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Spin Hall effect in a spin-1 chiral semimetal
Physical Review Research ( IF 3.5 ) Pub Date : 2021-07-29 , DOI: 10.1103/physrevresearch.3.033101
Ke Tang 1, 2 , Yong-Chang Lau 3, 4 , Kenji Nawa 1, 5 , Zhenchao Wen 1 , Qingyi Xiang 1 , Hiroaki Sukegawa 1 , Takeshi Seki 3, 4 , Yoshio Miura 1 , Koki Takanashi 3, 4, 6 , Seiji Mitani 1, 2
Affiliation  

The spin-1 chiral semimetal is a state of quantum matter hosting unconventional chiral fermions that extend beyond the common Dirac and Weyl fermions. B20-type CoSi is a prototypal material that accommodates such an exotic quasiparticle. To date, the spin-transport properties in the spin-1 chiral semimetals have not been thoroughly explored. In this work, we fabricated B20-CoSi thin films on sapphire c-plane substrates by magnetron sputtering and studied the spin Hall effect (SHE) by combining experiments and first-principles calculations. The SHE of CoSi was investigated using CoSi/CoFeB/MgO heterostructures via spin Hall magnetoresistance and harmonic Hall measurements. First-principles calculations yield an intrinsic spin Hall conductivity (SHC) at the Fermi level that is consistent with the experiments and reveal its unique Fermi-energy dependence. Unlike the Dirac and Weyl fermion-mediated Hall conductivities that exhibit a peaklike structure centering around the topological node, SHC of B20-CoSi is odd and crosses zero at the node with two antisymmetric local extrema of opposite sign situated below and above in energy. Hybridization between Co d-Si p orbitals and spin-orbit coupling are essential for the SHC, despite the small (∼1%) weight of the Si p orbital near the Fermi level. This work expands the horizon of topological spintronics and highlights the importance of Fermi-level tuning in order to fully exploit the topology of spin-1 chiral fermions for spin-current generation.

中文翻译:

自旋 1 手性半金属中的自旋霍尔效应

自旋 1 手性半金属是一种量子物质状态,包含非常规手性费米子,超出了常见的狄拉克和外尔费米子。B 20 型 CoSi 是一种原型材料,可以容纳这种奇异的准粒子。迄今为止,spin-1 手性半金属的自旋输运特性尚未得到彻底探索。在这项工作中,我们在蓝宝石上制造了B 20-CoSi 薄膜C通过磁控溅射制备-平面衬底,并结合实验和第一性原理计算研究了自旋霍尔效应(SHE)。通过自旋霍尔磁阻和谐波霍尔测量,使用 CoSi/CoFeB/MgO 异质结构研究 CoSi 的 SHE。第一性原理计算得出费米能级的固有自旋霍尔电导率 (SHC),这与实验一致,并揭示了其独特的费米能量依赖性。与表现出以拓扑节点为中心的峰状结构的 Dirac 和 Weyl 费米子介导的霍尔电导率不同,B 20-CoSi 的SHC是奇数,并在节点处与零交叉,具有位于能量下方和上方的两个符号相反的反对称局部极值。Co之间的杂交d-Si 尽管 Si 的重量很小(~1%),但轨道和自旋轨道耦合对于 SHC 来说是必不可少的 费米能级附近的轨道。这项工作扩展了拓扑自旋电子学的视野,并强调了费米能级调谐的重要性,以便充分利用自旋 1 手性费米子的拓扑结构来产生自旋电流。
更新日期:2021-07-29
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