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Quasi-one-dimensional superconductivity in the pressurized charge-density-wave conductor HfTe3
npj Quantum Materials ( IF 5.7 ) Pub Date : 2021-11-10 , DOI: 10.1038/s41535-021-00393-8
Z. Y. Liu 1, 2 , Y. Sui 1 , J. Li 2, 2, 3, 3 , P. T. Yang 2 , S. Zhang 2, 3 , G. F. Chen 2, 3 , H. X. Yang 2, 3 , J.-G. Cheng 2, 3 , J. F. Zhang 4 , K. Liu 4 , Y. Uwatoko 5
Affiliation  

HfTe3 single crystal undergoes a charge-density-wave (CDW) transition at TCDW = 93 K without the appearance of superconductivity (SC) down to 50 mK at ambient pressure. Here, we determined its CDW vector q = 0.91(1) a* + 0.27(1) c* via low-temperature transmission electron microscope and then performed comprehensive high-pressure transport measurements along three major crystallographic axes. Our results indicate that the superconducting pairing starts to occur within the quasi-one-dimensional (Q1D) -Te2-Te3- chain at 4–5 K but the phase coherence between the superconducting chains cannot be realized along either the b- or c-axis down to at least 1.4 K, giving rise to an extremely anisotropic SC rarely seen in real materials. We have discussed the prominent Q1D SC in pressurized HfTe3 in terms of the anisotropic Fermi surfaces arising from the unidirectional Te-5px electronic states and the local pairs formed along the -Te2-Te3- chains based on the first-principles electronic structure calculations.



中文翻译:

加压电荷密度波导体 HfTe3 中的准一维超导性

HfTe 3单晶在T CDW  = 93 K 时经历电荷密度波 (CDW) 跃迁,而在环境压力下低至 50 mK 时不会出现超导性 (SC)。在这里,我们通过低温透射电子显微镜确定了其 CDW 矢量q  = 0.91(1) a * + 0.27(1) c *,然后沿三个主要晶轴进行了全面的高压输运测量。我们的结果表明超导配对开始发生在准一维 (Q1D) -Te2-Te3- 链中,温度为 4-5 K,但超导链之间的相位相干无法沿b-c- 实现轴下降到至少 1.4 K,从而产生在真实材料中很少见的极其各向异性的 SC。我们已经讨论了加压 HfTe 3中突出的 Q1D SC,这涉及基于第一性原理电子结构计算的单向 Te-5p x电子态和沿 -Te2-Te3- 链形成的局部对产生的各向异性费米表面.

更新日期:2021-11-10
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