Chiral Bioinspired Plasmonics: A Paradigm Shift for Optical Activity and Photochemistry,ACS Photonics

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Chiral Bioinspired Plasmonics: A Paradigm Shift for Optical Activity and Photochemistry
ACS Photonics ( IF 6.5 ) Pub Date : 2022-06-07 , DOI: 10.1021/acsphotonics.2c00445
Oscar Ávalos-Ovando _{1,

2} , Eva Yazmin Santiago ₂ , Artur Movsesyan _{1,

2} , Xiang-Tian Kong ₃ , Peng Yu _{1,

4} , Lucas V. Besteiro ₅ , Larousse Khosravi Khorashad ₆ , Hiromi Okamoto ₇ , Joseph M. Slocik ₈ , Miguel A. Correa-Duarte ₅ , Miguel Comesaña-Hermo ₉ , Tim Liedl ₁₀ , Zhiming Wang _{1,

11} , Gil Markovich ₁₂ , Sven Burger _{13,

14} , Alexander O. Govorov ₂

Affiliation

Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China
Department of Physics and Astronomy and Nanoscale and Quantum Phenomena Institute, Ohio University, Athens, Ohio 45701, United States
School of Physics, Nankai University, Tianjin 300071, China
College of Optoelectronic Technology, Chengdu University of Information Technology, Chengdu, 610225, China
CINBIO, Universidade de Vigo, 36310 Vigo, Spain
Department of Electrical & Computer Engineering, University of Nebraska─Lincoln, Lincoln, Nebraska 68588, United States
Institute for Molecular Science and Graduate University for Advanced Studies (SOKENDAI), Okazaki, Aichi 444-8585, Japan
Soft Matter Materials Branch, Materials and Manufacturing Directorate, Air Force Research Laboratory, Wright Patterson Air Force Base, Ohio 45433-7750, United States
CNRS, ITODYS, Université de Paris, F-75013 Paris, France
Faculty of Physics and Center for NanoScience (CeNS), Ludwig Maximilians University, 80539 Munich, Germany
Institute for Advanced Study, Chengdu University, Chengdu 610106, China
School of Chemistry, Raymond and Beverly Sackler Faculty of Exact Sciences, Tel Aviv University, Tel Aviv 6997801, Israel
Zuse Institute Berlin, 14195 Berlin, Germany
JCMwave GmbH, 14050 Berlin, Germany

This Perspective concerns the latest developments in the field of chiral nanocrystals (NCs) and metastructures, focusing primarily on plasmonic nanostructures. Such nanomaterials exhibit unusually strong near-field and electromagnetic responses that enable efficient biosensing and light manipulation. Herein we share our thoughts on the latest trends that mark what we call a paradigm shift for the vast and dynamic field of chiroptical materials. The topics to be considered include polarization-sensitive photocatalysis with chiral plasmonic NCs, chiral bioconjugates, DNA-based assemblies, chiral growth, and we also describe the fundamental challenges for optical induction of chirality, transfer of chirality between different scales, and theoretical issues that nanoscience is facing.

中文翻译：

手性仿生等离子体：光学活动和光化学的范式转变

本展望关注手性纳米晶体 (NC) 和超结构领域的最新发展，主要关注等离子体纳米结构。这种纳米材料表现出异常强的近场和电磁响应，可实现有效的生物传感和光操纵。在此，我们分享我们对最新趋势的看法，这些趋势标志着我们所谓的手性材料广阔而动态领域的范式转变。需要考虑的主题包括手性等离子体 NC 的偏振敏感光催化、手性生物共轭物、基于 DNA 的组装、手性生长，我们还描述了手性的光学诱导、不同尺度之间的手性转移以及理论问题的基本挑战。纳米科学面临。

更新日期：2022-06-07

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