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Solar-Driven Artificial Carbon Cycle
Chinese Journal of Chemistry ( IF 5.5 ) Pub Date : 2021-09-17 , DOI: 10.1002/cjoc.202100549
Chao Gao 1 , Yujie Xiong 1
Affiliation  

Constituting the artificial carbon cycle, for example, through recycling CO2 and converting CH4 to value-added fuels and chemicals with solar energy, offers a sustainable future for humankind to tackle the global environmental issues and energy crisis. However, significant bottlenecks remain in such photocatalytic conversion, mainly related to the reaction activity and product selectivity. Herein, we share our efforts and systematic research progress on addressing the double bottlenecks for achieving solar-driven artificial carbon cycle, with specifically focusing on the photocatalytic CO2 and CH4 conversion. We further elucidate the common fundamentals behind various designed photocatalytic materials systems. Toward future development, we highlight the opportunities and challenges in the research field.

中文翻译:

太阳能驱动的人工碳循环

例如,通过回收 CO 2并利用太阳能将 CH 4转化为增值燃料和化学品,构成人工碳循环,为人类解决全球环境问题和能源危机提供了一个可持续的未来。然而,这种光催化转化仍存在重大瓶颈,主要与反应活性和产物选择性有关。在此,我们分享了我们在解决实现太阳能驱动的人工碳循环的双重瓶颈方面的努力和系统研究进展,特别关注光催化 CO 2和 CH 4转换。我们进一步阐明了各种设计的光催化材料系统背后的共同基础。面向未来发展,我们强调研究领域的机遇和挑战。
更新日期:2021-09-17
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