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Nanoarchitectonics of low-dimensional metal-organic frameworks toward photo/electrochemical CO2 reduction reactions
Journal of CO2 Utilization ( IF 7.2 ) Pub Date : 2022-01-07 , DOI: 10.1016/j.jcou.2022.101883
Xiaoxu Xuan 1, 2 , Mengjie Wang 1 , Meng Zhang 3 , Yusuf Valentino Kaneti 4 , Xingtao Xu 5 , Xun Sun 1, 2 , Yusuke Yamauchi 4, 5
Affiliation  

Low-dimensional metal-organic frameworks (LD MOFs) have attracted increasing attention in recent years. Their unique properties, including ultrathin structures, fully exposed active sites, and tunable compositions make them excellent catalysts for CO2 catalytic reduction. Even though numerous efforts have been attempted to modify the morphologies of LD MOFs, it is still highly important to explore the synthetic principles and catalytic properties of LD MOFs. In this review, various synthetic methods for preparing LD MOFs are summarized. The unique properties and applications of LD MOFs in CO2 catalytic reduction reaction are introduced and discussed. Finally, several challenges and prospects of this emerging research field are proposed. The present review could provide a comprehensive understanding on the design and synthesis of LD MOFs for CO2 reduction.



中文翻译:

低维金属有机框架的纳米结构对光/电化学 CO2 还原反应

近年来,低维金属有机框架(LD MOFs)引起了越来越多的关注。它们的独特性能,包括超薄结构、完全暴露的活性位点和可调节的组成,使其成为 CO 2催化还原的出色催化剂。尽管已经尝试了许多努力来改变 LD MOFs 的形态,但探索 LD MOFs 的合成原理和催化性能仍然非常重要。在这篇综述中,总结了制备 LD MOF 的各种合成方法。LD MOFs在CO 2 中的独特性能和应用介绍和讨论了催化还原反应。最后,提出了这一新兴研究领域的几个挑战和前景。本综述可以全面了解用于减少CO 2的 LD MOF 的设计和合成。

更新日期:2022-01-08
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