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Superconductivity and magnetism in a novel La0.85Ga0.15FeAsO compound
Physica C: Superconductivity and its Applications ( IF 1.3 ) Pub Date : 2022-08-28 , DOI: 10.1016/j.physc.2022.1354139
C. Boyraz , P. Aksu , A. Guler , Y. Oner

We report magnetization measurements on samples of La0.85Ga0.15FeAsO in the wide temperature range of 10 K-400 K, up to the field of 90 kOe having been prepared by solid-state reaction. This novel compound crystallizes with the tetragonal ZrCuSiAs-type structure. The crystal structure was determined by X-ray powder diffraction (P4/nmm: a = 4.032 Å, and c = 8.741 Å).

Temperature dependence of magnetization for this compound is measured with zero-field cooling (ZFC) and field cooling (FC) with an application of H = 50 Oe. The large bifurcation between the ZFC and FC curves has been observed starting at around 370 K. At lower temperatures below Tscseton 37 K, superconductivity and magnetism coexist. Intermediate temperature range (37 K< T < 300 K), the sample is in a mixed state of the ferromagnetic clusters with paramagnetic moments, described well by the Modified Curie Weiss expression. At higher temperatures above 360 K, it is a pure paramagnetic, described perfectly by the simple Curie-Weiss expression.

The natures of the superconducting flux-pinning centers are revealed based on analysis of the pinning force, Fpin at T = 10 K. The normalized pinning force, Fp/Fp, max versus H indicates the filamentary character owing to the pinning parameters, p = 0.5, q = 2. These results point out that, in the superconductivity, the dominance of grain boundary with single-vortex pinning (μ =1/7) mechanism

The Curie temperature, Tcurie was estimated using the modified Arrot plots. The critical exponents, β, ϒ, and δ were estimated, and their values are in close agreement with those predicted for a mean-field-like behavior at a magnetic phase transition.



中文翻译:

新型 La0.85Ga0.15FeAsO 化合物的超导性和磁性

我们报告了在 10 K-400 K 的宽温度范围内对 La 0.85 Ga 0.15 FeAsO样品进行的磁化测量,通过固态反应制备了高达 90 kOe 的磁场。这种新型化合物以四方 ZrCuSiAs 型结构结晶。晶体结构由 X 射线粉末衍射测定(P4/nmm:a  = 4.032 Å,c  = 8.741 Å)。

该化合物的磁化温度依赖性通过零场冷却 (ZFC) 和场冷却 (FC) 以及H  = 50 Oe 的应用来测量。从大约 370 K 开始观察到 ZFC 和 FC 曲线之间的大分岔。在低于sCse-n 37 K,超导和磁共存。中间温度范围(37 K < T < 300 K),样品处于具有顺磁矩的铁磁团簇的混合状态,由修正的居里魏斯表达式很好地描述。在高于 360 K 的较高温度下,它是纯顺磁性的,由简单的居里-魏斯表达式完美描述。

基于对T = 10 K 时的钉扎力 F pin的分析揭示了超导通量钉扎中心的性质 。归一化钉扎力 F p /F p 最大与 H 的关系表明由于钉扎参数而导致的丝状特征, p  = 0.5, q  = 2。这些结果表明,在超导中,单涡钉扎(μ =1/7)机制的晶界占主导地位

使用修改后的 Arrot 图估计居里温度 T居里。估计了临界指数 β、ϒ 和 δ,它们的值与磁相变中的平均场样行为的预测值非常一致。

更新日期:2022-08-28
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