Understanding Synthesis–Structure–Performance Correlations of Nanoarchitectured Activated Carbons for Electrochemical Applications and Carbon Capture,Advanced Functional Materials

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Understanding Synthesis–Structure–Performance Correlations of Nanoarchitectured Activated Carbons for Electrochemical Applications and Carbon Capture
Advanced Functional Materials ( IF 18.5 ) Pub Date : 2022-08-07 , DOI: 10.1002/adfm.202204714
Songtao Zhang ₁ , Mingbo Zheng ₂ , Yijian Tang ₁ , Rui Zang ₂ , Xinyu Zhang ₁ , Xiang Huang ₁ , Yong Chen ₃ , Yusuke Yamauchi _{4,

5} , Stefan Kaskel ₆ , Huan Pang ₁

Affiliation

Activated carbons are one of the most important classes of high-surface-area porous materials. Owing to their unique structure, low price, and large-scale production technology, these porous carbons have been traditionally used as sorbents for eliminating contamination. In the past decade, many innovations have been seen in the synthesis, structure, applications, and theoretical and experimental methods. Herein, a comprehensive review of the up-to-date progress of activated carbons is presented from the viewpoint of synthetic chemistry and materials science. First, the critical textural properties are discussed, with special emphasis on the porous texture, heteroatom doping, surface functional groups, and partial graphitization. Next, the advanced synthetic strategies of activated carbons are summarized. Special attention is given to the reaction mechanism between activating agents and carbon sources, as well as the design of controlled forms and morphology. Then, their applicability in various emerging fields is covered, including supercapacitors, capacitive deionization, batteries, electrocatalysis, and carbon capture. In particular, this review highlights the potential synthesis–structure–property correlations of these porous materials. Finally, we present the future challenges and outlook for their success in energy and environmental science.

中文翻译：

了解用于电化学应用和碳捕获的纳米结构活性炭的合成-结构-性能相关性

活性炭是最重要的一类高表面积多孔材料。由于其独特的结构、低廉的价格和大规模的生产技术，这些多孔碳传统上被用作消除污染的吸附剂。在过去的十年中，在合成、结构、应用、理论和实验方法等方面出现了许多创新。本文从合成化学和材料科学的角度全面回顾了活性炭的最新进展。首先，讨论了关键的织构特性，特别强调了多孔织构、杂原子掺杂、表面官能团和部分石墨化。接下来，总结了活性炭的先进合成策略。特别关注活化剂和碳源之间的反应机理，以及受控形式和形态的设计。然后，涵盖了它们在各种新兴领域的应用，包括超级电容器、电容去离子、电池、电催化和碳捕获。特别是，这篇综述强调了这些多孔材料潜在的合成-结构-性能相关性。最后，我们介绍了他们在能源和环境科学领域取得成功的未来挑战和前景。这篇综述强调了这些多孔材料潜在的合成-结构-性能相关性。最后，我们介绍了他们在能源和环境科学领域取得成功的未来挑战和前景。这篇综述强调了这些多孔材料潜在的合成-结构-性能相关性。最后，我们介绍了他们在能源和环境科学领域取得成功的未来挑战和前景。

更新日期：2022-08-07

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