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Dynamics of reversible optical properties switching of Ge2Sb2Te5 thin films at laser-induced phase transitions
Optics & Laser Technology ( IF 4.6 ) Pub Date : 2021-11-23 , DOI: 10.1016/j.optlastec.2021.107701
Alexey V. Kiselev 1 , Vitaly V. Ionin 1 , Anton A. Burtsev 1 , Nikolai N. Eliseev 1 , Vladimir A. Mikhalevsky 1 , Natalya A. Arkharova 1 , Dmitry N. Khmelenin 1 , Andrey A. Lotin 1
Affiliation  

Paper presents the study of Ge2Sb2Te5 (GST) thin films phase transitions’ dynamics determined by the rate of their optical coefficients change. The phase transitions were initialized by laser pulses with 15 ns duration at a wavelength of 532 nm and confirmed by X-ray diffraction analysis. Energy fluence was 22 mJ/cm2 for film crystallization and 54 mJ/cm2 for reamorphization. The time for a complete change of GST film reflectivity associated with the crystallization process was 23 ns, while the time for a transmissivity change was 32 ns. Taking into account that the reflection is determined to a greater extent by the surface, and the transmission is exclusively by the film thickness, the estimated crystallization rate was ∼3.125 m/s. The time for a complete change in the reflectivity during the film reamorphization 62 ns, and the transmissivity changed in 65 ns. The estimated reamorphization rate was ∼1.538 m/s.



中文翻译:

Ge2Sb2Te5薄膜在激光诱导相变过程中可逆光学性质转换的动力学

本文介绍了 Ge 2 Sb 2 Te 5 (GST) 薄膜相变动力学的研究,由其光学系数变化率决定。相变由持续时间为 15 ns、波长为 532 nm 的激光脉冲初始化,并通过 X 射线衍射分析证实。膜结晶的能量注量为 22 mJ/cm 2和 54 mJ/cm 2用于重晶化。与结晶过程相关的 GST 膜反射率完全变化的时间为 23 ns,而透射率变化的时间为 32 ns。考虑到反射在很大程度上由表面决定,而透射仅由薄膜厚度决定,估计结晶速率为~3.125 m/s。薄膜再晶化过程中反射率完全变化的时间为 62 ns,透射率发生变化的时间为 65 ns。估计的重晶化速率约为 1.538 m/s。

更新日期:2021-11-23
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