The reverse water gas shift reaction: a process systems engineering perspective,Reaction Chemistry & Engineering

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The reverse water gas shift reaction: a process systems engineering perspective
Reaction Chemistry & Engineering ( IF 3.4 ) Pub Date : 2021-3-10 , DOI: 10.1039/d0re00478b
Miriam González-Castaño _{1,

2,

3,

4} , Bogdan Dorneanu _{1,

2,

3,

4} , Harvey Arellano-García _{1,

2,

3,

4}

Affiliation

The catalytic reduction of CO₂ into value-added products has been considered a compelling solution for alleviating global warming and energy crises. The reverse water gas shift (RWGS) reaction plays a pivotal role among the various CO₂ utilization approaches, due to the fact that it produces syngas, the building block of numerous conversion processes. Although a lot of work has been carried out towards the development of a RWGS process, ranging from efficient catalytic systems to reactor units, and even pilot scale processes, there is still a lack of understanding of the fundamental phenomena that take place at the various levels and scales of the process. This contribution presents the main solutions and remaining challenges for a structured, trans- and multidisciplinary framework in which catalysis engineering and process systems engineering can work together to incorporate understanding and methods from both sides, to accelerate the investigation, creation and operation of an efficient industrial CO₂ conversion process based on the RWGS reaction.

中文翻译：

反向水煤气变换反应：过程系统工程学的观点

将CO ₂催化还原成增值产品被认为是缓解全球变暖和能源危机的有效解决方案。反向水煤气变换（RWGS）反应在各种CO _2中起着关键作用由于它会产生合成气，这是许多转化过程的基础，因此采用了多种利用方法。尽管为开发RWGS工艺进行了大量工作，从有效的催化系统到反应器装置，甚至是中试规模的工艺，但仍然缺乏对各个层面发生的基本现象的理解。和过程的规模。这项贡献提出了结构化，跨学科和多学科框架的主要解决方案和尚待解决的挑战，在该框架中，催化工程和工艺系统工程可以协同工作，将双方的理解和方法结合起来，以加快高效工业的研究，创建和运营一氧化碳₂ 基于RWGS反应的转化过程。

更新日期：2021-03-16

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