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The Impact of Ligand Carboxylates on Electrocatalyzed Water Oxidation
Accounts of Chemical Research ( IF 16.4 ) Pub Date : 2021-08-17 , DOI: 10.1021/acs.accounts.1c00298 Biswanath Das 1 , Ahibur Rahaman 1 , Andrey Shatskiy 2 , Oscar Verho 3 , Markus D Kärkäs 2 , Björn Åkermark 1
Accounts of Chemical Research ( IF 16.4 ) Pub Date : 2021-08-17 , DOI: 10.1021/acs.accounts.1c00298 Biswanath Das 1 , Ahibur Rahaman 1 , Andrey Shatskiy 2 , Oscar Verho 3 , Markus D Kärkäs 2 , Björn Åkermark 1
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Fossil fuel shortage and severe climate changes due to global warming have prompted extensive research on carbon-neutral and renewable energy resources. Hydrogen gas (H2), a clean and high energy density fuel, has emerged as a potential solution for both fulfilling energy demands and diminishing the emission of greenhouse gases. Currently, water oxidation (WO) constitutes the bottleneck in the overall process of producing H2 from water. As a result, the design of efficient catalysts for WO has become an intensively pursued area of research in recent years. Among all the molecular catalysts reported to date, ruthenium-based catalysts have attracted particular attention due to their robust nature and higher activity compared to catalysts based on other transition metals.
中文翻译：
配体羧酸盐对电催化水氧化的影响
由于全球变暖，化石燃料短缺和严重的气候变化促使人们对碳中和和可再生能源进行了广泛的研究。氢气 (H 2 ) 是一种清洁且能量密度高的燃料，已成为满足能源需求和减少温室气体排放的潜在解决方案。目前，水氧化（WO）构成了从水中生产H 2的整个过程的瓶颈。因此，设计用于 WO 的高效催化剂已成为近年来备受关注的研究领域。在迄今为止报道的所有分子催化剂中，与基于其他过渡金属的催化剂相比，基于钌的催化剂因其稳健的性质和更高的活性而受到特别关注。
更新日期：2021-09-07
中文翻译：
配体羧酸盐对电催化水氧化的影响
由于全球变暖，化石燃料短缺和严重的气候变化促使人们对碳中和和可再生能源进行了广泛的研究。氢气 (H 2 ) 是一种清洁且能量密度高的燃料，已成为满足能源需求和减少温室气体排放的潜在解决方案。目前，水氧化（WO）构成了从水中生产H 2的整个过程的瓶颈。因此，设计用于 WO 的高效催化剂已成为近年来备受关注的研究领域。在迄今为止报道的所有分子催化剂中，与基于其他过渡金属的催化剂相比，基于钌的催化剂因其稳健的性质和更高的活性而受到特别关注。
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