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Phonon Anomalies Associated with Spin Reorientation in the Kagome Ferromagnet Fe3Sn2
Physica Status Solidi (B) - Basic Solid State Physics ( IF 1.5 ) Pub Date : 2021-08-24 , DOI: 10.1002/pssb.202100169 Ge He 1 , Leander Peis 1 , Ramona Stumberger 1, 2 , Lilian Prodan 3 , Vladimir Tsurkan 3 , Nico Unglert 4 , Liviu Chioncel 4 , István Kézsmárki 3 , Rudi Hackl 1, 2
Physica Status Solidi (B) - Basic Solid State Physics ( IF 1.5 ) Pub Date : 2021-08-24 , DOI: 10.1002/pssb.202100169 Ge He 1 , Leander Peis 1 , Ramona Stumberger 1, 2 , Lilian Prodan 3 , Vladimir Tsurkan 3 , Nico Unglert 4 , Liviu Chioncel 4 , István Kézsmárki 3 , Rudi Hackl 1, 2
Affiliation
Polarization- and temperature-dependent Raman data along with theoretical simulations are presented for the Kagome ferromagnet . Eight out of nine expected phonon modes are identified. The experimental energies compare well with those from the simulations. The analysis of the line widths indicates relatively strong phonon–phonon coupling in the range 0.1–1. The temperature-dependent frequencies of three modes show weak anomalies at ≈100 K. In contrast, the linewidths of all phonon modes follow the conventional exponential broadening up to room temperature except for the softest mode, whose width exhibits a kink close to 100 K and becomes nearly constant for . These features are indicative of a spin reorientation taking place in the temperature range above 100 K, which might arise from spin–phonon coupling. The low-energy part of the electronic continuum in symmetry depends strongly on temperature. The possible reasons include particle–hole excitation tracking the resistivity, a spin-dependent gap, or spin fluctuations.
中文翻译:
Kagome 铁磁体 Fe3Sn2 中与自旋重定向相关的声子异常
为 Kagome 铁磁体提供了与极化和温度相关的拉曼数据以及理论模拟. 确定了九个预期声子模式中的八个。实验能量与模拟能量相比较。线宽的分析表明在 0.1-1 范围内的声子 - 声子耦合相对较强。三个温度相关的频率模式在 ≈100 K 处显示出微弱的异常。相反,所有声子模式的线宽都遵循常规的指数展宽至室温,除了最软的模式,其宽度表现出接近 100 K 的扭结,并且对于. 这些特征表明在 100 K 以上的温度范围内发生了自旋重新定向,这可能是由自旋 - 声子耦合引起的。电子连续体的低能部分对称性很大程度上取决于温度。可能的原因包括粒子-空穴激发跟踪电阻率、自旋相关间隙或自旋波动。
更新日期:2021-08-24
中文翻译:
Kagome 铁磁体 Fe3Sn2 中与自旋重定向相关的声子异常
为 Kagome 铁磁体提供了与极化和温度相关的拉曼数据以及理论模拟. 确定了九个预期声子模式中的八个。实验能量与模拟能量相比较。线宽的分析表明在 0.1-1 范围内的声子 - 声子耦合相对较强。三个温度相关的频率模式在 ≈100 K 处显示出微弱的异常。相反,所有声子模式的线宽都遵循常规的指数展宽至室温,除了最软的模式,其宽度表现出接近 100 K 的扭结,并且对于. 这些特征表明在 100 K 以上的温度范围内发生了自旋重新定向,这可能是由自旋 - 声子耦合引起的。电子连续体的低能部分对称性很大程度上取决于温度。可能的原因包括粒子-空穴激发跟踪电阻率、自旋相关间隙或自旋波动。