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Molecular-Switch-Embedded Solution-Processed Semiconductors
Advanced Materials ( IF 27.4 ) Pub Date : 2022-08-04 , DOI: 10.1002/adma.202203401
Seong Hoon Yu 1 , Syed Zahid Hassan 1 , Chan So 1 , Mingyun Kang 1 , Dae Sung Chung 1
Affiliation  

Recent improvements in the performance of solution-processed semiconductor materials and optoelectronic devices have shifted research interest to the diversification/advancement of their functionality. Embedding a molecular switch capable of transition between two or more metastable isomers by light stimuli is one of the most straightforward and widely accepted methods to potentially realize the multifunctionality of optoelectronic devices. A molecular switch embedded in a semiconductor can effectively control various parameters such as trap-level, dielectric constant, electrical resistance, charge mobility, and charge polarity, which can be utilized in photoprogrammable devices including transistors, memory, and diodes. This review classifies the mechanism of each optoelectronic transition driven by molecular switches regardless of the type of semiconductor material or molecular switch or device. In addition, the basic characteristics of molecular switches and the persisting technical/scientific issues corresponding to each mechanism are discussed to help researchers. Finally, interesting yet infrequently reported applications of molecular switches and their mechanisms are also described.

中文翻译:

分子开关嵌入式溶液处理半导体

溶液处理的半导体材料和光电器件性能的最新改进已将研究兴趣转移到其功能的多样化/发展上。嵌入能够通过光刺激在两种或多种亚稳态异构体之间转换的分子开关是潜在实现光电器件多功能性的最直接和广泛接受的方法之一。嵌入半导体中的分子开关可以有效控制陷阱能级、介电常数、电阻、电荷迁移率和电荷极性等各种参数,可用于晶体管、存储器和二极管等光可编程器件。这篇综述对分子开关驱动的每个光电跃迁的机制进行了分类,而不管半导体材料或分子开关或器件的类型如何。此外,还讨论了分子开关的基本特征以及与每种机制相对应的持续存在的技术/科学问题,以帮助研究人员。最后,还描述了有趣但不常报道的分子开关及其机制的应用。
更新日期:2022-08-04
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