• The unique 0D-2D ZnS nanodots/Ti₃C₂T_x MXene hybrids with strong interfacial interaction enable to achieve stable cyclability and excellent rate performance for lithium storage.

• The lithium storage mechanism of ZnS is clarified and new insights into phase transition mechanism are proposed.

• The strong interfacial interaction between ZnS nanodots and MXene nanosheets at the ZnS-MXene heterointerface exhibits high lithium adsorption capability, enhanced interfacial electron transfer, and low lithium diffusion energy barrier.

中文翻译：

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MOF 衍生的 ZnS 纳米点/Ti3C2Tx MXene 混合材料提升了卓越的锂存储性能

• 独特的0D-2D ZnS纳米点/Ti ₃ C ₂ T _x MXene杂化物具有强界面相互作用，可实现稳定的循环性和优异的锂存储倍率性能。

• 阐明了 ZnS 的锂存储机制，并提出了对相变机制的新见解。

• ZnS-MXene 异质界面处 ZnS 纳米点和 MXene 纳米片之间的强界面相互作用表现出高的锂吸附能力、增强的界面电子转移和低的锂扩散能垒。