Greenificated Molecularly Imprinted Materials for Advanced Applications,Advanced Materials

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Greenificated Molecularly Imprinted Materials for Advanced Applications
Advanced Materials ( IF 27.4 ) Pub Date : 2022-06-23 , DOI: 10.1002/adma.202203154
Abbas Ostovan _{1,

2} , Maryam Arabi _{1,

2} , Yunqing Wang _{1,

2} , Jinhua Li _{1,

2} , Bowei Li _{1,

2} , Xiaoyan Wang ₃ , Lingxin Chen _{1,

2,

4,

5}

Affiliation

Molecular imprinting technology (MIT) produces artificial binding sites with precise complementarity to substrates and thereby is capable of exquisite molecular recognition. Over five decades of evolution, it is predicted that the resulting host imprinted materials will overtake natural receptors for research and application purposes, but in practice, this has not yet been realized due to the unsustainability of their life cycles (i.e., precursors, creation, use, recycling, and end-of-life). To address this issue, greenificated molecularly imprinted polymers (GMIPs) are a new class of plastic antibodies that have approached sustainability by following one or more of the greenification principles, while also demonstrating more far-reaching applications compared to their natural counterparts. In this review, the most recent developments in the delicate design and advanced application of GMIPs in six fast-growing and emerging fields are surveyed, namely biomedicine/therapy, catalysis, energy harvesting/storage, nanoparticle detection, gas sensing/adsorption, and environmental remediation. In addition, their distinct features are highlighted, and the optimal means to utilize these features for attaining incredibly far-reaching applications are discussed. Importantly, the obscure technical challenges of the greenificated MIT are revealed, and conceivable solutions are offered. Lastly, several perspectives on future research directions are proposed.

中文翻译：

用于高级应用的绿色分子印迹材料

分子印迹技术（MIT）产生与底物精确互补的人工结合位点，从而能够进行精细的分子识别。经过 5 年的进化，据预测，由此产生的宿主印迹材料将超越天然受体用于研究和应用目的，但在实践中，由于其生命周期的不可持续性（即前体、创造、使用、回收和报废）。为了解决这个问题，绿色分子印迹聚合物 (GMIP) 是一类新的塑料抗体，它通过遵循一个或多个绿色化原则实现了可持续性，同时与天然对应物相比，还展示了更深远的应用。在本次审查中，调查了 GMIP 在六个快速发展和新兴领域的精细设计和先进应用的最新进展，即生物医学/治疗、催化、能量收集/存储、纳米粒子检测、气体传感/吸附和环境修复。此外，还强调了它们的独特特性，并讨论了利用这些特性实现影响深远的应用的最佳方法。重要的是，绿色麻省理工学院的晦涩技术挑战被揭示，并提供了可以想象的解决方案。最后，提出了未来研究方向的几个观点。气体传感/吸附和环境修复。此外，还强调了它们的独特特性，并讨论了利用这些特性实现影响深远的应用的最佳方法。重要的是，绿色麻省理工学院的晦涩技术挑战被揭示，并提供了可以想象的解决方案。最后，提出了未来研究方向的几个观点。气体传感/吸附和环境修复。此外，还强调了它们的独特特性，并讨论了利用这些特性实现影响深远的应用的最佳方法。重要的是，绿色麻省理工学院的晦涩技术挑战被揭示，并提供了可以想象的解决方案。最后，提出了未来研究方向的几个观点。

更新日期：2022-06-23

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