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Electrical and structural properties of VO2 in an electric field
Current Applied Physics ( IF 2.4 ) Pub Date : 2021-06-10 , DOI: 10.1016/j.cap.2021.05.010
In-Hui Hwang , Zhenlan Jin , Chang-In Park , Cheng-Jun Sun , Dale L. Brewe , Sang-Wook Han

We examined the electrical and local structural properties of a VO2 film at different electric fields using electrical resistance and x-ray absorption fine structure (XAFS) measurements at the V K edge in the temperature range of 30–100 °C. The Tc value of the metal-to-insulator transition (MIT) during both heating and cooling decreases with electric field. When the electric field exceeds a certain value, the MIT becomes sharper due to Joule heating. The MIT, the structural phase transition (SPT), and the pre-edge peak transition of the VO2 do not congruently occur at a uniform temperature. A metallic VO2 is observed in only the rutile (or M2) symmetry. An electric field induces a substantial amount of conduction electrons in insulating VO2. Simultaneously measured resistance and XAFS reveal that Joule heating caused by an external electric field significantly affects the MIT and SPT of VO2.



中文翻译:

VO 2在电场中的电学和结构特性

我们在 30–100 °C 的温度范围内使用电阻和 X 射线吸收精细结构 (XAFS) 在 VK 边缘测量不同电场下VO 2薄膜的电学和局部结构特性。在加热和冷却过程中,金属到绝缘体转变 (MIT)的 T c值随着电场的增加而降低。当电场超过某个值时,由于焦耳热,MIT 变得更尖锐。MIT、结构相变 (SPT) 和 VO 2的前边缘峰转变不会在均匀温度下一致发生。金属 VO 2仅在金红石(或 M2)对称性中观察到。电场在绝缘的VO 2 中感应出大量的传导电子。同时测量的电阻和 XAFS 表明,由外部电场引起的焦耳热显着影响 VO 2的 MIT 和 SPT 。

更新日期:2021-06-10
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