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Crossover behavior of the localized to itinerant transition of5felectrons in the antiferromagnetic Kondo latticeUSb2
Physical Review B ( IF 3.7 ) Pub Date : 2021-12-02 , DOI: 10.1103/physrevb.104.235103
W. Feng , D. H. Xie , X. B. Luo , S. Y. Tan , Y. Liu , Q. Liu , Q. Q. Hao , X. G. Zhu , Q. Zhang , Y. Zhang , Q. Y. Chen , X. C. Lai

In uranium-based heavy fermion systems, the 5f electrons display an intermediate character between partial localization and partial itinerancy, which makes the Kondo problem more complicated. Here we use scanning tunneling microscopy/spectroscopy to investigate the (001) surface of the Kondo lattice antiferromagnet USb2. Temperature-dependent dI/dV spectra from 4.7 K up to 140 K reveal several peak structures around the Fermi level. Two pronounced peaks originate from the hybridization between the conduction and 5f electrons. We did not observe the mysteriously abrupt change of the electronic state at 45 K, which was previously reported by another scanning tunneling microscopy group and attributed to a novel first-order-like transition. Instead, we only observe continuous evolution of the dI/dV spectra with temperature. Furthermore, in some scanning regions, we find significant Sb atoms missing from the top layer, which gives us the opportunity to investigate the electronic structure of the U-terminated surface. For the U-terminated surface, an additional sharp peak emerges, which is closely related to the magnetic order.

中文翻译:

反铁磁近藤晶格USb2中5f电子的局部到巡回跃迁的交叉行为

在铀基重费米子系统中, 5F电子显示出部分定位和部分巡回之间的中间特征,这使得 Kondo 问题更加复杂。在这里,我们使用扫描隧道显微镜/光谱来研究 Kondo 晶格反铁磁体的 (001) 表面USB2. 温度相关d一世/d从 4.7 K 到 140 K 的光谱揭示了费米能级周围的几个峰结构。两个明显的峰值源于传导和5F电子。我们没有观察到 45 K 时电子状态的神秘突然变化,这是另一个扫描隧道显微镜组先前报道的,并归因于一种新的类一阶跃迁。相反,我们只观察到d一世/d光谱与温度。此外,在某些扫描区域,我们发现顶层缺少大量的 Sb 原子,这使我们有机会研究 U 端表面的电子结构。对于 U 端表面,会出现一个额外的尖峰,这与磁序密切相关。
更新日期:2021-12-02
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