当前位置: X-MOL 学术Intermetallics › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Double magnetic phase transitions and magnetotransport anomalies in a new compound Gd2AgSi3
Intermetallics ( IF 4.3 ) Pub Date : 2021-05-16 , DOI: 10.1016/j.intermet.2021.107214
Baidyanath Sahu , R. Djoumessi Fobasso , André M. Strydom

Dc and acmagnetic susceptibility (χ), specific heat (CP), electrical resistivity (ρ) and magnetoresistance measurements performed on the new polycrystalline compound Gd2AgSi3, crystallizing in the αThSi2 tetragonal structure, are reported. Two magnetic phase transitions were observed in dc and ac susceptibility, specific heat and resistivity measurements at temperatures TN1=11 K and TN2=20 K, despite a single site occupied by Gd atom, which is an indication of the complex magnetic behavior. Gd2AgSi3 turns out be one of the rare Gd compound in which a minimum is observed in the temperature dependence of resistivity in the paramagnetic state and also negative magnetoresistance over a wide temperature range (above TN2), mimicking the behavior of exotic Gd2PdSi3, in this ternary family. The isothermal magnetic entropy change, adiabatic temperature change, and refrigerant capacity reach a value of 9.5 J/kg-K, 7.5 K and 302 J/kg, respectively for the change of magnetic field 0-9 T.



中文翻译:

新型化合物Gd 2 AgSi 3中的双磁相变和磁输运异常

直流和交流磁化率(χ),比热(CP),对新的多晶化合物进行的电阻率(ρ)和磁阻测量 d2个银硅3,在α中结晶2个四角形结构,已有报道。在直流和交流磁化率,比热和温度下的电阻率测量中观察到两个磁性相变Ťñ1个=11 K和 Ťñ2个=20 尽管有单个位点被Gd原子占据,但K仍是K,这表明了复杂的磁行为。 d2个银硅3 成为稀有的Gd化合物之一,其中在顺磁状态下的电阻率与温度的相关性最小,并且在较宽的温度范围内也具有负磁阻(以上) Ťñ2个),模仿异国情调的行为 d2个钯硅3在这个三元家庭中 磁场0-9 T的变化,等温磁熵变,绝热温度变化和制冷剂容量分别达到9.5 J / kg-K,7.5 K和302 J / kg。

更新日期:2021-05-17
down
wechat
bug