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CO2 absorption intensification using three-dimensional printed dynamic polarity packing in a bench-scale integrated CO2 capture system
AIChE Journal ( IF 3.5 ) Pub Date : 2022-01-04 , DOI: 10.1002/aic.17570
Min Xiao 1 , Moushumi Sarma 1 , Jesse Thompson 1, 2 , Du Nguyen 3 , Samantha Ruelas 3 , Kunlei Liu 1, 4
Affiliation  

Postcombustion carbon capture using a chemical absorbent is a promising technology to reduce CO2 emission. However, the overall construction and operating costs remain a major challenge. In order to intensify the absorption process and to reduce these costs, a novel dynamic polarity structured packing (DP packing) with alternate patterns of surface polarity has been developed to enhance local macro-scale turbulence within the advanced viscous solvent to reduce the mass transfer diffusion resistance. Three DP structured packings that incorporate multiple polymeric materials were fabricated using three-dimensional printing technique and evaluated through parametric testing using a bench-scale integrated CO2 capture unit with 76.2 mm ID absorber. At optimized operating conditions, the DP packing showed a relative 22.7% increase in absorption and 20.0% decrease in energy penalty.

中文翻译:

在台式集成 CO2 捕获系统中使用 3D 打印动态极性填料增强 CO2 吸收

使用化学吸收剂的燃烧后碳捕获是减少CO 2排放的有前途的技术。然而,总体建设和运营成本仍然是一个重大挑战。为了加强吸收过程并降低这些成本,已经开发了一种具有交替表面极性模式的新型动态极性规整填料(DP 填料),以增强先进粘性溶剂内的局部宏观尺度湍流,从而减少传质扩散反抗。使用 3D 打印技术制造了三种包含多种聚合物材料的 DP 规整填料,并通过使用小型集成 CO 2的参数测试进行了评估带有 76.2 毫米 ID 吸收器的捕获单元。在优化的操作条件下,DP 填料吸收增加了 22.7%,能量损失减少了 20.0%。
更新日期:2022-01-04
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