g⁻¹) and cationic rhodamine B (345.7 mg g⁻¹) as well as 51–101 times its own weight of various solvents/oils. In addition, the MIL-101(Cr)/GA showed superior recycling stability for dyes and a rapid adsorption rate for solvents/oils. The excellent adsorption performance was attributed to a synergistic effect between MIL-101 and the graphene aerogel. The kinetic behavior for adsorption observed for MIL-101(Cr)/GA was well-fitted by a pseudo-second-order kinetic model. It is envisaged that MIL-101(Cr)/GA will be a promising adsorbent for the removal of pollutants and wastewater purification.

MIL-101（Cr）/石墨烯气凝胶（MIL-101（Cr）/ GA）使用两步合成法合成，并用作废水净化的高效吸附剂。使用XRD，FTIR和拉曼光谱，XPS和FESEM对制得的MIL-101（Cr）/ GA进行表征，以研究其结构，组成和形态。MIL-101（Cr）/ GA展示了由石墨烯片组成的3D互连大孔骨架，MIL-101（Cr）颗粒均匀地分散在该骨架上。染料，有机溶剂和油被用来评估MIL-101（Cr）的/ GA，其表现出优异的吸附能力两者阴离子甲基橙（331.5毫克克的吸附性能^-1）和阳离子罗丹明B（345.7毫克克^{- 1个}）以及各种溶剂/油自身重量的51-101倍。此外，MIL-101（Cr）/ GA表现出优异的染料回收稳定性和对溶剂/油的快速吸附速率。优异的吸附性能归因于MIL-101和石墨烯气凝胶之间的协同作用。拟二级动力学模型很好地拟合了MIL-101（Cr）/ GA的吸附动力学行为。可以预期，MIL-101（Cr）/ GA将成为一种有前途的吸附剂，用于去除污染物和净化废水。