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Improved triethylamine sensing properties of fish-scale-like porous SnO2 nanosheets by decorating with Ag nanoparticles
Journal of Materiomics ( IF 8.4 ) Pub Date : 2021-06-24 , DOI: 10.1016/j.jmat.2021.06.005
Jingyi Zhang 1, 2 , Bowen Zhang 1, 2 , Shujuan Yao 1, 2 , Hongyuan Li 1, 2 , Can Chen 1, 2 , Hari Bala 1, 2 , Zhanying Zhang 1, 2
Affiliation  

Three dimensional (3D) porous nanostructures assembled by low-dimensional nanomaterials are widely applied in gas sensor according to porous structure which can facilitate the transport of gas molecules. In this work, fish-scale-like porous SnO2 nanomaterials assembled from ultrathin nanosheets with thickness of 16.8 nm were synthesized by a facile hydrothermal route. Then Ag nanoparticles were decorated on the surface of SnO2 nanosheets via one-step method to improve their gas-sensing performances. The sensing properties of pristine SnO2 and Ag/SnO2 nanosheets were investigated intensively. After decorating with Ag nanoparticles, the characteristics of SnO2 based sensor for triethylamine detection were significantly improved. Especially, the Ag/SnO2 based sensor with Ag content of 2 at% exhibited the highest triethylamine sensing sensitivity at optimum work temperature of 170 °C. The improved sensing properties of Ag/SnO2 sensors were attributed to the sensitizing actions of Ag nanoparticles as well as the unique hierarchical porous architecture.



中文翻译:

Ag纳米粒子修饰改善鱼鳞状多孔SnO2纳米片的三乙胺传感性能

由低维纳米材料组装而成的三维(3D)多孔纳米结构根据多孔结构可促进气体分子的传输,广泛应用于气体传感器。在这项工作中,通过简便的水热路线合成了由厚度为16.8 nm的超薄纳米片组装而成的鱼鳞状多孔SnO 2纳米材料。然后通过一步法将Ag纳米颗粒修饰在SnO 2纳米片的表面以提高其气敏性能。对原始SnO 2和Ag/SnO 2纳米片的传感特性进行了深入研究。用Ag纳米粒子装饰后,SnO 2的特性基于传感器的三乙胺检测得到显着改善。特别是Ag含量为2 at%的Ag/SnO 2基传感器在170 ℃的最佳工作温度下表现出最高的三乙胺传感灵敏度。Ag/SnO 2传感器的改进传感特性归因于Ag纳米颗粒的敏化作用以及独特的分层多孔结构。

更新日期:2021-06-24
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