The current needs of finding more efficient materials with tunable properties have served as a motivation for the scientific community to move toward nature-inspired hierarchical materials adhering to the green analytical chemistry principles also because of the high complexity and efficiency of systems in nature. Such type of materials has exhibited highly dynamic interfacial interactions, which are outstandingly valuable for sensing and energy storage applications. Nature-based systems have displayed remarkable features, in terms of energy density, coulombic efficiency behavior, cycling stability energy, durability, and sensitivity. More interestingly, the aforementioned properties could be tuned by modifying the interfacial interactions within the material components. Along this contribution, recent developments on the design of green analytical nature-inspired hierarchical materials will be addressed, especially paying attention to the relationship between interfacial interactions and material features.

由于自然界中系统的高度复杂性和效率，当前寻找具有可调特性的更有效材料的需求已成为科学界转向遵循绿色分析化学原理的受自然启发的分层材料的动力。这种类型的材料表现出高度动态的界面相互作用，这对于传感和储能应用非常有价值。基于自然的系统在能量密度、库伦效率行为、循环稳定性能、耐久性和灵敏度方面表现出显着的特征。更有趣的是，可以通过修改材料组分内的界面相互作用来调整上述特性。伴随着这一贡献，