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Peculiarity of magnetocaloric and magnetoresistance effects in Ni–Mn–Sn–Fe alloy with successive metamagnetic structural transitions
Intermetallics ( IF 4.3 ) Pub Date : 2022-08-04 , DOI: 10.1016/j.intermet.2022.107651
Hehe Zhang , Xuexi Zhang , Yuchen Xiao , Man Yang , Ziqi Xu , Zongxiang Yao , Mingfang Qian , Liping Zhang , Limeng Yin , Dongyong Jia

Magnetocaloric and magnetoresistance properties originated from a metamagnetic structural transition were investigated in a Fe-doped Ni46.8Mn38.1Sn11.6Fe3.5 alloy. After annealing, the alloy exhibited the intermartensite phase that contributed to the multiple abrupt magnetization and resistivity changes during heating process of martensite transformation. As a result, three successive magnetic entropy change ΔSM peaks of 10.7, 14.5 and 9.7 J/kg·K at temperatures 275, 279 and 285 K respectively were observed, which was responsible for a wide working temperature span ΔTFWHM of 273–287 K and thus a large effective refrigeration capacity RCeff of 98.1 J/kg under 5.0 T. At the same time, a large negative magnetoresistance MR (e.g. over 26.7% at 275 K) was also revealed during heating process under 5.0 T. Such multi-functional magnetocaloric and magnetoresistance effects render Ni–Mn–Sn–Fe alloys promising working materials for magnetic refrigerants, information storage and thermal magnetoelectricity conversions.



中文翻译:

具有连续超磁结构转变的 Ni-Mn-Sn-Fe 合金中磁热和磁阻效应的特殊性

在铁掺杂的 Ni 46.8 Mn 38.1 Sn 11.6 Fe 3.5合金中研究了源自超磁结构转变的磁热和磁阻特性。退火后合金呈现出马氏体间相,在马氏体转变加热过程中产生了多次突变磁化和电阻率变化。结果,在 275、279 和 285 K 温度下分别观察到三个连续的磁熵变化ΔS M峰,分别为 10.7、14.5 和 9.7 J/kg·K,这导致工作温度跨度ΔT FWHM为 273-287 K,因此有效制冷量RC在 5.0 T 下的eff为 98.1 J/kg。同时,在 5.0 T 下的加热过程中也显示出较大的负磁阻MR(例如,在 275 K 时超过 26.7%)。这种多功能磁热和磁阻效应使 Ni– Mn-Sn-Fe 合金有望成为磁性制冷剂、信息存储和热磁电转换的工作材料。

更新日期:2022-08-05
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