Carbon capture, utilization, and storage (CCUS) is a promising pathway to decarbonize fossil-based power and industrial sectors and is a bridging technology for a sustainable transition to a net-zero emission energy future. This work provides an overview of process systems engineering (PSE) research challenges, advances, and opportunities for CCUS applications. We review PSE methods, tools, and techniques in process modeling, simulation, optimization, control, material screening, strategic planning, and supply chain network design for CO₂ management. We also attempt to give a PSE perspective on emerging CCUS research interests in molecular and materials systems engineering, multiscale modeling and optimization, systems design and integration under uncertainty, and the application of intelligent systems. The purpose is not to cover all aspects of PSE research for CCUS but rather to foster discussion by presenting some plausible future directions and ideas.

碳捕集、利用和封存 (CCUS) 是实现化石能源和工业部门脱碳的一条有前景的途径，也是可持续过渡到净零排放能源未来的桥梁技术。这项工作概述了 CCUS 应用的过程系统工程 (PSE) 研究挑战、进展和机遇。_{我们回顾了 CO 2}的过程建模、模拟、优化、控制、材料筛选、战略规划和供应链网络设计中的 PSE 方法、工具和技术管理。我们还试图对新兴的 CCUS 研究兴趣在分子和材料系统工程、多尺度建模和优化、不确定性下的系统设计和集成以及智能系统的应用等方面提供 PSE 视角。目的不是涵盖 CCUS 的 PSE 研究的所有方面，而是通过提出一些似是而非的未来方向和想法来促进讨论。