npj Climate and Atmospheric Science ( IF 8.5 ) Pub Date : 2021-08-17 , DOI: 10.1038/s41612-021-00200-y Huang Zheng 1, 2 , Shaofei Kong 1, 2, 3 , Zewei Fan 1 , Ying Zhang 1 , Liquan Yao 1, 2 , Yi Cheng 1, 2 , Shurui Zheng 1, 2 , Yingying Yan 1 , Shihua Qi 2 , Nan Chen 3, 4 , Dantong Liu 5 , Delong Zhao 6 , Chao Liu 7 , Tianliang Zhao 7 , Jianping Guo 8
The result of Aethalometer model to black carbon (BC) source apportionment is highly determined by the absorption Ångström exponent (α) of aerosols from fossil fuel combustion (αff) and wood burning (αwb). A method using hourly measured potassium to calculate the αff and αwb values was developed in this study. Results showed that the optimal αff and αwb were 1.09 and 1.79 for the whole dataset. The optimal α values in the diurnal resolution were also calculated with αff and αwb varied in 1.02 –1.19 and 1.71–1.90, respectively. Using the dynamic α values, the Pearson correlation coefficient between BC and potassium from wood burning substantially improved compared to the results derived from the fixed α values. The method developed in this study is expected to provide more reasonable BC source identification results, which are helpful for air quality, climate, and human health modeling studies.
中文翻译:
一种在线监测钾离子动态约束黑碳气溶胶源的方法
Aethalometer模型黑碳(BC)源解析的结果是高度由吸收埃指数(确定α来自化石燃料燃烧的气溶胶)(α FF)和木材燃烧(α WB)。本研究开发了一种使用每小时测量的钾来计算α ff和α wb值的方法。结果表明,整个数据集的最佳α ff和α wb分别为 1.09 和 1.79。也用α ff和α wb计算了昼夜分辨率中的最佳α值分别在 1.02-1.19 和 1.71-1.90 之间变化。使用动态α值,与来自固定α值的结果相比,BC 和木材燃烧产生的钾之间的 Pearson 相关系数显着提高。本研究开发的方法有望提供更合理的BC源识别结果,有助于空气质量、气候和人类健康建模研究。