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Tunable fabrication of single-crystalline CsPbI3 nanobelts and their application as photodetectors
International Journal of Minerals, Metallurgy and Materials ( IF 5.6 ) Pub Date : 2021-06-05 , DOI: 10.1007/s12613-020-2173-2
Tao Yang , Ya-peng Zheng , Kuo-Chih Chou , Xin-mei Hou

Lead halide perovskites have received increasing attention recently as a candidate material in various optoelectronic areas because of their high performance as light absorbers. Herein, we report the growth of CsPbI3 nanobelts via a solution process. A single-crystalline CsPbI3 nanobelt with uniform morphology can be achieved by controlling the amount of PbI2. A single-crystalline CsPbI3 nanobelt possesses a mean width, length, and thickness of 100 nm, 5 µm, and 20 nm, respectively. In this work, photodetectors (PDs) based on individual CsPbI3 nanobelts are constructed and found to perform well with an external quantum efficiency and responsivity of 2.39 × 105% and 770 A/W, respectively. The PDs also show a high detectivity of up to 3.12 × 1012 Jones, which is at par with that of Si PDs. The PDs developed in this work exhibit great promise in various optoelectronic nanodevices.



中文翻译:

单晶 CsPbI3 纳米带的可调制造及其作为光电探测器的应用

由于其作为光吸收剂的高性能,卤化铅钙钛矿最近作为各种光电领域的候选材料受到越来越多的关注。在此,我们报告了 CsPbI 3纳米带通过溶液过程的生长。通过控制PbI 2的量可以实现具有均匀形态的单晶CsPbI 3纳米带。单晶 CsPbI 3纳米带的平均宽度、长度和厚度分别为 100 nm、5 µm 和 20 nm。在这项工作中,构建了基于单个 CsPbI 3纳米带的光电探测器 (PD)并发现其性能良好,外部量子效率和响应度为 2.39 × 10 5% 和 770 A/W,分别。PD 还显示出高达 3.12 × 10 12 Jones的高探测率,与 Si PD 相当。在这项工作中开发的 PD 在各种光电纳米器件中表现出巨大的潜力。

更新日期:2021-06-05
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