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Catalytic and inhibitory roles of K and Ca in the pyrolysis and CO2 or steam gasification of Erianthus, and their effects on co-gasification performance
Biomass & Bioenergy ( IF 5.8 ) Pub Date : 2021-10-20 , DOI: 10.1016/j.biombioe.2021.106257
Kenji Koido 1 , Kakeru Kurosawa 2 , Kenji Endo 3 , Michio Sato 3
Affiliation  

Increasing biomass demand for domestic power production due to feed-in tariffs has led to the use of herbaceous perennial energy crops such as Erianthus arundinaceus (Erianthus) as a biomass resource. Erianthus (JES1) is obtained in a yield of approximately 14 t/ha on a dry basis in Nasu-shiobara, a temperate climate region of Japan and its standing-dead characteristics permit a small drying cost. In this study, the catalytic roles of Ca and K on the CO2 and steam gasification of Erianthus char were investigated using thermogravimetry-differential thermal analysis (TG-DTA), and the effect of blending Erianthus with timber waste on the co-gasification performance was elucidated. The obtained results showed that the loading of K into the demineralised char (DC) enhanced both the CO2 and steam gasification processes. In contrast, the loading of Ca on DC slightly inhibited CO2 gasification, while steam gasification was significantly inhibited. In the co-gasification of an Erianthus-blended timber waste feedstock, the conversion to gas and cold-gas efficiency was promoted in the case of an Erianthus blend ≤30% due to the presence of inorganic components, such as K, in the blended feedstock.



中文翻译:

钾、钙在毛楸热解和CO2或蒸汽气化中的催化和抑制作用及其对共气化性能的影响

由于上网电价,国内电力生产对生物质的需求不断增加,导致使用多年生草本能源作物,如 Erianthus arundinaceus (Erianthus) 作为生物质资源。Erianthus (JES1) 在日本的温带气候地区那须盐原以干基的产量约为 14 吨/公顷,其立枯特性允许较低的干燥成本。在本研究中,使用热重-差热分析 (TG-DTA)研究了 Ca 和 K 对Erianthus char CO 2和蒸汽气化的催化作用,以及将 Erianthus 与木材废料混合对共气化性能的影响被阐明。获得的结果表明,将 K 负载到脱矿炭 (DC) 中增强了 CO 2和蒸汽气化过程。相比之下,DC上的Ca负载略微抑制了CO 2气化,而显着抑制了蒸汽气化。在 Erianthus 混合木材废料原料的共气化中,在 Erianthus 混合物≤30% 的情况下,由于混合中存在无机成分(如 K),促进了气体和冷气的转化效率原料。

更新日期:2021-10-21
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