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Surface acoustic device for high response NO2 gas sensor using p-phenylenediamine-reduced graphene oxide nanocomposite coated on langasite
Smart Materials and Structures ( IF 3.7 ) Pub Date : 2021-08-17 , DOI: 10.1088/1361-665x/ac1956
Jung-Bum Lim 1 , Maddaka Reddeppa 2 , Dongjin Nam 1 , Kedhareswara Sairam Pasupuleti 1 , Na-Hyun Bak 1 , Song-Gang Kim 3 , Hak Dong Cho 4 , Moon-Deock Kim 1, 2
Affiliation  

In this study, we fabricated a surface acoustic wave (SAW) device using a langasite (LGS) substrate. The p-phenylenediamine-reduced graphene oxide (PrGO)-coated LGS substrate resulted in high response sensor systems for very short time scale detection of NO2 and CO. With the catalytic reaction of PrGO, the resonant frequency of 100 ppm of NO2 gas changed by ∼3.50 kHz, which is nearly eight times higher than that of the pristine LGS SAW device. Further, we conducted selectivity tests for NO, NH3, H2S, and CO gases; the results showed that the PrGO-coated LGS had higher selectivity for NO2 compared to other gases. Accordingly, the underlying mechanism for the superior NO2 sensing was discussed in relation to the morphological characteristics and configuration of PrGO. In addition, the effect of humidity on the SAW performance was studied under ambient NO2.



中文翻译:

使用对苯二胺还原氧化石墨烯纳米复合材料涂覆在langasite上的用于高响应NO2气体传感器的表面声学装置

在这项研究中,我们使用 langasite (LGS) 衬底制造了表面声波 (SAW) 器件。对二胺还原氧化石墨烯 (PrGO) 涂层的 LGS 基板产生了高响应传感器系统,用于在非常短的时间内检测 NO 2和 CO。在 PrGO 的催化反应下,100 ppm NO 2气体的共振频率变化了~3.50 kHz,几乎是原始 LGS SAW 器件的 8 倍。此外,我们还对 NO、NH 3、H 2 S 和 CO 气体进行了选择性测试;结果表明,与其他气体相比,PrGO 涂层的 LGS 对 NO 2具有更高的选择性。因此,优越的 NO 2的潜在机制讨论了与 PrGO 的形态特征和配置相关的传感。此外,在环境 NO 2下研究了湿度对 SAW 性能的影响。

更新日期:2021-08-17
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