当前位置: X-MOL 学术J. Phys. D: Appl. Phys. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Millimeter-scale growth of highly ordered CsPbBr3 single-crystalline microplatelets on SiO2/Si substrate by chemical vapor deposition
Journal of Physics D: Applied Physics ( IF 3.4 ) Pub Date : 2021-06-08 , DOI: 10.1088/1361-6463/ac0463
Jiepeng Song 1 , Chun Li 1, 2 , Qiuyu Shang 1 , Yuxuan Ke 1 , Liyun Zhao 1 , Yin Liang 1 , Li Zhang 1, 3 , Qing Zhang 1
Affiliation  

Recently, all-inorganic cesium lead bromide (CsPbBr3) perovskite has attracted tremendous interest due to its promise for green light photonic and optoelectronic devices. The growth of high-quality planar micro-/nano-structures of CsPbBr3 on the technologically important silicon substrate is an important issue for these applications, which has not yet been well explored. Herein we fabricate millimeter-scale single-crystalline CsPbBr3 microplatelets (MPs) on SiO2/Si substrate by chemical vapor deposition. A preferred growth direction is demonstrated with the [110] direction parallel to the flux direction of carrier gas. Strong green emission is observed at room temperature with superior photo-stability, long lifetime, and excitonic features. Furthermore, the room temperature whispering-gallery-mode lasing is achieved from the focused ion beam fabricated microdisks with the thresholds comparable to those of pristine square MPs. These results suggest the great potentials of CsPbBr3 MPs for the Si-based photonic devices.



中文翻译:

通过化学气相沉积在 SiO2/Si 衬底上毫米级生长高度有序的 CsPbBr3 单晶微片

最近,全无机溴化铯铅 (CsPbBr 3 ) 钙钛矿因其在绿光光子和光电器件方面的前景而引起了极大的兴趣。在技​​术上重要的硅衬底上生长高质量的 CsPbBr 3平面微/纳米结构是这些应用的一个重要问题,尚未得到很好的探索。在此,我们在 SiO 2上制造毫米级单晶 CsPbBr 3微片 (MPs)/Si衬底通过化学气相沉积。优选的生长方向用平行于载气流动方向的[110]方向证明。在室温下观察到强烈的绿色发射,具有优异的光稳定性、长寿命和激子特征。此外,室温回音壁模式激光是通过聚焦离子束制造的微盘实现的,其阈值与原始方形 MP 的阈值相当。这些结果表明 CsPbBr 3 MPs 在 Si 基光子器件中的巨大潜力。

更新日期:2021-06-08
down
wechat
bug