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Influences of different Bi2O3 additive amounts on static magnetic characteristics, micromorphology and ferromagnetic resonance linewidth of M-type Sr hexaferrites
Journal of Magnetism and Magnetic Materials ( IF 2.5 ) Pub Date : 2021-08-23 , DOI: 10.1016/j.jmmm.2021.168443
Yue Dai 1 , Zhongwen Lan 1 , Zhong Yu 1 , Ke Sun 1 , Xiaofeng Zhang 1 , Xiaona Jiang 1 , Chuanjian Wu 1 , Wei Tong 2
Affiliation  

Considering the improvement of electronics regarding high frequency and miniaturization, SrM hexaferrites need to exhibit high anisotropy field Ha, high remanence ratio Mr/Ms, and low ferromagnetic resonance linewidth ΔH to create microwave devices and equipment with planarisation, miniaturisation, and high frequencies. The key to achieving self-biased microwave devices with high-frequency is to simultaneously achieve high Ha, high Mr/Ms, and low ΔH. However, it is hard to meet these requirements. In this study, Sr0.4La0.3Ca0.3Fe11.85Al1.0Co0.15O19 was used to study the effect of different doping amounts of Bi2O3 on its magnetic characteristics, micromorphology and FMR linewidth. With the increase of Bi2O3 doping, the grain size of the sample gradually increased, and the uniformity of the grain size gradually decreased. When the Bi2O3 doping amount x increased from 0 to 1.2 wt%, the 4πMs and 4πMr values increased and the coercivity displayed the opposite tendency. The samples showed great uniaxial anisotropy. The magnetocrystalline anisotropy field Ha shows a trend of initially decreased and then increased. When x = 1.0 wt%, Ha reaches the maximum value of 28.9 kOe. At this time, the ferromagnetic resonance linewidth ΔH of the sample is 1578 Oe. The theory of IGA was adopted to divide the FMR linewidth into two parts ΔHa and ΔHp. Accroding to the results, ΔHa takes the bigger proportion of linewidth. However, the change in ΔHp is not negligible. When x = 1.0 wt%, the sample showed its best performance (4πMs = 3412 Gs, 4πMr = 2905 Gs, Hc = 2649 Oe, Mr/Ms = 85.1%, large Ha = 28.864 kOe, and ΔH = 1578 Oe). The SrM ferrite materials provided in this study can potentially be used in the microwave engineering, high-frequency, and self-biased devices.



中文翻译:

不同Bi2O3添加量对M型Sr六铁氧体静磁特性、微观形貌和铁磁共振线宽的影响

考虑到电子器件在高频和小型化方面的改进,SrM 六铁氧体需要表现出高各向异性场H a、高剩磁比M r / M s和低铁磁共振线宽 Δ H以创建具有平面化、小型化和高频。实现高频自偏置微波器件的关键是同时实现高H a、高M r / M s和低Δ H。但是,要满足这些要求是很困难的。在本研究中,Sr 0.4 La0.3 Ca 0.3 Fe 11.85 Al 1.0 Co 0.15 O 19用于研究不同Bi 2 O 3掺杂量对其磁特性、微观形貌和FMR线宽的影响。随着Bi 2 O 3掺杂量的增加,样品的晶粒尺寸逐渐增大,晶粒尺寸的均匀性逐渐降低。当 Bi 2 O 3掺杂量x从 0 增加到 1.2 wt% 时,4π M s和 4π M r值增加,矫顽力显示出相反的趋势。样品显示出很大的单轴各向异性。晶磁各向异性场H a呈现先减小后增大的趋势。当x  = 1.0 wt% 时,H a达到最大值 28.9 kOe。此时,样品的铁磁共振线宽ΔH为1578 Oe。采用IGA理论将FMR线宽分为ΔH a和Δ H p两部分。根据结果​​,Δ H a占线宽的比例较大。然而,ΔH p的变化不容忽视。当x  = 1.0 wt%时,样品表现出最佳性能(4π M s  = 3412 Gs,4π M r  = 2905 Gs,H c  = 2649 Oe,M r / M s  = 85.1%,大H a  = 28.864 kOe,和 Δ H  = 1578 Oe)。本研究中提供的 SrM 铁氧体材料可用于微波工程、高频和自偏置器件。

更新日期:2021-09-04
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