Halide-Based Materials and Chemistry for Rechargeable Batteries.,Angewandte Chemie International Edition

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Halide-Based Materials and Chemistry for Rechargeable Batteries.
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2019-07-30 , DOI: 10.1002/anie.201902842
Xiangyu Zhao ₁ , Zhirong Zhao-Karger ₂ , Maximilian Fichtner _{2,

3} , Xiaodong Shen ₁

Affiliation

Rechargeable batteries are considered one of the most effective energy storage technologies to bridge the production and consumption of renewable energy. The further development of rechargeable batteries with characteristics such as high energy density, low cost, safety, and a long cycle life is required to meet the ever-increasing energy-storage demands. This Review highlights the progress achieved with halide-based materials in rechargeable batteries, including the use of halide electrodes, bulk and/or surface halogen-doping of electrodes, electrolyte design, and additives that enable fast ion shuttling and stable electrode/electrolyte interfaces, as well as realization of new battery chemistry. Battery chemistry based on monovalent cation, multivalent cation, anion, and dual-ion transfer is covered. This Review aims to promote the understanding of halide-based materials to stimulate further research and development in the area of high-performance rechargeable batteries. It also offers a perspective on the exploration of new materials and systems for electrochemical energy storage.

中文翻译：

基于卤化物的可充电电池材料和化学。

可充电电池被认为是桥接可再生能源生产和消耗的最有效的能量存储技术之一。为了满足不断增长的能量存储需求，需要进一步开发具有高能量密度，低成本，安全性和长寿命的特性的可再充电电池。这篇评论重点介绍了可充电电池中基于卤化物的材料所取得的进展，包括卤化物电极的使用，电极的本体和/或表面卤素掺杂，电解质设计以及能够实现快速离子穿梭和稳定的电极/电解质界面的添加剂，以及实现新的电池化学。涵盖了基于单价阳离子，多价阳离子，阴离子和双离子转移的电池化学。这篇综述旨在增进人们对基于卤化物的材料的理解，从而促进高性能可充电电池领域的进一步研究与开发。它还为探索用于电化学储能的新材料和新系统提供了一个视角。

更新日期：2020-01-10

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