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In-situ methyl red doped MoS2 field effect transistor made by atomically thin MoS2 channel
Organic Electronics ( IF 3.2 ) Pub Date : 2024-01-01 , DOI: 10.1016/j.orgel.2023.106989
Muhammad Shamim Al Mamun , Hiroki Waizumi , Tsuyoshi Takaoka , Zhipeng Wang , Atsushi Ando , Tadahiro Komeda

Here we present the effects of Methyl Red (MR) doping on the electrical properties of the MoS2 field effect transistor (FET) in in-situ experimental system where the doping and electrical measurement are carried out in a single ultra-high vacuum chamber. A single-layered MoS2 flake was used as channel material for the FET preparation. N-type doping by MR was confirmed by the left shift of threshold voltage (Vth) and the surface vibrational change measured by Raman spectroscopy. The n-doping by MR is implied by the Fermi level shift towards greater binding energy with MR coverage, as proven by an X-ray photoelectron spectroscopy (XPS) measurement. It is estimated from XPS that the MoS2-FET device may detect the doping effect from the sub-monolayer MR. MR was detected on the MoS2 surface by the Time-of-Flight Secondary Ionization Mass Spectroscopy (ToF-SIMS). The findings may pave the way for innovations in electronic device design, with potential implications for fields ranging from nanoelectronics to sensor technology.



中文翻译:

由原子级薄MoS2沟道制成的原位甲基红掺杂MoS2场效应晶体管

在这里,我们在原位实验系统中展示了甲基红(MR)掺杂对MoS 2场效应晶体管(FET)电学性能的影响,其中掺杂和电学测量在单个超高真空室中进行。单层MoS 2薄片用作FET制备的沟道材料。通过阈值电压( V th )的左移和拉曼光谱测量的表面振动变化证实了MR的N型掺杂。X 射线光电子能谱 (XPS) 测量证明,MR 覆盖范围内的费米能级向更大结合能的转变暗示了 MR 的 n 掺杂。从XPS估计MoS 2 -FET器件可以检测来自亚单层MR的掺杂效应。通过飞行时间二次电离质谱 (ToF-SIMS)在 MoS 2表面检测到 MR。这些发现可能为电子设备设计的创新铺平道路,对从纳米电子学到传感器技术等领域都有潜在影响。

更新日期:2024-01-01
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