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Electrochemical atomic force microscopy of two-dimensional trinuclear ruthenium clusters molecular assembly and dynamics under redox state control
Nanoscale ( IF 5.8 ) Pub Date : 2022-06-09 , DOI: 10.1039/d2nr01666d Soichiro Yoshimoto 1 , Jinnosuke Kato 2 , Hiroki Sakamoto 3 , Hironori Minamoto 2 , Keita Daicho 4 , Kazuki Takamura 4 , Naoki Shimomoto 4 , Masaaki Abe 4
Nanoscale ( IF 5.8 ) Pub Date : 2022-06-09 , DOI: 10.1039/d2nr01666d Soichiro Yoshimoto 1 , Jinnosuke Kato 2 , Hiroki Sakamoto 3 , Hironori Minamoto 2 , Keita Daicho 4 , Kazuki Takamura 4 , Naoki Shimomoto 4 , Masaaki Abe 4
Affiliation
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Mixed-valence ruthenium trinuclear clusters containing dichloroacetates were synthesized, and the self-assembly of a single molecular adlayer composed of these clusters on a graphite surface was investigated by atomic force microscopy (AFM). AFM clearly revealed the dynamics of two-dimensional (2D) structure formation as well as the molecular characteristics of the adlayers at different electrochemical interfaces. The results verified that the design of metal complexes is important not only for redox chemistry but also for molecular assembly and nanoarchitecture construction.
中文翻译：
氧化还原态控制下二维三核钌簇分子组装和动力学的电化学原子力显微镜
合成了含有二氯乙酸盐的混合价钌三核簇，并通过原子力显微镜 (AFM) 研究了由这些簇组成的单个分子吸附层在石墨表面的自组装。AFM 清楚地揭示了二维 (2D) 结构形成的动力学以及不同电化学界面处的 adlayer 的分子特征。结果证实，金属配合物的设计不仅对氧化还原化学很重要，而且对分子组装和纳米结构构建也很重要。
更新日期：2022-06-14
中文翻译：
氧化还原态控制下二维三核钌簇分子组装和动力学的电化学原子力显微镜
合成了含有二氯乙酸盐的混合价钌三核簇，并通过原子力显微镜 (AFM) 研究了由这些簇组成的单个分子吸附层在石墨表面的自组装。AFM 清楚地揭示了二维 (2D) 结构形成的动力学以及不同电化学界面处的 adlayer 的分子特征。结果证实，金属配合物的设计不仅对氧化还原化学很重要，而且对分子组装和纳米结构构建也很重要。
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