Nine-Electron Transfer of Binder Synergistic π-d Conjugated Coordination Polymers as High-Performance Lithium Storage Materials,Angewandte Chemie International Edition

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Nine-Electron Transfer of Binder Synergistic π-d Conjugated Coordination Polymers as High-Performance Lithium Storage Materials
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2022-12-01 , DOI: 10.1002/anie.202215864
Yiwen Wu ₁ , Jiadong Shen ₁ , Zhaoyu Sun ₁ , Yan Yang ₁ , Fangkun Li ₁ , Shaomin Ji ₂ , Min Zhu ₁ , Jun Liu ₁

Affiliation

The π-d conjugated coordination polymer Ni-DHBQ exhibits an ultra-high lithium storage capacity of 9-electron transfer and excellent rate performance due to its multiple redox active centers, π-d conjugation and laminar structure. Meanwhile, the binder CMC, like an octopus, has an appropriate interaction with both the ligand and Ni²⁺ of Ni-DHBQ, thus reducing the solubility of Ni-DHBQ and enhancing its cycle life.

中文翻译：

结合剂协同π-d共轭配位聚合物的九电子转移作为高性能储锂材料

π-d共轭配位聚合物Ni-DHBQ由于具有多个氧化还原活性中心、π-d共轭和层状结构，表现出超高的9电子转移储锂能力和优异的倍率性能。同时，粘合剂CMC像章鱼一样，与Ni-DHBQ的配体和Ni ²⁺均有适度的相互作用，从而降低了Ni-DHBQ的溶解度，提高了其循环寿命。

更新日期：2022-12-01

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