Advanced Materials for Energy-Water Systems: The Central Role of Water/Solid Interfaces in Adsorption, Reactivity, and Transport,Chemical Reviews

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Advanced Materials for Energy-Water Systems: The Central Role of Water/Solid Interfaces in Adsorption, Reactivity, and Transport
Chemical Reviews ( IF 51.4 ) Pub Date : 2021-07-02 , DOI: 10.1021/acs.chemrev.1c00069
Edward Barry _{1,

2,

3} , Raelyn Burns _{1,

2} , Wei Chen _{1,

3,

4,

5} , Guilhem X De Hoe _{1,

3,

4,

5} , Joan Manuel Montes De Oca _{1,

5} , Juan J de Pablo _{1,

4,

5} , James Dombrowski _{1,

6} , Jeffrey W Elam _{1,

2,

3} , Alanna M Felts _{1,

7} , Giulia Galli _{1,

4,

5} , John Hack _{1,

8} , Qiming He _{1,

3,

4,

5} , Xiang He _{1,

9} , Eli Hoenig _{1,

5} , Aysenur Iscen _{1,

6} , Benjamin Kash ₅ , Harold H Kung _{1,

6} , Nicholas H C Lewis _{1,

8} , Chong Liu _{1,

5} , Xinyou Ma _{1,

8} , Anil Mane _{1,

2} , Alex B F Martinson _{1,

3,

4} , Karen L Mulfort _{1,

9} , Julia Murphy _{1,

8} , Kristian Mølhave _{1,

10} , Paul Nealey _{1,

4,

5} , Yijun Qiao _{1,

3,

4} , Vepa Rozyyev _{1,

2} , George C Schatz _{1,

7} , Steven J Sibener _{1,

8} , Dmitri Talapin _{1,

8} , David M Tiede _{1,

9} , Matthew V Tirrell _{1,

3,

4,

5} , Andrei Tokmakoff _{1,

8} , Gregory A Voth _{1,

8} , Zhongyang Wang _{1,

5} , Zifan Ye _{1,

5} , Murat Yesibolati _{1,

10} , Nestor J Zaluzec _{1,

11} , Seth B Darling _{1,

3,

5,

9}

Affiliation

Advanced Materials for Energy-Water Systems (AMEWS) Energy Frontier Research Center (EFRC), Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.
Applied Materials Division, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.
Center for Molecular Engineering, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.
Materials Science Division, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.
Pritzker School of Molecular Engineering, University of Chicago, 5640 South Ellis Avenue, Chicago, Illinois 60637 United States.
Department of Chemical and Biological Engineering, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208 United States.
Department of Chemistry, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208 United States.
Department of Chemistry, University of Chicago, 5735 South Ellis Avenue, Chicago, Illinois 60637 United States.
Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.
Technical University of Denmark, Anker Engelunds Vej 1 Bygning 101A, Kgs. Lyngby, Lyngby, Hovedstaden 2800, DK Denmark.
Photon Sciences Directorate, Argonne National Laboratory, 9700 South Cass Avenue, Lemont, Illinois 60439 United States.

The structure, chemistry, and charge of interfaces between materials and aqueous fluids play a central role in determining properties and performance of numerous water systems. Sensors, membranes, sorbents, and heterogeneous catalysts almost uniformly rely on specific interactions between their surfaces and components dissolved or suspended in the water—and often the water molecules themselves—to detect and mitigate contaminants. Deleterious processes in these systems such as fouling, scaling (inorganic deposits), and corrosion are also governed by interfacial phenomena. Despite the importance of these interfaces, much remains to be learned about their multiscale interactions. Developing a deeper understanding of the molecular- and mesoscale phenomena at water/solid interfaces will be essential to driving innovation to address grand challenges in supplying sufficient fit-for-purpose water in the future. In this Review, we examine the current state of knowledge surrounding adsorption, reactivity, and transport in several key classes of water/solid interfaces, drawing on a synergistic combination of theory, simulation, and experiments, and provide an outlook for prioritizing strategic research directions.

中文翻译：

能源-水系统的先进材料：水/固体界面在吸附、反应和传输中的核心作用

材料和水性流体之间界面的结构、化学和电荷在确定众多水系统的特性和性能方面发挥着核心作用。传感器、膜、吸附剂和非均相催化剂几乎一致地依赖其表面与溶解或悬浮在水中的组分（通常是水分子本身）之间的特定相互作用来检测和减轻污染物。这些系统中的有害过程，例如结垢、结垢（无机沉积物）和腐蚀，也受界面现象的支配。尽管这些接口很重要，但关于它们的多尺度交互仍有许多需要了解。深入了解水/固体界面处的分子和中尺度现象对于推动创新以应对未来在提供足够的适合用途的水方面面临的巨大挑战至关重要。在这篇综述中，我们利用理论、模拟和实验的协同组合，研究了在几个关键类别的水/固体界面中吸附、反应性和传输的当前知识状态，并为优先战略研究方向提供了展望.

更新日期：2021-08-11

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