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Recent Development of Halide Perovskite Materials and Devices for Ionizing Radiation Detection
Chemical Reviews ( IF 51.4 ) Pub Date : 2023-02-02 , DOI: 10.1021/acs.chemrev.2c00404 Xiaoyu He 1 , Yao Deng 1 , Decai Ouyang 1 , Na Zhang 1 , Jing Wang 1 , Akshay A Murthy 2 , Ioannis Spanopoulos 3 , Saiful M Islam 4 , Qing Tu 5 , Guichuan Xing 6 , Yuan Li 1 , Vinayak P Dravid 2 , Tianyou Zhai 1
Chemical Reviews ( IF 51.4 ) Pub Date : 2023-02-02 , DOI: 10.1021/acs.chemrev.2c00404 Xiaoyu He 1 , Yao Deng 1 , Decai Ouyang 1 , Na Zhang 1 , Jing Wang 1 , Akshay A Murthy 2 , Ioannis Spanopoulos 3 , Saiful M Islam 4 , Qing Tu 5 , Guichuan Xing 6 , Yuan Li 1 , Vinayak P Dravid 2 , Tianyou Zhai 1
Affiliation
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Ionizing radiation such as X-rays and γ-rays has been extensively studied and used in various fields such as medical imaging, radiographic nondestructive testing, nuclear defense, homeland security, and scientific research. Therefore, the detection of such high-energy radiation with high-sensitivity and low-cost-based materials and devices is highly important and desirable. Halide perovskites have emerged as promising candidates for radiation detection due to the large light absorption coefficient, large resistivity, low leakage current, high mobility, and simplicity in synthesis and processing as compared with commercial silicon (Si) and amorphous selenium (a-Se). In this review, we provide an extensive overview of current progress in terms of materials development and corresponding device architectures for radiation detection. We discuss the properties of a plethora of reported compounds involving organic–inorganic hybrid, all-inorganic, all-organic perovskite and antiperovskite structures, as well as the continuous breakthroughs in device architectures, performance, and environmental stability. We focus on the critical advancements of the field in the past few years and we provide valuable insight for the development of next-generation materials and devices for radiation detection and imaging applications.
中文翻译：
用于电离辐射检测的卤化物钙钛矿材料和器件的最新进展
X射线、γ射线等电离辐射已被广泛研究并应用于医学成像、射线无损检测、核防御、国土安全和科学研究等各个领域。因此，利用高灵敏度、低成本的材料和器件来检测这种高能辐射是非常重要和可取的。与商用硅（Si）和非晶硒（ a -Se）相比，卤化物钙钛矿具有光吸收系数大、电阻率大、漏电流低、迁移率高以及合成和加工简单等优点，已成为辐射检测的有前景的候选材料。 。在这篇综述中，我们对辐射检测材料开发和相应设备架构方面的当前进展进行了广泛的概述。我们讨论了大量已报道的涉及有机-无机杂化、全无机、全有机钙钛矿和反钙钛矿结构的化合物的特性，以及器件结构、性能和环境稳定性方面的不断突破。我们专注于过去几年该领域的关键进展，并为开发用于辐射检测和成像应用的下一代材料和设备提供宝贵的见解。
更新日期：2023-02-02
中文翻译：
用于电离辐射检测的卤化物钙钛矿材料和器件的最新进展
X射线、γ射线等电离辐射已被广泛研究并应用于医学成像、射线无损检测、核防御、国土安全和科学研究等各个领域。因此，利用高灵敏度、低成本的材料和器件来检测这种高能辐射是非常重要和可取的。与商用硅（Si）和非晶硒（ a -Se）相比，卤化物钙钛矿具有光吸收系数大、电阻率大、漏电流低、迁移率高以及合成和加工简单等优点，已成为辐射检测的有前景的候选材料。 。在这篇综述中，我们对辐射检测材料开发和相应设备架构方面的当前进展进行了广泛的概述。我们讨论了大量已报道的涉及有机-无机杂化、全无机、全有机钙钛矿和反钙钛矿结构的化合物的特性，以及器件结构、性能和环境稳定性方面的不断突破。我们专注于过去几年该领域的关键进展，并为开发用于辐射检测和成像应用的下一代材料和设备提供宝贵的见解。
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