In this study, an innovative wet carbonation process was developed to prepare aragonite whisker-rich materials (AWM) from cement and simulated flue gas, which subsequently served as micro-fiber additions to cement. The parameters including temperature, duration and MgCl₂ concentration governing the aragonite formation were investigated, and the formation mechanism was explored. The results showed that needle-like aragonite whisker with a single crystal length of 10–30 μm and diameter of 0.5–2 μm could be synthesized rapidly when the cement suspension containing 0.05 M/L MgCl₂ was carbonated at 80 °C. The formation of aragonite was favored in a suspension with a high concentration of Ca²⁺ and a minimum Mg²⁺/Ca²⁺ molar ratio >0.12. Additionally, amorphous phases including alumina-silica gel and silica gel were also detected. By mixing the AWM with cement, a new type of micro-fiber reinforced cement was developed, which showed significant mechanical performance improvement and embodied CO₂ content (25.3 %).

在这项研究中，开发了一种创新的湿法碳化工艺，用于从水泥和模拟烟气中制备富含文石晶须的材料 (AWM)，随后将其用作水泥中的微纤维添加剂。研究了影响文石形成的温度、持续时间和MgCl _{2浓度等参数，并探讨了其形成机制。结果表明，含0.05 M/L MgCl 2}的水泥悬浮液在80 ℃碳化时，可以快速合成出单晶长10~30 μm、直径0.5~2 μm的针状文石晶须。^{在具有高浓度 Ca 2+}和最小 Mg ²⁺ /Ca ²⁺的悬浮液中有利于文石的形成摩尔比 > 0.12。此外，还检测到了非晶相，包括氧化铝-硅胶和硅胶。通过将 AWM 与水泥混合，开发了一种新型的微纤维增强水泥，该水泥显示出显着的机械性能改进并体现了 CO ₂含量（25.3 %）。