Superstructures of Organic–Polyoxometalate Co-crystals as Precursors for Hydrogen Evolution Electrocatalysts,Angewandte Chemie International Edition

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Superstructures of Organic–Polyoxometalate Co-crystals as Precursors for Hydrogen Evolution Electrocatalysts
Angewandte Chemie International Edition ( IF 16.1 ) Pub Date : 2021-10-28 , DOI: 10.1002/anie.202112298
Shuang Li _{1,

2} , Zhenyang Zhao ₂ , Tian Ma ₂ , Pradip Pachfule ₁ , Arne Thomas ₁

Affiliation

The synthesis of 2D mesoporous Mo carbides/nitrides for catalytic hydrogen production was realized by a series of organic–polyoxometalate co-crystals (O-POCs). These metal–organic precursors enable to create Mo-based electrocatalysts composed of abundant nanocrystallites and heterojunctions with tunable micro- and nanostructure and mesoporosity, therefore resulted in high HER activity and stability in both alkaline condition and seawater.

中文翻译：

有机多金属氧酸盐共晶的超结构作为析氢电催化剂的前驱体

通过一系列有机-多金属氧酸盐共晶（O-POC）实现了用于催化制氢的二维介孔碳化物/氮化物的合成。这些金属有机前体能够制造出由丰富的纳米微晶和异质结组成的钼基电催化剂，具有可调的微米和纳米结构以及介孔率，因此在碱性条件和海水中都具有高的HER活性和稳定性。

更新日期：2021-12-02

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