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Modelling the dependence of equivalent dose determined from a dose recovery test on preheating temperature: The intervention of shallow electron traps
Radiation Measurements ( IF 1.6 ) Pub Date : 2021-03-18 , DOI: 10.1016/j.radmeas.2021.106566
Jun Peng , Xulong Wang , Grzegorz Adamiec , Vasilis Pagonis , Jeong-Heon Choi

In optically stimulated luminescence (OSL) dating, the performance of the single-aliquot regenerative-dose (SAR) protocol is commonly tested using a dose recovery test. The dependence of equivalent dose (De) determined in a dose recovery test on preheating temperature using quartz OSL was reported in previous studies which demonstrated that using a lower preheating temperature prior to the measurement of the test dose OSL response may result in serious underestimation of the recovered De. In this study, we simulate the variation of normalised sensitivity-corrected OSL signals as a function of cycle number and the dependence of the recovered De on preheating conditions, using a kinetic model consisting of four electron traps and two recombination centres. Experimentally observed phenomena are successfully reproduced using the model with a set of optimised kinetic parameters. We suggest that the intervention of shallow electron traps may play a significant role in affecting the accuracy of De determination. Relevant mechanisms are explained, and implications on dose measurements using the SAR protocol are discussed.



中文翻译:

模拟剂量恢复测试确定的等效剂量对预热温度的依赖性:浅电子陷阱的干预

在光学激发发光(OSL)测年中,通常使用剂量恢复测试来测试单等分再生剂量(SAR)协议的性能。先前的研究报道了使用石英OSL在剂量恢复测试中确定的等效剂量(D e)对预热温度的依赖性,这表明在测量测试剂量OSL响应之前使用较低的预热温度可能会严重低估恢复的D e。在这项研究中,我们模拟归一化灵敏度校正的OSL信号随循环次数的变化以及所恢复的D e的依赖性在预热条件下,使用由四个电子陷阱和两个复合中心组成的动力学模型。使用具有一组优化动力学参数的模型,可以成功地复制实验观察到的现象。我们建议浅电子陷阱的干预可能在影响D e测定的准确性中起重要作用。解释了相关的机制,并讨论了使用SAR协议进行剂量测量的意义。

更新日期:2021-03-22
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